Growth and Scintillation Properties of Directionally Solidified Ce:LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) Eutectic System

Ce-doped LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) eutectics were grown using the Bridgman–Stockbarger (BS) method in quartz ampoules. The eutectics (AE = Mg and Ca) showed optical transparency like optical fiber bundles. A grown Ce-doped LaBr<sub>3</su...

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Main Authors: Kyoung Jin Kim, Yuki Furuya, Kei Kamada, Rikito Murakami, Vladimir V. Kochurikhin, Masao Yoshino, Hiroyuki Chiba, Shunsuke Kurosawa, Akihiro Yamaji, Yasuhiro Shoji, Satoshi Toyoda, Hiroki Sato, Yuui Yokota, Yuji Ohashi, Akira Yoshikawa
Format: Article
Language:English
Published: MDPI AG 2020-07-01
Series:Crystals
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Online Access:https://www.mdpi.com/2073-4352/10/7/584
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author Kyoung Jin Kim
Yuki Furuya
Kei Kamada
Rikito Murakami
Vladimir V. Kochurikhin
Masao Yoshino
Hiroyuki Chiba
Shunsuke Kurosawa
Akihiro Yamaji
Yasuhiro Shoji
Satoshi Toyoda
Hiroki Sato
Yuui Yokota
Yuji Ohashi
Akira Yoshikawa
author_facet Kyoung Jin Kim
Yuki Furuya
Kei Kamada
Rikito Murakami
Vladimir V. Kochurikhin
Masao Yoshino
Hiroyuki Chiba
Shunsuke Kurosawa
Akihiro Yamaji
Yasuhiro Shoji
Satoshi Toyoda
Hiroki Sato
Yuui Yokota
Yuji Ohashi
Akira Yoshikawa
author_sort Kyoung Jin Kim
collection DOAJ
description Ce-doped LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) eutectics were grown using the Bridgman–Stockbarger (BS) method in quartz ampoules. The eutectics (AE = Mg and Ca) showed optical transparency like optical fiber bundles. A grown Ce-doped LaBr<sub>3</sub>/MgBr<sub>2</sub> eutectic shows a 355 nm emission ascribed to Ce<sup>3+</sup> 4f-5d transition under X-ray excitation. The smaller the ionic size of AE, the higher the light yield of the sample was. The light yield of Ce:LaBr<sub>3</sub>/MgBr<sub>2</sub> was 34,300 photon/MeV, which is higher than Ce:LYSO standard. Scintillation decay time under 662 keV gamma-ray excitation was 18.8 ns.
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spelling doaj.art-46fb7e80aa154c2780c2dc73860ffefa2023-11-20T05:58:28ZengMDPI AGCrystals2073-43522020-07-0110758410.3390/cryst10070584Growth and Scintillation Properties of Directionally Solidified Ce:LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) Eutectic SystemKyoung Jin Kim0Yuki Furuya1Kei Kamada2Rikito Murakami3Vladimir V. Kochurikhin4Masao Yoshino5Hiroyuki Chiba6Shunsuke Kurosawa7Akihiro Yamaji8Yasuhiro Shoji9Satoshi Toyoda10Hiroki Sato11Yuui Yokota12Yuji Ohashi13Akira Yoshikawa14New Industry Creation Hatchery Center (NICHe), Tohoku University, 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai 980-8579, JapanInstitute for Material Research (IMR), Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, JapanNew Industry Creation Hatchery Center (NICHe), Tohoku University, 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai 980-8579, JapanC&A Corporation, 1-16-23 Ichibancho, Aoba-ku, Sendai 980-0811, JapanC&A Corporation, 1-16-23 Ichibancho, Aoba-ku, Sendai 980-0811, JapanInstitute for Material Research (IMR), Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, JapanInstitute for Material Research (IMR), Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, JapanNew Industry Creation Hatchery Center (NICHe), Tohoku University, 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai 980-8579, JapanInstitute for Material Research (IMR), Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, JapanC&A Corporation, 1-16-23 Ichibancho, Aoba-ku, Sendai 980-0811, JapanNew Industry Creation Hatchery Center (NICHe), Tohoku University, 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai 980-8579, JapanNew Industry Creation Hatchery Center (NICHe), Tohoku University, 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai 980-8579, JapanInstitute for Material Research (IMR), Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, JapanNew Industry Creation Hatchery Center (NICHe), Tohoku University, 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai 980-8579, JapanNew Industry Creation Hatchery Center (NICHe), Tohoku University, 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai 980-8579, JapanCe-doped LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) eutectics were grown using the Bridgman–Stockbarger (BS) method in quartz ampoules. The eutectics (AE = Mg and Ca) showed optical transparency like optical fiber bundles. A grown Ce-doped LaBr<sub>3</sub>/MgBr<sub>2</sub> eutectic shows a 355 nm emission ascribed to Ce<sup>3+</sup> 4f-5d transition under X-ray excitation. The smaller the ionic size of AE, the higher the light yield of the sample was. The light yield of Ce:LaBr<sub>3</sub>/MgBr<sub>2</sub> was 34,300 photon/MeV, which is higher than Ce:LYSO standard. Scintillation decay time under 662 keV gamma-ray excitation was 18.8 ns.https://www.mdpi.com/2073-4352/10/7/584directional solidificationgrowth from melthalidesscintillators
spellingShingle Kyoung Jin Kim
Yuki Furuya
Kei Kamada
Rikito Murakami
Vladimir V. Kochurikhin
Masao Yoshino
Hiroyuki Chiba
Shunsuke Kurosawa
Akihiro Yamaji
Yasuhiro Shoji
Satoshi Toyoda
Hiroki Sato
Yuui Yokota
Yuji Ohashi
Akira Yoshikawa
Growth and Scintillation Properties of Directionally Solidified Ce:LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) Eutectic System
Crystals
directional solidification
growth from melt
halides
scintillators
title Growth and Scintillation Properties of Directionally Solidified Ce:LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) Eutectic System
title_full Growth and Scintillation Properties of Directionally Solidified Ce:LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) Eutectic System
title_fullStr Growth and Scintillation Properties of Directionally Solidified Ce:LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) Eutectic System
title_full_unstemmed Growth and Scintillation Properties of Directionally Solidified Ce:LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) Eutectic System
title_short Growth and Scintillation Properties of Directionally Solidified Ce:LaBr<sub>3</sub>/AEBr<sub>2</sub> (AE = Mg, Ca, Sr, Ba) Eutectic System
title_sort growth and scintillation properties of directionally solidified ce labr sub 3 sub aebr sub 2 sub ae mg ca sr ba eutectic system
topic directional solidification
growth from melt
halides
scintillators
url https://www.mdpi.com/2073-4352/10/7/584
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