Toward Self‐Supported Bifunctional Air Electrodes for Flexible Solid‐State Zn–Air Batteries
The demand for flexibility and rechargeability in tandem with high energy density, reliability, and safety in energy‐storage devices to power wearable electronics has translated to significant advances in flexible solid‐state Zn–air batteries (FSZABs) technology. FSZABs using self‐supported bifuncti...
Main Authors: | , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Wiley-VCH
2023-10-01
|
Series: | Small Science |
Subjects: | |
Online Access: | https://doi.org/10.1002/smsc.202300066 |
_version_ | 1797659506463735808 |
---|---|
author | Xixi Wang Lei Xu Chuan Zhou Ngie Hing Wong Jaka Sunarso Ran Ran Wei Zhou Zongping Shao |
author_facet | Xixi Wang Lei Xu Chuan Zhou Ngie Hing Wong Jaka Sunarso Ran Ran Wei Zhou Zongping Shao |
author_sort | Xixi Wang |
collection | DOAJ |
description | The demand for flexibility and rechargeability in tandem with high energy density, reliability, and safety in energy‐storage devices to power wearable electronics has translated to significant advances in flexible solid‐state Zn–air batteries (FSZABs) technology. FSZABs using self‐supported bifunctional air electrodes are currently one of the most attractive alternatives to Li‐ion battery technology for next‐generation wearable electronics. Unlike the conventional powder‐based air electrodes, self‐supported bifunctional air electrodes offer higher electron‐transfer rate, larger specific surface area (and catalyst–reactant–product interfacial contact area), mechanical flexibility, and better operational robustness. To realize their potential nonetheless, self‐supported bifunctional air electrodes should have high and stable bifunctional catalytic activity, low cost, and environmental compatibility. This review first summarizes the three typical configurations and working principles of FSZABs. Then, significant development of self‐supported bifunctional air electrodes for FSZABs and efficient synthesis strategies are emphasized. The review concludes by providing perspectives on how to further improve the electrochemical performance of FSZABs and their suitability for next‐generation wearable electronic devices. |
first_indexed | 2024-03-11T18:16:05Z |
format | Article |
id | doaj.art-4f816a9bae9544a2ba696b68ad066b8d |
institution | Directory Open Access Journal |
issn | 2688-4046 |
language | English |
last_indexed | 2024-03-11T18:16:05Z |
publishDate | 2023-10-01 |
publisher | Wiley-VCH |
record_format | Article |
series | Small Science |
spelling | doaj.art-4f816a9bae9544a2ba696b68ad066b8d2023-10-16T07:06:38ZengWiley-VCHSmall Science2688-40462023-10-01310n/an/a10.1002/smsc.202300066Toward Self‐Supported Bifunctional Air Electrodes for Flexible Solid‐State Zn–Air BatteriesXixi Wang0Lei Xu1Chuan Zhou2Ngie Hing Wong3Jaka Sunarso4Ran Ran5Wei Zhou6Zongping Shao7State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Nanjing 210009 ChinaState Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Nanjing 210009 ChinaState Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Nanjing 210009 ChinaResearch Centre for Sustainable Technologies Faculty of Engineering, Computing, and Science Swinburne University of Technology Jalan Simpang Tiga Kuching Sarawak 93350 MalaysiaResearch Centre for Sustainable Technologies Faculty of Engineering, Computing, and Science Swinburne University of Technology Jalan Simpang Tiga Kuching Sarawak 93350 MalaysiaState Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Nanjing 210009 ChinaState Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Nanjing 210009 ChinaState Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Nanjing 210009 ChinaThe demand for flexibility and rechargeability in tandem with high energy density, reliability, and safety in energy‐storage devices to power wearable electronics has translated to significant advances in flexible solid‐state Zn–air batteries (FSZABs) technology. FSZABs using self‐supported bifunctional air electrodes are currently one of the most attractive alternatives to Li‐ion battery technology for next‐generation wearable electronics. Unlike the conventional powder‐based air electrodes, self‐supported bifunctional air electrodes offer higher electron‐transfer rate, larger specific surface area (and catalyst–reactant–product interfacial contact area), mechanical flexibility, and better operational robustness. To realize their potential nonetheless, self‐supported bifunctional air electrodes should have high and stable bifunctional catalytic activity, low cost, and environmental compatibility. This review first summarizes the three typical configurations and working principles of FSZABs. Then, significant development of self‐supported bifunctional air electrodes for FSZABs and efficient synthesis strategies are emphasized. The review concludes by providing perspectives on how to further improve the electrochemical performance of FSZABs and their suitability for next‐generation wearable electronic devices.https://doi.org/10.1002/smsc.202300066flexible solid-state Zn–air batteriesoxygen reduction and evolution reactionself-supported bifunctional air electrodessynthesis strategieswearable electronic devices |
spellingShingle | Xixi Wang Lei Xu Chuan Zhou Ngie Hing Wong Jaka Sunarso Ran Ran Wei Zhou Zongping Shao Toward Self‐Supported Bifunctional Air Electrodes for Flexible Solid‐State Zn–Air Batteries Small Science flexible solid-state Zn–air batteries oxygen reduction and evolution reaction self-supported bifunctional air electrodes synthesis strategies wearable electronic devices |
title | Toward Self‐Supported Bifunctional Air Electrodes for Flexible Solid‐State Zn–Air Batteries |
title_full | Toward Self‐Supported Bifunctional Air Electrodes for Flexible Solid‐State Zn–Air Batteries |
title_fullStr | Toward Self‐Supported Bifunctional Air Electrodes for Flexible Solid‐State Zn–Air Batteries |
title_full_unstemmed | Toward Self‐Supported Bifunctional Air Electrodes for Flexible Solid‐State Zn–Air Batteries |
title_short | Toward Self‐Supported Bifunctional Air Electrodes for Flexible Solid‐State Zn–Air Batteries |
title_sort | toward self supported bifunctional air electrodes for flexible solid state zn air batteries |
topic | flexible solid-state Zn–air batteries oxygen reduction and evolution reaction self-supported bifunctional air electrodes synthesis strategies wearable electronic devices |
url | https://doi.org/10.1002/smsc.202300066 |
work_keys_str_mv | AT xixiwang towardselfsupportedbifunctionalairelectrodesforflexiblesolidstateznairbatteries AT leixu towardselfsupportedbifunctionalairelectrodesforflexiblesolidstateznairbatteries AT chuanzhou towardselfsupportedbifunctionalairelectrodesforflexiblesolidstateznairbatteries AT ngiehingwong towardselfsupportedbifunctionalairelectrodesforflexiblesolidstateznairbatteries AT jakasunarso towardselfsupportedbifunctionalairelectrodesforflexiblesolidstateznairbatteries AT ranran towardselfsupportedbifunctionalairelectrodesforflexiblesolidstateznairbatteries AT weizhou towardselfsupportedbifunctionalairelectrodesforflexiblesolidstateznairbatteries AT zongpingshao towardselfsupportedbifunctionalairelectrodesforflexiblesolidstateznairbatteries |