Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3

CrI3 is a van der Waals material which exhibits magnetic ordering down to the monolayer limit. Here, using ultrafast optical spectroscopy, Padmanabhan and Buessen et al. investigate the coupling between the magnetically ordered spins and lattice distortions, finding a coherent spin-coupled phonon mo...

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Main Authors: P. Padmanabhan, F. L. Buessen, R. Tutchton, K. W. C. Kwock, S. Gilinsky, M. C. Lee, M. A. McGuire, S. R. Singamaneni, D. A. Yarotski, A. Paramekanti, J.-X. Zhu, R. P. Prasankumar
Format: Article
Language:English
Published: Nature Portfolio 2022-08-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-31786-3
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author P. Padmanabhan
F. L. Buessen
R. Tutchton
K. W. C. Kwock
S. Gilinsky
M. C. Lee
M. A. McGuire
S. R. Singamaneni
D. A. Yarotski
A. Paramekanti
J.-X. Zhu
R. P. Prasankumar
author_facet P. Padmanabhan
F. L. Buessen
R. Tutchton
K. W. C. Kwock
S. Gilinsky
M. C. Lee
M. A. McGuire
S. R. Singamaneni
D. A. Yarotski
A. Paramekanti
J.-X. Zhu
R. P. Prasankumar
author_sort P. Padmanabhan
collection DOAJ
description CrI3 is a van der Waals material which exhibits magnetic ordering down to the monolayer limit. Here, using ultrafast optical spectroscopy, Padmanabhan and Buessen et al. investigate the coupling between the magnetically ordered spins and lattice distortions, finding a coherent spin-coupled phonon mode.
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spelling doaj.art-41f28a1cf9784d1c88679acbabf709c92022-12-22T02:33:36ZengNature PortfolioNature Communications2041-17232022-08-011311810.1038/s41467-022-31786-3Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3P. Padmanabhan0F. L. Buessen1R. Tutchton2K. W. C. Kwock3S. Gilinsky4M. C. Lee5M. A. McGuire6S. R. Singamaneni7D. A. Yarotski8A. Paramekanti9J.-X. Zhu10R. P. Prasankumar11Center for Integrated Nanotechnologies, Los Alamos National LaboratoryDepartment of Physics, University of TorontoCenter for Integrated Nanotechnologies, Los Alamos National LaboratoryCenter for Integrated Nanotechnologies, Los Alamos National LaboratoryCenter for Integrated Nanotechnologies, Los Alamos National LaboratoryCenter for Integrated Nanotechnologies, Los Alamos National LaboratoryMaterials Science and Technology Division, Oak Ridge National LaboratoryDepartment of Physics, The University of Texas at El PasoCenter for Integrated Nanotechnologies, Los Alamos National LaboratoryDepartment of Physics, University of TorontoCenter for Integrated Nanotechnologies, Los Alamos National LaboratoryCenter for Integrated Nanotechnologies, Los Alamos National LaboratoryCrI3 is a van der Waals material which exhibits magnetic ordering down to the monolayer limit. Here, using ultrafast optical spectroscopy, Padmanabhan and Buessen et al. investigate the coupling between the magnetically ordered spins and lattice distortions, finding a coherent spin-coupled phonon mode.https://doi.org/10.1038/s41467-022-31786-3
spellingShingle P. Padmanabhan
F. L. Buessen
R. Tutchton
K. W. C. Kwock
S. Gilinsky
M. C. Lee
M. A. McGuire
S. R. Singamaneni
D. A. Yarotski
A. Paramekanti
J.-X. Zhu
R. P. Prasankumar
Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3
Nature Communications
title Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3
title_full Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3
title_fullStr Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3
title_full_unstemmed Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3
title_short Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3
title_sort coherent helicity dependent spin phonon oscillations in the ferromagnetic van der waals crystal cri3
url https://doi.org/10.1038/s41467-022-31786-3
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