A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene

Nanofibrillated cellulose (NFC) as an environmentally friendly substrate material has superiority for flexible electrothermal composite, while there is currently no research on porous NFC based electrothermal aerogel. Therefore, this work used NFC as a skeleton, combined with multi-walled carbon nan...

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Main Authors: Bing Zhuo, Shuoang Cao, Xinpu Li, Jiahao Liang, Zhihong Bei, Yutong Yang, Quanping Yuan
Format: Article
Language:English
Published: MDPI AG 2020-08-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/25/17/3836
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author Bing Zhuo
Shuoang Cao
Xinpu Li
Jiahao Liang
Zhihong Bei
Yutong Yang
Quanping Yuan
author_facet Bing Zhuo
Shuoang Cao
Xinpu Li
Jiahao Liang
Zhihong Bei
Yutong Yang
Quanping Yuan
author_sort Bing Zhuo
collection DOAJ
description Nanofibrillated cellulose (NFC) as an environmentally friendly substrate material has superiority for flexible electrothermal composite, while there is currently no research on porous NFC based electrothermal aerogel. Therefore, this work used NFC as a skeleton, combined with multi-walled carbon nanotubes (MWCNTs) and graphene (GP), to prepare NFC/MWCNTs/GP aerogel (CCGA) via a simple and economic freeze-drying method. The electrothermal CCGA was finally assembled after connecting CCGA with electrodes. The results show that when the concentration of the NFC/MWCNTs/GP suspension was 5 mg mL<sup>−1</sup> and NFC amount was 80 wt.%, the maximum steady-state temperature rise of electrothermal CCGA at 3000 W m<sup>−2</sup> and 2000 W m<sup>−2</sup> was of about 62.0 °C and 40.4 °C, respectively. The resistance change rate of the CCGA was nearly 15% at the concentration of 7 mg mL<sup>−1</sup> under the power density of 2000 W m<sup>−2</sup>. The formed three-dimensional porous structure is conducive to the heat exchange. Consequently, the electrothermal CCGA can be used as a potential lightweight substrate for efficient electrothermal devices.
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spelling doaj.art-50e9b656e46442459b3ebe21e1ec9b9b2023-11-20T11:07:19ZengMDPI AGMolecules1420-30492020-08-012517383610.3390/molecules25173836A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and GrapheneBing Zhuo0Shuoang Cao1Xinpu Li2Jiahao Liang3Zhihong Bei4Yutong Yang5Quanping Yuan6School of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaNanofibrillated cellulose (NFC) as an environmentally friendly substrate material has superiority for flexible electrothermal composite, while there is currently no research on porous NFC based electrothermal aerogel. Therefore, this work used NFC as a skeleton, combined with multi-walled carbon nanotubes (MWCNTs) and graphene (GP), to prepare NFC/MWCNTs/GP aerogel (CCGA) via a simple and economic freeze-drying method. The electrothermal CCGA was finally assembled after connecting CCGA with electrodes. The results show that when the concentration of the NFC/MWCNTs/GP suspension was 5 mg mL<sup>−1</sup> and NFC amount was 80 wt.%, the maximum steady-state temperature rise of electrothermal CCGA at 3000 W m<sup>−2</sup> and 2000 W m<sup>−2</sup> was of about 62.0 °C and 40.4 °C, respectively. The resistance change rate of the CCGA was nearly 15% at the concentration of 7 mg mL<sup>−1</sup> under the power density of 2000 W m<sup>−2</sup>. The formed three-dimensional porous structure is conducive to the heat exchange. Consequently, the electrothermal CCGA can be used as a potential lightweight substrate for efficient electrothermal devices.https://www.mdpi.com/1420-3049/25/17/3836celluloseaerogelelectrothermal compositecarbon nanotubesgraphene
spellingShingle Bing Zhuo
Shuoang Cao
Xinpu Li
Jiahao Liang
Zhihong Bei
Yutong Yang
Quanping Yuan
A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene
Molecules
cellulose
aerogel
electrothermal composite
carbon nanotubes
graphene
title A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene
title_full A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene
title_fullStr A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene
title_full_unstemmed A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene
title_short A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene
title_sort nanofibrillated cellulose based electrothermal aerogel constructed with carbon nanotubes and graphene
topic cellulose
aerogel
electrothermal composite
carbon nanotubes
graphene
url https://www.mdpi.com/1420-3049/25/17/3836
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