Three-Dimensional Nondestructive Isotope-Selective Tomographic Imaging of <sup>208</sup>Pb Distribution via Nuclear Resonance Fluorescence

Combining the nuclear resonance fluorescence (NRF) transmission method with computed tomography (CT) can be a novel method for imaging the isotope distributions, which is indispensable in nuclear engineering. We performed an experiment to reconstruct a three-dimensional NRF-CT image with isotope sel...

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Main Authors: Khaled Ali, Heishun Zen, Hideaki Ohgaki, Toshiteru Kii, Takehito Hayakawa, Toshiyuki Shizuma, Hiroyuki Toyokawa, Masaki Fujimoto, Yoshitaka Taira, Masahiro Katoh
Format: Article
Language:English
Published: MDPI AG 2021-04-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/11/8/3415
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author Khaled Ali
Heishun Zen
Hideaki Ohgaki
Toshiteru Kii
Takehito Hayakawa
Toshiyuki Shizuma
Hiroyuki Toyokawa
Masaki Fujimoto
Yoshitaka Taira
Masahiro Katoh
author_facet Khaled Ali
Heishun Zen
Hideaki Ohgaki
Toshiteru Kii
Takehito Hayakawa
Toshiyuki Shizuma
Hiroyuki Toyokawa
Masaki Fujimoto
Yoshitaka Taira
Masahiro Katoh
author_sort Khaled Ali
collection DOAJ
description Combining the nuclear resonance fluorescence (NRF) transmission method with computed tomography (CT) can be a novel method for imaging the isotope distributions, which is indispensable in nuclear engineering. We performed an experiment to reconstruct a three-dimensional NRF-CT image with isotope selectivity of enriched lead isotope rods (<sup>208</sup>Pb) together with a set of different rods, including another enriched isotope (<sup>206</sup>Pb), iron, and aluminum rods, inserted into a cylindrical aluminum holder. Using a laser Compton scattering (LCS) gamma ray beam with a 5.528 MeV maximum energy, 2 mm beam size, and 10 photon·s<sup>−1</sup>·eV<sup>−1</sup> flux density, which is available at the BL1U beamline in the ultraviolet synchrotron orbital radiation-III (UVSOR-III) synchrotron radiation facility at the Institute of Molecular Science at the National Institutes of Natural Sciences in Japan, and we excited the J<sup>π</sup> = 1<sup>−</sup> NRF level at 5.512 MeV in <sup>208</sup>Pb. An isotope-selective three-dimensional NRF-CT image of the <sup>208</sup>Pb isotope distribution was experimentally obtained for the first time with a pixel resolution of 4 mm in the horizontal plane.
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spelling doaj.art-41b61bac648a4a8aa86fc5ad2195de472023-11-21T15:01:45ZengMDPI AGApplied Sciences2076-34172021-04-01118341510.3390/app11083415Three-Dimensional Nondestructive Isotope-Selective Tomographic Imaging of <sup>208</sup>Pb Distribution via Nuclear Resonance FluorescenceKhaled Ali0Heishun Zen1Hideaki Ohgaki2Toshiteru Kii3Takehito Hayakawa4Toshiyuki Shizuma5Hiroyuki Toyokawa6Masaki Fujimoto7Yoshitaka Taira8Masahiro Katoh9Institute of Advanced Energy (IAE), Kyoto University, Gokasho, Uji, Kyoto 611-0011, JapanInstitute of Advanced Energy (IAE), Kyoto University, Gokasho, Uji, Kyoto 611-0011, JapanInstitute of Advanced Energy (IAE), Kyoto University, Gokasho, Uji, Kyoto 611-0011, JapanInstitute of Advanced Energy (IAE), Kyoto University, Gokasho, Uji, Kyoto 611-0011, JapanTokai Quantum Beam Science Center, National Institutes for Quantum and Radiological Science and Technology (QST), Ibaraki 319-1106, JapanTokai Quantum Beam Science Center, National Institutes for Quantum and Radiological Science and Technology (QST), Ibaraki 319-1106, JapanInstitute of Advanced Industrial Science and Technology (AIST), Tsukuba Central 2-4, Ibaraki 305-8568, JapanUVSOR-III Synchrotron Facility, Institute for Molecular Science, National Institutes of Natural Sciences, Okazaki 444-8585, JapanUVSOR-III Synchrotron Facility, Institute for Molecular Science, National Institutes of Natural Sciences, Okazaki 444-8585, JapanUVSOR-III Synchrotron Facility, Institute for Molecular Science, National Institutes of Natural Sciences, Okazaki 444-8585, JapanCombining the nuclear resonance fluorescence (NRF) transmission method with computed tomography (CT) can be a novel method for imaging the isotope distributions, which is indispensable in nuclear engineering. We performed an experiment to reconstruct a three-dimensional NRF-CT image with isotope selectivity of enriched lead isotope rods (<sup>208</sup>Pb) together with a set of different rods, including another enriched isotope (<sup>206</sup>Pb), iron, and aluminum rods, inserted into a cylindrical aluminum holder. Using a laser Compton scattering (LCS) gamma ray beam with a 5.528 MeV maximum energy, 2 mm beam size, and 10 photon·s<sup>−1</sup>·eV<sup>−1</sup> flux density, which is available at the BL1U beamline in the ultraviolet synchrotron orbital radiation-III (UVSOR-III) synchrotron radiation facility at the Institute of Molecular Science at the National Institutes of Natural Sciences in Japan, and we excited the J<sup>π</sup> = 1<sup>−</sup> NRF level at 5.512 MeV in <sup>208</sup>Pb. An isotope-selective three-dimensional NRF-CT image of the <sup>208</sup>Pb isotope distribution was experimentally obtained for the first time with a pixel resolution of 4 mm in the horizontal plane.https://www.mdpi.com/2076-3417/11/8/3415gamma rayslaser Compton scattering (LCS)nondestructive inspectionnuclear resonance fluorescence (NRF)isotope-selective computed tomography (CT)
spellingShingle Khaled Ali
Heishun Zen
Hideaki Ohgaki
Toshiteru Kii
Takehito Hayakawa
Toshiyuki Shizuma
Hiroyuki Toyokawa
Masaki Fujimoto
Yoshitaka Taira
Masahiro Katoh
Three-Dimensional Nondestructive Isotope-Selective Tomographic Imaging of <sup>208</sup>Pb Distribution via Nuclear Resonance Fluorescence
Applied Sciences
gamma rays
laser Compton scattering (LCS)
nondestructive inspection
nuclear resonance fluorescence (NRF)
isotope-selective computed tomography (CT)
title Three-Dimensional Nondestructive Isotope-Selective Tomographic Imaging of <sup>208</sup>Pb Distribution via Nuclear Resonance Fluorescence
title_full Three-Dimensional Nondestructive Isotope-Selective Tomographic Imaging of <sup>208</sup>Pb Distribution via Nuclear Resonance Fluorescence
title_fullStr Three-Dimensional Nondestructive Isotope-Selective Tomographic Imaging of <sup>208</sup>Pb Distribution via Nuclear Resonance Fluorescence
title_full_unstemmed Three-Dimensional Nondestructive Isotope-Selective Tomographic Imaging of <sup>208</sup>Pb Distribution via Nuclear Resonance Fluorescence
title_short Three-Dimensional Nondestructive Isotope-Selective Tomographic Imaging of <sup>208</sup>Pb Distribution via Nuclear Resonance Fluorescence
title_sort three dimensional nondestructive isotope selective tomographic imaging of sup 208 sup pb distribution via nuclear resonance fluorescence
topic gamma rays
laser Compton scattering (LCS)
nondestructive inspection
nuclear resonance fluorescence (NRF)
isotope-selective computed tomography (CT)
url https://www.mdpi.com/2076-3417/11/8/3415
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