Flexible ceramic film capacitors for high-temperature power electronics

Flexible ceramic film capacitors with high dielectric constant and high breakdown strength hold special promise for applications in power electronics. We deposited lanthanum-doped lead zirconate titanate (PLZT) films on aluminum-metallized polyimide films at room temperature by an aerosol deposition...

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Main Authors: Beihai Ma, Tae H. Lee, Stephen E. Dorris, Rachel E. Koritala, Uthamalingam Balachandran
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2019-04-01
Series:Materials Science for Energy Technologies
Online Access:http://www.sciencedirect.com/science/article/pii/S2589299118301162
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author Beihai Ma
Tae H. Lee
Stephen E. Dorris
Rachel E. Koritala
Uthamalingam Balachandran
author_facet Beihai Ma
Tae H. Lee
Stephen E. Dorris
Rachel E. Koritala
Uthamalingam Balachandran
author_sort Beihai Ma
collection DOAJ
description Flexible ceramic film capacitors with high dielectric constant and high breakdown strength hold special promise for applications in power electronics. We deposited lanthanum-doped lead zirconate titanate (PLZT) films on aluminum-metallized polyimide films at room temperature by an aerosol deposition (AD) process and examined the electrical and dielectric properties of the PLZT films over a wide temperature range between −55 and 175 °C. The PLZT film capacitors fabricated by high deposition rate AD process not only satisfy X8R temperature rating but also exhibit superior volumetric and gravimetric specific capacitance. At room temperature, we measured a dielectric constant of ≈85, dielectric loss of ≈0.012, energy density of ≈13.2 J/cm3 with an applied voltage of ≈1000 V. A mean dielectric breakdown field strength (EB) of ≈1.25 MV/cm was determined by Weibull analysis for the ≈8-μm-thick PLZT film capacitors fabricated on flexible aluminum-metallized polyimide substrates. These results revealed that the PLZT-based ceramic film capacitors meet the requirements for advanced high-temperature power inverters. Our results demonstrated that AD process offers the greatest potential for producing low-cost, robust, compact and light-weight ceramic film capacitors with enhanced reliability for power inverters of electrical drive vehicles and various power electronic devices that are critical for high-efficiency energy conversion and renewable energy systems. Keywords: Ceramic coating, Aerosol deposition, Film capacitor, Energy conversion, Power electronics
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spelling doaj.art-4615212e04e34f0fb97a36e1443fd43b2022-12-21T22:11:52ZengKeAi Communications Co., Ltd.Materials Science for Energy Technologies2589-29912019-04-012196103Flexible ceramic film capacitors for high-temperature power electronicsBeihai Ma0Tae H. Lee1Stephen E. Dorris2Rachel E. Koritala3Uthamalingam Balachandran4Applied Materials Division, Argonne National Laboratory, Argonne, IL 60439, United States; Corresponding author.Applied Materials Division, Argonne National Laboratory, Argonne, IL 60439, United StatesApplied Materials Division, Argonne National Laboratory, Argonne, IL 60439, United StatesNanoscience and Technology Division, Argonne National Laboratory, Argonne, IL 60439, United StatesApplied Materials Division, Argonne National Laboratory, Argonne, IL 60439, United StatesFlexible ceramic film capacitors with high dielectric constant and high breakdown strength hold special promise for applications in power electronics. We deposited lanthanum-doped lead zirconate titanate (PLZT) films on aluminum-metallized polyimide films at room temperature by an aerosol deposition (AD) process and examined the electrical and dielectric properties of the PLZT films over a wide temperature range between −55 and 175 °C. The PLZT film capacitors fabricated by high deposition rate AD process not only satisfy X8R temperature rating but also exhibit superior volumetric and gravimetric specific capacitance. At room temperature, we measured a dielectric constant of ≈85, dielectric loss of ≈0.012, energy density of ≈13.2 J/cm3 with an applied voltage of ≈1000 V. A mean dielectric breakdown field strength (EB) of ≈1.25 MV/cm was determined by Weibull analysis for the ≈8-μm-thick PLZT film capacitors fabricated on flexible aluminum-metallized polyimide substrates. These results revealed that the PLZT-based ceramic film capacitors meet the requirements for advanced high-temperature power inverters. Our results demonstrated that AD process offers the greatest potential for producing low-cost, robust, compact and light-weight ceramic film capacitors with enhanced reliability for power inverters of electrical drive vehicles and various power electronic devices that are critical for high-efficiency energy conversion and renewable energy systems. Keywords: Ceramic coating, Aerosol deposition, Film capacitor, Energy conversion, Power electronicshttp://www.sciencedirect.com/science/article/pii/S2589299118301162
spellingShingle Beihai Ma
Tae H. Lee
Stephen E. Dorris
Rachel E. Koritala
Uthamalingam Balachandran
Flexible ceramic film capacitors for high-temperature power electronics
Materials Science for Energy Technologies
title Flexible ceramic film capacitors for high-temperature power electronics
title_full Flexible ceramic film capacitors for high-temperature power electronics
title_fullStr Flexible ceramic film capacitors for high-temperature power electronics
title_full_unstemmed Flexible ceramic film capacitors for high-temperature power electronics
title_short Flexible ceramic film capacitors for high-temperature power electronics
title_sort flexible ceramic film capacitors for high temperature power electronics
url http://www.sciencedirect.com/science/article/pii/S2589299118301162
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AT rachelekoritala flexibleceramicfilmcapacitorsforhightemperaturepowerelectronics
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