Engineering a Robust Quantum Spin Hall State in Graphene via Adatom Deposition

The 2007 discovery of quantized conductance in HgTe quantum wells delivered the field of topological insulators (TIs) its first experimental confirmation. While many three-dimensional TIs have since been identified, HgTe remains the only known two-dimensional system in this class. Difficulty fabrica...

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Main Authors: Conan Weeks, Jun Hu, Jason Alicea, Marcel Franz, Ruqian Wu
Format: Article
Language:English
Published: American Physical Society 2011-10-01
Series:Physical Review X
Online Access:http://doi.org/10.1103/PhysRevX.1.021001
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author Conan Weeks
Jun Hu
Jason Alicea
Marcel Franz
Ruqian Wu
author_facet Conan Weeks
Jun Hu
Jason Alicea
Marcel Franz
Ruqian Wu
author_sort Conan Weeks
collection DOAJ
description The 2007 discovery of quantized conductance in HgTe quantum wells delivered the field of topological insulators (TIs) its first experimental confirmation. While many three-dimensional TIs have since been identified, HgTe remains the only known two-dimensional system in this class. Difficulty fabricating HgTe quantum wells has, moreover, hampered their widespread use. With the goal of breaking this logjam, we provide a blueprint for stabilizing a robust TI state in a more readily available two-dimensional material—graphene. Using symmetry arguments, density functional theory, and tight-binding simulations, we predict that graphene endowed with certain heavy adatoms realizes a TI with substantial band gap. For indium and thallium, our most promising adatom candidates, a modest 6% coverage produces an estimated gap near 80 K and 240 K, respectively, which should be detectable in transport or spectroscopic measurements. Engineering such a robust topological phase in graphene could pave the way for a new generation of devices for spintronics, ultra-low-dissipation electronics, and quantum information processing.
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spelling doaj.art-4d1631fd53c44006a68877aeda21c8852022-12-21T18:37:27ZengAmerican Physical SocietyPhysical Review X2160-33082011-10-011202100110.1103/PhysRevX.1.021001Engineering a Robust Quantum Spin Hall State in Graphene via Adatom DepositionConan WeeksJun HuJason AliceaMarcel FranzRuqian WuThe 2007 discovery of quantized conductance in HgTe quantum wells delivered the field of topological insulators (TIs) its first experimental confirmation. While many three-dimensional TIs have since been identified, HgTe remains the only known two-dimensional system in this class. Difficulty fabricating HgTe quantum wells has, moreover, hampered their widespread use. With the goal of breaking this logjam, we provide a blueprint for stabilizing a robust TI state in a more readily available two-dimensional material—graphene. Using symmetry arguments, density functional theory, and tight-binding simulations, we predict that graphene endowed with certain heavy adatoms realizes a TI with substantial band gap. For indium and thallium, our most promising adatom candidates, a modest 6% coverage produces an estimated gap near 80 K and 240 K, respectively, which should be detectable in transport or spectroscopic measurements. Engineering such a robust topological phase in graphene could pave the way for a new generation of devices for spintronics, ultra-low-dissipation electronics, and quantum information processing.http://doi.org/10.1103/PhysRevX.1.021001
spellingShingle Conan Weeks
Jun Hu
Jason Alicea
Marcel Franz
Ruqian Wu
Engineering a Robust Quantum Spin Hall State in Graphene via Adatom Deposition
Physical Review X
title Engineering a Robust Quantum Spin Hall State in Graphene via Adatom Deposition
title_full Engineering a Robust Quantum Spin Hall State in Graphene via Adatom Deposition
title_fullStr Engineering a Robust Quantum Spin Hall State in Graphene via Adatom Deposition
title_full_unstemmed Engineering a Robust Quantum Spin Hall State in Graphene via Adatom Deposition
title_short Engineering a Robust Quantum Spin Hall State in Graphene via Adatom Deposition
title_sort engineering a robust quantum spin hall state in graphene via adatom deposition
url http://doi.org/10.1103/PhysRevX.1.021001
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