Infrared‐to‐THz Detection and Spectroscopy with Whispering‐Gallery‐Mode Microresonators

A novel room‐temperature photodetector based on a silica‐microsphere optical resonator operating from the mid‐infrared to the terahertz spectral region is reported. The sensor relies on a free‐space visible laser whose frequency is locked to the center of a whispering‐gallery mode (WGM). The devised...

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Main Authors: Davide D'Ambrosio, Marialuisa Capezzuto, Roberto Aiello, Maria Giulia Delli Santi, Alessia Sorgi, Pietro Malara, Saverio Avino, Antonio Giorgini, Pasquale Maddaloni, Luigi Consolino, Miriam Serena Vitiello, Paolo De Natale, Gianluca Gagliardi
Format: Article
Language:English
Published: Wiley-VCH 2022-12-01
Series:Advanced Photonics Research
Subjects:
Online Access:https://doi.org/10.1002/adpr.202200147
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author Davide D'Ambrosio
Marialuisa Capezzuto
Roberto Aiello
Maria Giulia Delli Santi
Alessia Sorgi
Pietro Malara
Saverio Avino
Antonio Giorgini
Pasquale Maddaloni
Luigi Consolino
Miriam Serena Vitiello
Paolo De Natale
Gianluca Gagliardi
author_facet Davide D'Ambrosio
Marialuisa Capezzuto
Roberto Aiello
Maria Giulia Delli Santi
Alessia Sorgi
Pietro Malara
Saverio Avino
Antonio Giorgini
Pasquale Maddaloni
Luigi Consolino
Miriam Serena Vitiello
Paolo De Natale
Gianluca Gagliardi
author_sort Davide D'Ambrosio
collection DOAJ
description A novel room‐temperature photodetector based on a silica‐microsphere optical resonator operating from the mid‐infrared to the terahertz spectral region is reported. The sensor relies on a free‐space visible laser whose frequency is locked to the center of a whispering‐gallery mode (WGM). The devised scheme automatically tracks any small change in the microresonator's size and refractive index that occurs upon illumination with radiation absorbed by silica. In this way, direct detection of quantum‐cascade laser beams around 4.3 and 111 μm wavelengths is shown, down to minimum noise‐equivalent power levels of ≈1 pW √Hz−1 with a dynamic range >100 dB. The microsphere resonator is then exploited, for the first time, as a photodetector in absorption spectroscopy of the 12CO2 fundamental ro‐vibrational band and of very‐weak 13CH3OH rotational lines.
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spelling doaj.art-4809517d99b047abb798ae7e83b473772022-12-22T04:41:02ZengWiley-VCHAdvanced Photonics Research2699-92932022-12-01312n/an/a10.1002/adpr.202200147Infrared‐to‐THz Detection and Spectroscopy with Whispering‐Gallery‐Mode MicroresonatorsDavide D'Ambrosio0Marialuisa Capezzuto1Roberto Aiello2Maria Giulia Delli Santi3Alessia Sorgi4Pietro Malara5Saverio Avino6Antonio Giorgini7Pasquale Maddaloni8Luigi Consolino9Miriam Serena Vitiello10Paolo De Natale11Gianluca Gagliardi12Consiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto di Nanoscienze (NANO) p.zza S. Silvestro 12 56127 Pisa ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyConsiglio Nazionale delle Ricerche Istituto Nazionale di Ottica (INO) via Campi Flegrei 34 Comprensorio A. Olivetti I-80078 Pozzuoli ItalyA novel room‐temperature photodetector based on a silica‐microsphere optical resonator operating from the mid‐infrared to the terahertz spectral region is reported. The sensor relies on a free‐space visible laser whose frequency is locked to the center of a whispering‐gallery mode (WGM). The devised scheme automatically tracks any small change in the microresonator's size and refractive index that occurs upon illumination with radiation absorbed by silica. In this way, direct detection of quantum‐cascade laser beams around 4.3 and 111 μm wavelengths is shown, down to minimum noise‐equivalent power levels of ≈1 pW √Hz−1 with a dynamic range >100 dB. The microsphere resonator is then exploited, for the first time, as a photodetector in absorption spectroscopy of the 12CO2 fundamental ro‐vibrational band and of very‐weak 13CH3OH rotational lines.https://doi.org/10.1002/adpr.202200147infrared detectionmolecular spectroscopyoptical microresonatorTHz detectionwhispering-gallery mode
spellingShingle Davide D'Ambrosio
Marialuisa Capezzuto
Roberto Aiello
Maria Giulia Delli Santi
Alessia Sorgi
Pietro Malara
Saverio Avino
Antonio Giorgini
Pasquale Maddaloni
Luigi Consolino
Miriam Serena Vitiello
Paolo De Natale
Gianluca Gagliardi
Infrared‐to‐THz Detection and Spectroscopy with Whispering‐Gallery‐Mode Microresonators
Advanced Photonics Research
infrared detection
molecular spectroscopy
optical microresonator
THz detection
whispering-gallery mode
title Infrared‐to‐THz Detection and Spectroscopy with Whispering‐Gallery‐Mode Microresonators
title_full Infrared‐to‐THz Detection and Spectroscopy with Whispering‐Gallery‐Mode Microresonators
title_fullStr Infrared‐to‐THz Detection and Spectroscopy with Whispering‐Gallery‐Mode Microresonators
title_full_unstemmed Infrared‐to‐THz Detection and Spectroscopy with Whispering‐Gallery‐Mode Microresonators
title_short Infrared‐to‐THz Detection and Spectroscopy with Whispering‐Gallery‐Mode Microresonators
title_sort infrared to thz detection and spectroscopy with whispering gallery mode microresonators
topic infrared detection
molecular spectroscopy
optical microresonator
THz detection
whispering-gallery mode
url https://doi.org/10.1002/adpr.202200147
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