Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking

The mechanism of the non-radiative recombination in halide perovskite nanocrystals has not been fully understood. Here Gerhard et al. resolve the contributions of individual recombination centers by photoluminescence blinking measurements and identify ion migration as the underlying mechanism.

Bibliographic Details
Main Authors: Marina Gerhard, Boris Louis, Rafael Camacho, Aboma Merdasa, Jun Li, Alexander Kiligaridis, Alexander Dobrovolsky, Johan Hofkens, Ivan G. Scheblykin
Format: Article
Language:English
Published: Nature Portfolio 2019-04-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-019-09640-w
_version_ 1831827537792073728
author Marina Gerhard
Boris Louis
Rafael Camacho
Aboma Merdasa
Jun Li
Alexander Kiligaridis
Alexander Dobrovolsky
Johan Hofkens
Ivan G. Scheblykin
author_facet Marina Gerhard
Boris Louis
Rafael Camacho
Aboma Merdasa
Jun Li
Alexander Kiligaridis
Alexander Dobrovolsky
Johan Hofkens
Ivan G. Scheblykin
author_sort Marina Gerhard
collection DOAJ
description The mechanism of the non-radiative recombination in halide perovskite nanocrystals has not been fully understood. Here Gerhard et al. resolve the contributions of individual recombination centers by photoluminescence blinking measurements and identify ion migration as the underlying mechanism.
first_indexed 2024-12-23T02:00:50Z
format Article
id doaj.art-4226ca788dda4eaa921933a411af3918
institution Directory Open Access Journal
issn 2041-1723
language English
last_indexed 2024-12-23T02:00:50Z
publishDate 2019-04-01
publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj.art-4226ca788dda4eaa921933a411af39182022-12-21T18:03:59ZengNature PortfolioNature Communications2041-17232019-04-0110111210.1038/s41467-019-09640-wMicroscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinkingMarina Gerhard0Boris Louis1Rafael Camacho2Aboma Merdasa3Jun Li4Alexander Kiligaridis5Alexander Dobrovolsky6Johan Hofkens7Ivan G. Scheblykin8Division of Chemical Physics and NanoLund, Lund UniversityDivision of Chemical Physics and NanoLund, Lund UniversityKU Leuven, Molecular Imaging and PhotonicsHybrid Materials Formation and Scaling, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Helmholtz-Zentrum BerlinDivision of Chemical Physics and NanoLund, Lund UniversityDivision of Chemical Physics and NanoLund, Lund UniversityDivision of Chemical Physics and NanoLund, Lund UniversityKU Leuven, Molecular Imaging and PhotonicsDivision of Chemical Physics and NanoLund, Lund UniversityThe mechanism of the non-radiative recombination in halide perovskite nanocrystals has not been fully understood. Here Gerhard et al. resolve the contributions of individual recombination centers by photoluminescence blinking measurements and identify ion migration as the underlying mechanism.https://doi.org/10.1038/s41467-019-09640-w
spellingShingle Marina Gerhard
Boris Louis
Rafael Camacho
Aboma Merdasa
Jun Li
Alexander Kiligaridis
Alexander Dobrovolsky
Johan Hofkens
Ivan G. Scheblykin
Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking
Nature Communications
title Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking
title_full Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking
title_fullStr Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking
title_full_unstemmed Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking
title_short Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking
title_sort microscopic insight into non radiative decay in perovskite semiconductors from temperature dependent luminescence blinking
url https://doi.org/10.1038/s41467-019-09640-w
work_keys_str_mv AT marinagerhard microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking
AT borislouis microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking
AT rafaelcamacho microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking
AT abomamerdasa microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking
AT junli microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking
AT alexanderkiligaridis microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking
AT alexanderdobrovolsky microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking
AT johanhofkens microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking
AT ivangscheblykin microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking