Al2O3/glass/hBN composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applications

Al2O3/glass/hBN composites were successfully fabricated for the LTCC applications. Alignment and homogeneous distribution of the platelet hBN particles during tape casting allowed high hBN (5 wt%) loading as well as facilitated densification at 800°C (density of 2.65 g/cm3, apparent porosity of 0.7%...

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Main Authors: Oğuzhan Bilaç, Cihangir Duran
Format: Article
Language:English
Published: Taylor & Francis Group 2021-01-01
Series:Journal of Asian Ceramic Societies
Subjects:
Online Access:http://dx.doi.org/10.1080/21870764.2020.1864897
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author Oğuzhan Bilaç
Cihangir Duran
author_facet Oğuzhan Bilaç
Cihangir Duran
author_sort Oğuzhan Bilaç
collection DOAJ
description Al2O3/glass/hBN composites were successfully fabricated for the LTCC applications. Alignment and homogeneous distribution of the platelet hBN particles during tape casting allowed high hBN (5 wt%) loading as well as facilitated densification at 800°C (density of 2.65 g/cm3, apparent porosity of 0.7%). XRD results proved that hBN neither chemically reacted with the other phases nor decomposed with temperature, which was critical to increase thermal conductivity and at the same time to decrease dielectric constant. Dielectric constant of the dense composites decreased (or, alternatively, enhanced) with increasing hBN content from 7.3 for the 0 wt% hBN to 6.55 for the 5 wt% hBN at 5 MHz. In addition, hBN addition strongly improved the mean thermal conductivity from 1.86 W/m·K for the 0 wt% hBN to 2.43 W/m·K for the 5 wt% hBN between 75°C and 250°C. Therefore, the hBN phase itself effectively optimized both dielectric and thermal properties at the same time and made the Al2O3/glass/hBN composites a promising candidate for the LTCC applications.
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spelling doaj.art-42b59757557642378fe9ff755814e1142022-12-21T18:46:57ZengTaylor & Francis GroupJournal of Asian Ceramic Societies2187-07642021-01-019128329010.1080/21870764.2020.18648971864897Al2O3/glass/hBN composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applicationsOğuzhan Bilaç0Cihangir Duran1Ankara Yıldırım Beyazıt UniversityAnkara Yıldırım Beyazıt UniversityAl2O3/glass/hBN composites were successfully fabricated for the LTCC applications. Alignment and homogeneous distribution of the platelet hBN particles during tape casting allowed high hBN (5 wt%) loading as well as facilitated densification at 800°C (density of 2.65 g/cm3, apparent porosity of 0.7%). XRD results proved that hBN neither chemically reacted with the other phases nor decomposed with temperature, which was critical to increase thermal conductivity and at the same time to decrease dielectric constant. Dielectric constant of the dense composites decreased (or, alternatively, enhanced) with increasing hBN content from 7.3 for the 0 wt% hBN to 6.55 for the 5 wt% hBN at 5 MHz. In addition, hBN addition strongly improved the mean thermal conductivity from 1.86 W/m·K for the 0 wt% hBN to 2.43 W/m·K for the 5 wt% hBN between 75°C and 250°C. Therefore, the hBN phase itself effectively optimized both dielectric and thermal properties at the same time and made the Al2O3/glass/hBN composites a promising candidate for the LTCC applications.http://dx.doi.org/10.1080/21870764.2020.1864897al2o3/glass compositehexagonal boron nitridelow temperature co-fired ceramicsthermal propertiesdielectric properties
spellingShingle Oğuzhan Bilaç
Cihangir Duran
Al2O3/glass/hBN composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applications
Journal of Asian Ceramic Societies
al2o3/glass composite
hexagonal boron nitride
low temperature co-fired ceramics
thermal properties
dielectric properties
title Al2O3/glass/hBN composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applications
title_full Al2O3/glass/hBN composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applications
title_fullStr Al2O3/glass/hBN composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applications
title_full_unstemmed Al2O3/glass/hBN composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applications
title_short Al2O3/glass/hBN composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applications
title_sort al2o3 glass hbn composites with high thermal conductivity and low dielectric constant for low temperature cofired ceramic applications
topic al2o3/glass composite
hexagonal boron nitride
low temperature co-fired ceramics
thermal properties
dielectric properties
url http://dx.doi.org/10.1080/21870764.2020.1864897
work_keys_str_mv AT oguzhanbilac al2o3glasshbncompositeswithhighthermalconductivityandlowdielectricconstantforlowtemperaturecofiredceramicapplications
AT cihangirduran al2o3glasshbncompositeswithhighthermalconductivityandlowdielectricconstantforlowtemperaturecofiredceramicapplications