Dispersive coherent Brillouin scattering spectroscopy

Frequency- and time-domain Brillouin scattering spectroscopy are powerful tools to read out the mechanical properties of complex systems in material and life sciences. Indeed, coherent acoustic phonons in the time-domain method offer superior depth resolution and a stronger signal than incoherent ac...

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Main Authors: Ayumu Ishijima, Shinga Okabe, Ichiro Sakuma, Keiichi Nakagawa
Format: Article
Language:English
Published: Elsevier 2023-02-01
Series:Photoacoustics
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2213597922001124
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author Ayumu Ishijima
Shinga Okabe
Ichiro Sakuma
Keiichi Nakagawa
author_facet Ayumu Ishijima
Shinga Okabe
Ichiro Sakuma
Keiichi Nakagawa
author_sort Ayumu Ishijima
collection DOAJ
description Frequency- and time-domain Brillouin scattering spectroscopy are powerful tools to read out the mechanical properties of complex systems in material and life sciences. Indeed, coherent acoustic phonons in the time-domain method offer superior depth resolution and a stronger signal than incoherent acoustic phonons in the frequency-domain method. However, it requires scanning of delay time between laser pulses for pumping and probing coherent acoustic phonons. Here, we present Brillouin scattering spectroscopy that spans the time and frequency domains to allow the multichannel detection of Brillouin scattering light from coherent acoustic phonons. Our technique traces the time-evolve Brillouin oscillations at the instantaneous frequency of a chromatic-dispersed laser pulse. The spectroscopic heterodyning of Brillouin scattering light in the frequency domain allows a single-frame readout of gigahertz-frequency oscillations with a spectrometer. As a proof of concept, we imaged heterogeneous thin films and biological cells over a wide bandwidth with nanometer depth resolution.
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spelling doaj.art-459544dac71f4bbc97ff928a1cd88bf22023-02-12T04:14:47ZengElsevierPhotoacoustics2213-59792023-02-0129100447Dispersive coherent Brillouin scattering spectroscopyAyumu Ishijima0Shinga Okabe1Ichiro Sakuma2Keiichi Nakagawa3Department of Precision Engineering, The University of Tokyo, Tokyo 113-8656, Japan; PRESTO, Japan Science and Technology Agency, Saitama 332-0012, Japan; Corresponding author at: Department of Precision Engineering, The University of Tokyo, Tokyo 113-8656, Japan.Department of Bioengineering, The University of Tokyo, Tokyo 113-8656, JapanDepartment of Precision Engineering, The University of Tokyo, Tokyo 113-8656, Japan; Department of Bioengineering, The University of Tokyo, Tokyo 113-8656, Japan; Medical Device Development and Regulation Research Center, The University of Tokyo, Tokyo 113-8656, JapanDepartment of Precision Engineering, The University of Tokyo, Tokyo 113-8656, Japan; Department of Bioengineering, The University of Tokyo, Tokyo 113-8656, JapanFrequency- and time-domain Brillouin scattering spectroscopy are powerful tools to read out the mechanical properties of complex systems in material and life sciences. Indeed, coherent acoustic phonons in the time-domain method offer superior depth resolution and a stronger signal than incoherent acoustic phonons in the frequency-domain method. However, it requires scanning of delay time between laser pulses for pumping and probing coherent acoustic phonons. Here, we present Brillouin scattering spectroscopy that spans the time and frequency domains to allow the multichannel detection of Brillouin scattering light from coherent acoustic phonons. Our technique traces the time-evolve Brillouin oscillations at the instantaneous frequency of a chromatic-dispersed laser pulse. The spectroscopic heterodyning of Brillouin scattering light in the frequency domain allows a single-frame readout of gigahertz-frequency oscillations with a spectrometer. As a proof of concept, we imaged heterogeneous thin films and biological cells over a wide bandwidth with nanometer depth resolution.http://www.sciencedirect.com/science/article/pii/S2213597922001124Brillouin microscopyBrillouin light scatteringBrillouin oscillationsPicosecond ultrasonicsPhonon spectroscopyChirped pulse spectroscopy
spellingShingle Ayumu Ishijima
Shinga Okabe
Ichiro Sakuma
Keiichi Nakagawa
Dispersive coherent Brillouin scattering spectroscopy
Photoacoustics
Brillouin microscopy
Brillouin light scattering
Brillouin oscillations
Picosecond ultrasonics
Phonon spectroscopy
Chirped pulse spectroscopy
title Dispersive coherent Brillouin scattering spectroscopy
title_full Dispersive coherent Brillouin scattering spectroscopy
title_fullStr Dispersive coherent Brillouin scattering spectroscopy
title_full_unstemmed Dispersive coherent Brillouin scattering spectroscopy
title_short Dispersive coherent Brillouin scattering spectroscopy
title_sort dispersive coherent brillouin scattering spectroscopy
topic Brillouin microscopy
Brillouin light scattering
Brillouin oscillations
Picosecond ultrasonics
Phonon spectroscopy
Chirped pulse spectroscopy
url http://www.sciencedirect.com/science/article/pii/S2213597922001124
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AT shingaokabe dispersivecoherentbrillouinscatteringspectroscopy
AT ichirosakuma dispersivecoherentbrillouinscatteringspectroscopy
AT keiichinakagawa dispersivecoherentbrillouinscatteringspectroscopy