The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezing

<p>To estimate the global co-variability between mineral dust aerosol and cloud glaciation, we combined an aerosol model reanalysis with satellite retrievals of cloud thermodynamic phase. We used the CALIPSO-GOCCP product from the A-Train satellite constellation to assess whether clouds are co...

Full description

Bibliographic Details
Main Authors: D. Villanueva, B. Heinold, P. Seifert, H. Deneke, M. Radenz, I. Tegen
Format: Article
Language:English
Published: Copernicus Publications 2020-02-01
Series:Atmospheric Chemistry and Physics
Online Access:https://www.atmos-chem-phys.net/20/2177/2020/acp-20-2177-2020.pdf
_version_ 1819289547080466432
author D. Villanueva
B. Heinold
P. Seifert
H. Deneke
M. Radenz
I. Tegen
author_facet D. Villanueva
B. Heinold
P. Seifert
H. Deneke
M. Radenz
I. Tegen
author_sort D. Villanueva
collection DOAJ
description <p>To estimate the global co-variability between mineral dust aerosol and cloud glaciation, we combined an aerosol model reanalysis with satellite retrievals of cloud thermodynamic phase. We used the CALIPSO-GOCCP product from the A-Train satellite constellation to assess whether clouds are composed of liquid or ice and the MACC reanalysis to estimate the dust mixing ratio in the atmosphere. Night-time retrievals within a temperature range from <span class="inline-formula">+3</span> to <span class="inline-formula">−42</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C for the period 2007–2010 were included. The results confirm that the cloud thermodynamic phase is highly dependent on temperature and latitude. However, at middle and high latitudes, at equal temperature and within narrow constraints for humidity and static stability, the average frequency of fully glaciated clouds increases by <span class="inline-formula">+5</span> to <span class="inline-formula">+10 <i>%</i></span> for higher mineral dust mixing ratios. The discrimination between humidity and stability regimes reduced the confounding influence of meteorology on the observed relationship between dust and cloud ice. Furthermore, for days with similar mixing ratios of mineral dust, the cloud ice occurrence frequency in the Northern Hemisphere was found to be higher than in the Southern Hemisphere at <span class="inline-formula">−30</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C but lower at <span class="inline-formula">−15</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C. This contrast may suggest a difference in the susceptibility of cloud glaciation to the presence of dust. Based on previous studies, the differences at <span class="inline-formula">−15</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C could be explained by higher feldspar fractions in the Southern Hemisphere, while the higher freezing efficiency of clay minerals in the Northern Hemisphere may explain the differences at <span class="inline-formula">−30</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C.</p>
first_indexed 2024-12-24T03:08:35Z
format Article
id doaj.art-448850aa78aa48188266805349aff13a
institution Directory Open Access Journal
issn 1680-7316
1680-7324
language English
last_indexed 2024-12-24T03:08:35Z
publishDate 2020-02-01
publisher Copernicus Publications
record_format Article
series Atmospheric Chemistry and Physics
spelling doaj.art-448850aa78aa48188266805349aff13a2022-12-21T17:17:55ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242020-02-01202177219910.5194/acp-20-2177-2020The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezingD. VillanuevaB. HeinoldP. SeifertH. DenekeM. RadenzI. Tegen<p>To estimate the global co-variability between mineral dust aerosol and cloud glaciation, we combined an aerosol model reanalysis with satellite retrievals of cloud thermodynamic phase. We used the CALIPSO-GOCCP product from the A-Train satellite constellation to assess whether clouds are composed of liquid or ice and the MACC reanalysis to estimate the dust mixing ratio in the atmosphere. Night-time retrievals within a temperature range from <span class="inline-formula">+3</span> to <span class="inline-formula">−42</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C for the period 2007–2010 were included. The results confirm that the cloud thermodynamic phase is highly dependent on temperature and latitude. However, at middle and high latitudes, at equal temperature and within narrow constraints for humidity and static stability, the average frequency of fully glaciated clouds increases by <span class="inline-formula">+5</span> to <span class="inline-formula">+10 <i>%</i></span> for higher mineral dust mixing ratios. The discrimination between humidity and stability regimes reduced the confounding influence of meteorology on the observed relationship between dust and cloud ice. Furthermore, for days with similar mixing ratios of mineral dust, the cloud ice occurrence frequency in the Northern Hemisphere was found to be higher than in the Southern Hemisphere at <span class="inline-formula">−30</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C but lower at <span class="inline-formula">−15</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C. This contrast may suggest a difference in the susceptibility of cloud glaciation to the presence of dust. Based on previous studies, the differences at <span class="inline-formula">−15</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C could be explained by higher feldspar fractions in the Southern Hemisphere, while the higher freezing efficiency of clay minerals in the Northern Hemisphere may explain the differences at <span class="inline-formula">−30</span>&thinsp;<span class="inline-formula"><sup>∘</sup></span>C.</p>https://www.atmos-chem-phys.net/20/2177/2020/acp-20-2177-2020.pdf
spellingShingle D. Villanueva
B. Heinold
P. Seifert
H. Deneke
M. Radenz
I. Tegen
The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezing
Atmospheric Chemistry and Physics
title The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezing
title_full The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezing
title_fullStr The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezing
title_full_unstemmed The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezing
title_short The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezing
title_sort day to day co variability between mineral dust and cloud glaciation a proxy for heterogeneous freezing
url https://www.atmos-chem-phys.net/20/2177/2020/acp-20-2177-2020.pdf
work_keys_str_mv AT dvillanueva thedaytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT bheinold thedaytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT pseifert thedaytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT hdeneke thedaytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT mradenz thedaytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT itegen thedaytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT dvillanueva daytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT bheinold daytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT pseifert daytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT hdeneke daytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT mradenz daytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing
AT itegen daytodaycovariabilitybetweenmineraldustandcloudglaciationaproxyforheterogeneousfreezing