Photothermal Thin Films with Highly Efficient NIR Conversion for Miniaturized Liquid-Crystal Elastomer Actuators

This work presents the development of highly efficient photothermal thin films (PTFs) and the demonstration of their application on miniaturized polymer-based soft actuators. The proposed PTF, which comprises acrylic-based black paint and EGaIn liquid metal (LM) microdroplets, serves as an excellent...

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Main Authors: Wei-Yi Wang, Bo-You Lin, Yen-Peng Liao, Yao-Joe Yang
Format: Article
Language:English
Published: MDPI AG 2022-07-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/14/15/2997
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author Wei-Yi Wang
Bo-You Lin
Yen-Peng Liao
Yao-Joe Yang
author_facet Wei-Yi Wang
Bo-You Lin
Yen-Peng Liao
Yao-Joe Yang
author_sort Wei-Yi Wang
collection DOAJ
description This work presents the development of highly efficient photothermal thin films (PTFs) and the demonstration of their application on miniaturized polymer-based soft actuators. The proposed PTF, which comprises acrylic-based black paint and EGaIn liquid metal (LM) microdroplets, serves as an excellent absorber for efficiently converting near-infrared (NIR) irradiation into heat for actuating liquid-crystal elastomer (LCE) actuators. The introduction of LM microdroplets into the PTFs effectively increases the overall thermal efficiency of PTFs. Miniaturized soft crawlers monolithically integrated with the NIR-driven LCE actuators are also implemented for demonstrating the application of the proposed PTF. The crawler’s locomotion, which is inspired by the rectilinear movement of snakes, is generated with the proposed PTF for inducing the LC-to-isotropic phase transition of the LCEs. The experimental results show that introducing LM microdroplets into the PTF can effectively reduce the thermal time constants of LCE actuators by 70%. Under periodic on/off NIR illumination cycles, the locomotion of crawlers with different dimensions is also demonstrated. The measurement results indicate that the proposed PTF is not only essential for enabling photothermal LCE actuation but also quite efficient and durable for repeated operation.
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spelling doaj.art-51bd03e937ec49469a31ca96477538db2023-12-03T12:55:56ZengMDPI AGPolymers2073-43602022-07-011415299710.3390/polym14152997Photothermal Thin Films with Highly Efficient NIR Conversion for Miniaturized Liquid-Crystal Elastomer ActuatorsWei-Yi Wang0Bo-You Lin1Yen-Peng Liao2Yao-Joe Yang3Department of Mechanical Engineering, National Taiwan University, Taipei 10617, TaiwanDepartment of Mechanical Engineering, National Taiwan University, Taipei 10617, TaiwanDepartment of Mechanical Engineering, National Taiwan University, Taipei 10617, TaiwanDepartment of Mechanical Engineering, National Taiwan University, Taipei 10617, TaiwanThis work presents the development of highly efficient photothermal thin films (PTFs) and the demonstration of their application on miniaturized polymer-based soft actuators. The proposed PTF, which comprises acrylic-based black paint and EGaIn liquid metal (LM) microdroplets, serves as an excellent absorber for efficiently converting near-infrared (NIR) irradiation into heat for actuating liquid-crystal elastomer (LCE) actuators. The introduction of LM microdroplets into the PTFs effectively increases the overall thermal efficiency of PTFs. Miniaturized soft crawlers monolithically integrated with the NIR-driven LCE actuators are also implemented for demonstrating the application of the proposed PTF. The crawler’s locomotion, which is inspired by the rectilinear movement of snakes, is generated with the proposed PTF for inducing the LC-to-isotropic phase transition of the LCEs. The experimental results show that introducing LM microdroplets into the PTF can effectively reduce the thermal time constants of LCE actuators by 70%. Under periodic on/off NIR illumination cycles, the locomotion of crawlers with different dimensions is also demonstrated. The measurement results indicate that the proposed PTF is not only essential for enabling photothermal LCE actuation but also quite efficient and durable for repeated operation.https://www.mdpi.com/2073-4360/14/15/2997photothermal filmliquid metalshape-memory polymerliquid-crystal elastomerNIR-driven actuatorrectilinear locomotion
spellingShingle Wei-Yi Wang
Bo-You Lin
Yen-Peng Liao
Yao-Joe Yang
Photothermal Thin Films with Highly Efficient NIR Conversion for Miniaturized Liquid-Crystal Elastomer Actuators
Polymers
photothermal film
liquid metal
shape-memory polymer
liquid-crystal elastomer
NIR-driven actuator
rectilinear locomotion
title Photothermal Thin Films with Highly Efficient NIR Conversion for Miniaturized Liquid-Crystal Elastomer Actuators
title_full Photothermal Thin Films with Highly Efficient NIR Conversion for Miniaturized Liquid-Crystal Elastomer Actuators
title_fullStr Photothermal Thin Films with Highly Efficient NIR Conversion for Miniaturized Liquid-Crystal Elastomer Actuators
title_full_unstemmed Photothermal Thin Films with Highly Efficient NIR Conversion for Miniaturized Liquid-Crystal Elastomer Actuators
title_short Photothermal Thin Films with Highly Efficient NIR Conversion for Miniaturized Liquid-Crystal Elastomer Actuators
title_sort photothermal thin films with highly efficient nir conversion for miniaturized liquid crystal elastomer actuators
topic photothermal film
liquid metal
shape-memory polymer
liquid-crystal elastomer
NIR-driven actuator
rectilinear locomotion
url https://www.mdpi.com/2073-4360/14/15/2997
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AT yenpengliao photothermalthinfilmswithhighlyefficientnirconversionforminiaturizedliquidcrystalelastomeractuators
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