A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene
Nanofibrillated cellulose (NFC) as an environmentally friendly substrate material has superiority for flexible electrothermal composite, while there is currently no research on porous NFC based electrothermal aerogel. Therefore, this work used NFC as a skeleton, combined with multi-walled carbon nan...
Main Authors: | , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
MDPI AG
2020-08-01
|
Series: | Molecules |
Subjects: | |
Online Access: | https://www.mdpi.com/1420-3049/25/17/3836 |
_version_ | 1827707943172177920 |
---|---|
author | Bing Zhuo Shuoang Cao Xinpu Li Jiahao Liang Zhihong Bei Yutong Yang Quanping Yuan |
author_facet | Bing Zhuo Shuoang Cao Xinpu Li Jiahao Liang Zhihong Bei Yutong Yang Quanping Yuan |
author_sort | Bing Zhuo |
collection | DOAJ |
description | Nanofibrillated cellulose (NFC) as an environmentally friendly substrate material has superiority for flexible electrothermal composite, while there is currently no research on porous NFC based electrothermal aerogel. Therefore, this work used NFC as a skeleton, combined with multi-walled carbon nanotubes (MWCNTs) and graphene (GP), to prepare NFC/MWCNTs/GP aerogel (CCGA) via a simple and economic freeze-drying method. The electrothermal CCGA was finally assembled after connecting CCGA with electrodes. The results show that when the concentration of the NFC/MWCNTs/GP suspension was 5 mg mL<sup>−1</sup> and NFC amount was 80 wt.%, the maximum steady-state temperature rise of electrothermal CCGA at 3000 W m<sup>−2</sup> and 2000 W m<sup>−2</sup> was of about 62.0 °C and 40.4 °C, respectively. The resistance change rate of the CCGA was nearly 15% at the concentration of 7 mg mL<sup>−1</sup> under the power density of 2000 W m<sup>−2</sup>. The formed three-dimensional porous structure is conducive to the heat exchange. Consequently, the electrothermal CCGA can be used as a potential lightweight substrate for efficient electrothermal devices. |
first_indexed | 2024-03-10T16:56:45Z |
format | Article |
id | doaj.art-50e9b656e46442459b3ebe21e1ec9b9b |
institution | Directory Open Access Journal |
issn | 1420-3049 |
language | English |
last_indexed | 2024-03-10T16:56:45Z |
publishDate | 2020-08-01 |
publisher | MDPI AG |
record_format | Article |
series | Molecules |
spelling | doaj.art-50e9b656e46442459b3ebe21e1ec9b9b2023-11-20T11:07:19ZengMDPI AGMolecules1420-30492020-08-012517383610.3390/molecules25173836A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and GrapheneBing Zhuo0Shuoang Cao1Xinpu Li2Jiahao Liang3Zhihong Bei4Yutong Yang5Quanping Yuan6School of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaSchool of Resources, Environment and Materials, Guangxi University, Nanning 530004, ChinaNanofibrillated cellulose (NFC) as an environmentally friendly substrate material has superiority for flexible electrothermal composite, while there is currently no research on porous NFC based electrothermal aerogel. Therefore, this work used NFC as a skeleton, combined with multi-walled carbon nanotubes (MWCNTs) and graphene (GP), to prepare NFC/MWCNTs/GP aerogel (CCGA) via a simple and economic freeze-drying method. The electrothermal CCGA was finally assembled after connecting CCGA with electrodes. The results show that when the concentration of the NFC/MWCNTs/GP suspension was 5 mg mL<sup>−1</sup> and NFC amount was 80 wt.%, the maximum steady-state temperature rise of electrothermal CCGA at 3000 W m<sup>−2</sup> and 2000 W m<sup>−2</sup> was of about 62.0 °C and 40.4 °C, respectively. The resistance change rate of the CCGA was nearly 15% at the concentration of 7 mg mL<sup>−1</sup> under the power density of 2000 W m<sup>−2</sup>. The formed three-dimensional porous structure is conducive to the heat exchange. Consequently, the electrothermal CCGA can be used as a potential lightweight substrate for efficient electrothermal devices.https://www.mdpi.com/1420-3049/25/17/3836celluloseaerogelelectrothermal compositecarbon nanotubesgraphene |
spellingShingle | Bing Zhuo Shuoang Cao Xinpu Li Jiahao Liang Zhihong Bei Yutong Yang Quanping Yuan A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene Molecules cellulose aerogel electrothermal composite carbon nanotubes graphene |
title | A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene |
title_full | A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene |
title_fullStr | A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene |
title_full_unstemmed | A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene |
title_short | A Nanofibrillated Cellulose-Based Electrothermal Aerogel Constructed with Carbon Nanotubes and Graphene |
title_sort | nanofibrillated cellulose based electrothermal aerogel constructed with carbon nanotubes and graphene |
topic | cellulose aerogel electrothermal composite carbon nanotubes graphene |
url | https://www.mdpi.com/1420-3049/25/17/3836 |
work_keys_str_mv | AT bingzhuo ananofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT shuoangcao ananofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT xinpuli ananofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT jiahaoliang ananofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT zhihongbei ananofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT yutongyang ananofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT quanpingyuan ananofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT bingzhuo nanofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT shuoangcao nanofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT xinpuli nanofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT jiahaoliang nanofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT zhihongbei nanofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT yutongyang nanofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene AT quanpingyuan nanofibrillatedcellulosebasedelectrothermalaerogelconstructedwithcarbonnanotubesandgraphene |