Combining Spin-Seebeck and Nernst Effects in Aligned MnBi/Bi Composites

The spin-Seebeck effect (SSE) is an advective transport process traditionally studied in bilayers composed of a ferromagnet (FM) and a non-magnetic metal (NM) with strong spin-orbit coupling. In a temperature gradient, the flux of magnons in the FM transfers spin-angular momentum to electrons in the...

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Main Authors: Brandi L. Wooten, Koen Vandaele, Stephen R. Boona, Joseph P. Heremans
Format: Article
Language:English
Published: MDPI AG 2020-10-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/10/10/2083
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author Brandi L. Wooten
Koen Vandaele
Stephen R. Boona
Joseph P. Heremans
author_facet Brandi L. Wooten
Koen Vandaele
Stephen R. Boona
Joseph P. Heremans
author_sort Brandi L. Wooten
collection DOAJ
description The spin-Seebeck effect (SSE) is an advective transport process traditionally studied in bilayers composed of a ferromagnet (FM) and a non-magnetic metal (NM) with strong spin-orbit coupling. In a temperature gradient, the flux of magnons in the FM transfers spin-angular momentum to electrons in the NM, which by the inverse spin-Hall effect generates an SSE voltage. In contrast, the Nernst effect is a bulk transport phenomenon in homogeneous NMs or FMs. These effects share the same geometry, and we show here that they can be added to each other in a new combination of FM/NM composites where synthesis via in-field annealing results in the FM material (MnBi) forming aligned needles inside an NM matrix with strong spin-orbit coupling (SOC) (Bi). Through examination of the materials’ microstructural, magnetic, and transport properties, we searched for signs of enhanced transverse thermopower facilitated by an SSE contribution from MnBi adding to the Nernst effect in Bi. Our results indicate that these two signals are additive in samples with lower MnBi concentrations, suggesting a new way forward in the study of SSE composite materials.
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spelling doaj.art-49509df10800467bae1d745eb200d0f52023-11-20T17:59:38ZengMDPI AGNanomaterials2079-49912020-10-011010208310.3390/nano10102083Combining Spin-Seebeck and Nernst Effects in Aligned MnBi/Bi CompositesBrandi L. Wooten0Koen Vandaele1Stephen R. Boona2Joseph P. Heremans3Department of Materials Science and Engineering, The Ohio State University, Columbus, OH 43210, USADepartment of Mechanical and Aerospace Engineering, The Ohio State University, Columbus, OH 43210, USADepartment of Materials Science and Engineering, The Ohio State University, Columbus, OH 43210, USADepartment of Materials Science and Engineering, The Ohio State University, Columbus, OH 43210, USAThe spin-Seebeck effect (SSE) is an advective transport process traditionally studied in bilayers composed of a ferromagnet (FM) and a non-magnetic metal (NM) with strong spin-orbit coupling. In a temperature gradient, the flux of magnons in the FM transfers spin-angular momentum to electrons in the NM, which by the inverse spin-Hall effect generates an SSE voltage. In contrast, the Nernst effect is a bulk transport phenomenon in homogeneous NMs or FMs. These effects share the same geometry, and we show here that they can be added to each other in a new combination of FM/NM composites where synthesis via in-field annealing results in the FM material (MnBi) forming aligned needles inside an NM matrix with strong spin-orbit coupling (SOC) (Bi). Through examination of the materials’ microstructural, magnetic, and transport properties, we searched for signs of enhanced transverse thermopower facilitated by an SSE contribution from MnBi adding to the Nernst effect in Bi. Our results indicate that these two signals are additive in samples with lower MnBi concentrations, suggesting a new way forward in the study of SSE composite materials.https://www.mdpi.com/2079-4991/10/10/2083spin-Seebeck effectanomalous Nernst effectthermoelectric compositeMnBi
spellingShingle Brandi L. Wooten
Koen Vandaele
Stephen R. Boona
Joseph P. Heremans
Combining Spin-Seebeck and Nernst Effects in Aligned MnBi/Bi Composites
Nanomaterials
spin-Seebeck effect
anomalous Nernst effect
thermoelectric composite
MnBi
title Combining Spin-Seebeck and Nernst Effects in Aligned MnBi/Bi Composites
title_full Combining Spin-Seebeck and Nernst Effects in Aligned MnBi/Bi Composites
title_fullStr Combining Spin-Seebeck and Nernst Effects in Aligned MnBi/Bi Composites
title_full_unstemmed Combining Spin-Seebeck and Nernst Effects in Aligned MnBi/Bi Composites
title_short Combining Spin-Seebeck and Nernst Effects in Aligned MnBi/Bi Composites
title_sort combining spin seebeck and nernst effects in aligned mnbi bi composites
topic spin-Seebeck effect
anomalous Nernst effect
thermoelectric composite
MnBi
url https://www.mdpi.com/2079-4991/10/10/2083
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AT koenvandaele combiningspinseebeckandnernsteffectsinalignedmnbibicomposites
AT stephenrboona combiningspinseebeckandnernsteffectsinalignedmnbibicomposites
AT josephpheremans combiningspinseebeckandnernsteffectsinalignedmnbibicomposites