The classical Heisenberg model on the centred pyrochlore lattice
The centred pyrochlore lattice is a novel geometrically frustrated lattice, realized in the metal-organic framework Mn(ta)$_2$ [Phys. Rev. Research 5, L022018 (2023)] where the basic unit of spins is a five site centred tetrahedron. Here, we present an in-depth theoretical study of the $J_1-J_2$ cla...
Main Author: | |
---|---|
Format: | Article |
Language: | English |
Published: |
SciPost
2023-08-01
|
Series: | SciPost Physics |
Online Access: | https://scipost.org/SciPostPhys.15.2.040 |
_version_ | 1797767111646380032 |
---|---|
author | Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet |
author_facet | Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet |
author_sort | Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet |
collection | DOAJ |
description | The centred pyrochlore lattice is a novel geometrically frustrated lattice, realized in the metal-organic framework Mn(ta)$_2$ [Phys. Rev. Research 5, L022018 (2023)] where the basic unit of spins is a five site centred tetrahedron. Here, we present an in-depth theoretical study of the $J_1-J_2$ classical Heisenberg model on this lattice, using a combination of mean-field analytical methods and Monte Carlo simulations. We find a rich phase diagram with low temperature states exhibiting ferrimagnetic order, partial ordering, and a highly degenerate spin liquid with distinct regimes of low temperature correlations. We discuss in detail how the regime displaying broadened pinch points in its spin structure factor is consistent with an effective description in terms of a fluid of interacting charges. We also show how this picture holds in two dimensions on the analogous centred kagome lattice and elucidate the connection to the physics of thin films in ($d+1$) dimensions. Furthermore, we show that a Coulomb phase can be stabilized on the centred pyrochlore lattice by the addition of further neighbour couplings. This demonstrates the centred pyrochlore lattice is an experimentally relevant geometry which naturally hosts emergent gauge fields in the presence of charges at low energies. |
first_indexed | 2024-03-12T20:35:04Z |
format | Article |
id | doaj.art-42c9304c7df646bfac86edd7ea36f63d |
institution | Directory Open Access Journal |
issn | 2542-4653 |
language | English |
last_indexed | 2024-03-12T20:35:04Z |
publishDate | 2023-08-01 |
publisher | SciPost |
record_format | Article |
series | SciPost Physics |
spelling | doaj.art-42c9304c7df646bfac86edd7ea36f63d2023-08-01T13:55:38ZengSciPostSciPost Physics2542-46532023-08-0115204010.21468/SciPostPhys.15.2.040The classical Heisenberg model on the centred pyrochlore latticeRajah P. Nutakki, Ludovic D. C. Jaubert, Lode PolletThe centred pyrochlore lattice is a novel geometrically frustrated lattice, realized in the metal-organic framework Mn(ta)$_2$ [Phys. Rev. Research 5, L022018 (2023)] where the basic unit of spins is a five site centred tetrahedron. Here, we present an in-depth theoretical study of the $J_1-J_2$ classical Heisenberg model on this lattice, using a combination of mean-field analytical methods and Monte Carlo simulations. We find a rich phase diagram with low temperature states exhibiting ferrimagnetic order, partial ordering, and a highly degenerate spin liquid with distinct regimes of low temperature correlations. We discuss in detail how the regime displaying broadened pinch points in its spin structure factor is consistent with an effective description in terms of a fluid of interacting charges. We also show how this picture holds in two dimensions on the analogous centred kagome lattice and elucidate the connection to the physics of thin films in ($d+1$) dimensions. Furthermore, we show that a Coulomb phase can be stabilized on the centred pyrochlore lattice by the addition of further neighbour couplings. This demonstrates the centred pyrochlore lattice is an experimentally relevant geometry which naturally hosts emergent gauge fields in the presence of charges at low energies.https://scipost.org/SciPostPhys.15.2.040 |
spellingShingle | Rajah P. Nutakki, Ludovic D. C. Jaubert, Lode Pollet The classical Heisenberg model on the centred pyrochlore lattice SciPost Physics |
title | The classical Heisenberg model on the centred pyrochlore lattice |
title_full | The classical Heisenberg model on the centred pyrochlore lattice |
title_fullStr | The classical Heisenberg model on the centred pyrochlore lattice |
title_full_unstemmed | The classical Heisenberg model on the centred pyrochlore lattice |
title_short | The classical Heisenberg model on the centred pyrochlore lattice |
title_sort | classical heisenberg model on the centred pyrochlore lattice |
url | https://scipost.org/SciPostPhys.15.2.040 |
work_keys_str_mv | AT rajahpnutakkiludovicdcjaubertlodepollet theclassicalheisenbergmodelonthecentredpyrochlorelattice AT rajahpnutakkiludovicdcjaubertlodepollet classicalheisenbergmodelonthecentredpyrochlorelattice |