The classical Heisenberg model on the centred pyrochlore lattice

The centred pyrochlore lattice is a novel geometrically frustrated lattice, realized in the metal-organic framework Mn(ta)$_2$ [Phys. Rev. Research 5, L022018 (2023)] where the basic unit of spins is a five site centred tetrahedron. Here, we present an in-depth theoretical study of the $J_1-J_2$ cla...

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Main Author: Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet
Format: Article
Language:English
Published: SciPost 2023-08-01
Series:SciPost Physics
Online Access:https://scipost.org/SciPostPhys.15.2.040
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author Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet
author_facet Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet
author_sort Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet
collection DOAJ
description The centred pyrochlore lattice is a novel geometrically frustrated lattice, realized in the metal-organic framework Mn(ta)$_2$ [Phys. Rev. Research 5, L022018 (2023)] where the basic unit of spins is a five site centred tetrahedron. Here, we present an in-depth theoretical study of the $J_1-J_2$ classical Heisenberg model on this lattice, using a combination of mean-field analytical methods and Monte Carlo simulations. We find a rich phase diagram with low temperature states exhibiting ferrimagnetic order, partial ordering, and a highly degenerate spin liquid with distinct regimes of low temperature correlations. We discuss in detail how the regime displaying broadened pinch points in its spin structure factor is consistent with an effective description in terms of a fluid of interacting charges. We also show how this picture holds in two dimensions on the analogous centred kagome lattice and elucidate the connection to the physics of thin films in ($d+1$) dimensions. Furthermore, we show that a Coulomb phase can be stabilized on the centred pyrochlore lattice by the addition of further neighbour couplings. This demonstrates the centred pyrochlore lattice is an experimentally relevant geometry which naturally hosts emergent gauge fields in the presence of charges at low energies.
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spelling doaj.art-42c9304c7df646bfac86edd7ea36f63d2023-08-01T13:55:38ZengSciPostSciPost Physics2542-46532023-08-0115204010.21468/SciPostPhys.15.2.040The classical Heisenberg model on the centred pyrochlore latticeRajah P. Nutakki, Ludovic D. C. Jaubert, Lode PolletThe centred pyrochlore lattice is a novel geometrically frustrated lattice, realized in the metal-organic framework Mn(ta)$_2$ [Phys. Rev. Research 5, L022018 (2023)] where the basic unit of spins is a five site centred tetrahedron. Here, we present an in-depth theoretical study of the $J_1-J_2$ classical Heisenberg model on this lattice, using a combination of mean-field analytical methods and Monte Carlo simulations. We find a rich phase diagram with low temperature states exhibiting ferrimagnetic order, partial ordering, and a highly degenerate spin liquid with distinct regimes of low temperature correlations. We discuss in detail how the regime displaying broadened pinch points in its spin structure factor is consistent with an effective description in terms of a fluid of interacting charges. We also show how this picture holds in two dimensions on the analogous centred kagome lattice and elucidate the connection to the physics of thin films in ($d+1$) dimensions. Furthermore, we show that a Coulomb phase can be stabilized on the centred pyrochlore lattice by the addition of further neighbour couplings. This demonstrates the centred pyrochlore lattice is an experimentally relevant geometry which naturally hosts emergent gauge fields in the presence of charges at low energies.https://scipost.org/SciPostPhys.15.2.040
spellingShingle Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet
The classical Heisenberg model on the centred pyrochlore lattice
SciPost Physics
title The classical Heisenberg model on the centred pyrochlore lattice
title_full The classical Heisenberg model on the centred pyrochlore lattice
title_fullStr The classical Heisenberg model on the centred pyrochlore lattice
title_full_unstemmed The classical Heisenberg model on the centred pyrochlore lattice
title_short The classical Heisenberg model on the centred pyrochlore lattice
title_sort classical heisenberg model on the centred pyrochlore lattice
url https://scipost.org/SciPostPhys.15.2.040
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