Structural characterization of quaternary selenites of tungsten(VI), A2W3SeO12 (A = NH4, Cs, Rb, K or Tl)

The quaternary A2W3SeO12 (A = NH4, Cs, Rb, K or Tl) selenites have been prepared in the form of single crystals by hydrothermal and novel solid-state reactions. They were characterized by X-ray diffraction, thermal and spectroscopic studies. All of them have a hexagonal tungsten oxide (HTO) related...

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Main Authors: Vineela Balisetty, Kanamaluru Vidyasagar
Format: Article
Language:English
Published: International Union of Crystallography 2021-04-01
Series:Acta Crystallographica Section E: Crystallographic Communications
Subjects:
Online Access:http://scripts.iucr.org/cgi-bin/paper?S2056989021002735
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author Vineela Balisetty
Kanamaluru Vidyasagar
author_facet Vineela Balisetty
Kanamaluru Vidyasagar
author_sort Vineela Balisetty
collection DOAJ
description The quaternary A2W3SeO12 (A = NH4, Cs, Rb, K or Tl) selenites have been prepared in the form of single crystals by hydrothermal and novel solid-state reactions. They were characterized by X-ray diffraction, thermal and spectroscopic studies. All of them have a hexagonal tungsten oxide (HTO) related [W3SeO12]2− anionic framework with pyramidally coordinated Se4+ ions. The known A2W3SeO12 (A = NH4, Cs or Rb) compounds are isostructural with the Cs2W3TeO12 compound and have a non-centrosymmetric layered structure containing intra-layer Se—O bonds. The new compound K2W3SeO12(α) is isostructural with the K2W3TeO12 compound and has a centrosymmetric three-dimensional structure containing interlayer Se—O bonds. It is inferred that the new Tl2W3SeO12 compound has the same three-dimensional structure as K2W3SeO12(α).
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spelling doaj.art-5018b7942f504539a39753693b32e9942022-12-22T01:39:59ZengInternational Union of CrystallographyActa Crystallographica Section E: Crystallographic Communications2056-98902021-04-0177440641110.1107/S2056989021002735ru2074Structural characterization of quaternary selenites of tungsten(VI), A2W3SeO12 (A = NH4, Cs, Rb, K or Tl)Vineela Balisetty0Kanamaluru Vidyasagar1Department of Chemistry, Indian Institute of Technology Madras, Chennai 600 036, IndiaDepartment of Chemistry, Indian Institute of Technology Madras, Chennai 600 036, IndiaThe quaternary A2W3SeO12 (A = NH4, Cs, Rb, K or Tl) selenites have been prepared in the form of single crystals by hydrothermal and novel solid-state reactions. They were characterized by X-ray diffraction, thermal and spectroscopic studies. All of them have a hexagonal tungsten oxide (HTO) related [W3SeO12]2− anionic framework with pyramidally coordinated Se4+ ions. The known A2W3SeO12 (A = NH4, Cs or Rb) compounds are isostructural with the Cs2W3TeO12 compound and have a non-centrosymmetric layered structure containing intra-layer Se—O bonds. The new compound K2W3SeO12(α) is isostructural with the K2W3TeO12 compound and has a centrosymmetric three-dimensional structure containing interlayer Se—O bonds. It is inferred that the new Tl2W3SeO12 compound has the same three-dimensional structure as K2W3SeO12(α).http://scripts.iucr.org/cgi-bin/paper?S2056989021002735single-crystal x-ray structurequaternary selenitetungsten
spellingShingle Vineela Balisetty
Kanamaluru Vidyasagar
Structural characterization of quaternary selenites of tungsten(VI), A2W3SeO12 (A = NH4, Cs, Rb, K or Tl)
Acta Crystallographica Section E: Crystallographic Communications
single-crystal x-ray structure
quaternary selenite
tungsten
title Structural characterization of quaternary selenites of tungsten(VI), A2W3SeO12 (A = NH4, Cs, Rb, K or Tl)
title_full Structural characterization of quaternary selenites of tungsten(VI), A2W3SeO12 (A = NH4, Cs, Rb, K or Tl)
title_fullStr Structural characterization of quaternary selenites of tungsten(VI), A2W3SeO12 (A = NH4, Cs, Rb, K or Tl)
title_full_unstemmed Structural characterization of quaternary selenites of tungsten(VI), A2W3SeO12 (A = NH4, Cs, Rb, K or Tl)
title_short Structural characterization of quaternary selenites of tungsten(VI), A2W3SeO12 (A = NH4, Cs, Rb, K or Tl)
title_sort structural characterization of quaternary selenites of tungsten vi a2w3seo12 a nh4 cs rb k or tl
topic single-crystal x-ray structure
quaternary selenite
tungsten
url http://scripts.iucr.org/cgi-bin/paper?S2056989021002735
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