Graphene aerogel stabilized phase change material for thermal energy storage

Phase change material (PCM) with thermal energy storage capacity has been a hot topic due to the advantages of satisfying the demand for energy storage, saving and conversion. In this work, graphene oxide (GO) was introduced to prepare a three-dimensional (3D) continuous network of graphene aerogel...

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Main Authors: Yajing Zhao, Kai Zhang, Xin Min, Jun Xiao, Ziling Xu, Zhaohui Huang, Yan'gai Liu, Xiaowen Wu, Minghao Fang
Format: Article
Language:English
Published: Elsevier 2022-12-01
Series:Case Studies in Thermal Engineering
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2214157X22007341
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author Yajing Zhao
Kai Zhang
Xin Min
Jun Xiao
Ziling Xu
Zhaohui Huang
Yan'gai Liu
Xiaowen Wu
Minghao Fang
author_facet Yajing Zhao
Kai Zhang
Xin Min
Jun Xiao
Ziling Xu
Zhaohui Huang
Yan'gai Liu
Xiaowen Wu
Minghao Fang
author_sort Yajing Zhao
collection DOAJ
description Phase change material (PCM) with thermal energy storage capacity has been a hot topic due to the advantages of satisfying the demand for energy storage, saving and conversion. In this work, graphene oxide (GO) was introduced to prepare a three-dimensional (3D) continuous network of graphene aerogel (GA) via a simple hydrothermal process, and the GA was further employed to pack polyethylene glycols (PEG). Benefited from the abundant porous structure and high specific surface area, the mass fraction of PEG in the composite PCM was up to 96.0 wt%. Besides, the heat latent of the composite was 223.2 J/g, illustrating a high energy storage density. Moreover, due to the crosslinking graphene skeleton and its inherent high thermal conductivity, the heat transfer rate was enhanced to 116% of the pure PEG. This work could simultaneously solve the drawbacks of leakage and low thermal conductivity of PCM. And the composite PCM could be considered as a clean, energy-saving and recycled material in the application of building heat preservation.
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spelling doaj.art-51e944fefe994d0385f385a57a1f6d462022-12-22T03:48:48ZengElsevierCase Studies in Thermal Engineering2214-157X2022-12-0140102497Graphene aerogel stabilized phase change material for thermal energy storageYajing Zhao0Kai Zhang1Xin Min2Jun Xiao3Ziling Xu4Zhaohui Huang5Yan'gai Liu6Xiaowen Wu7Minghao Fang8Beijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaBeijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaCorresponding author.; Beijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaBeijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaBeijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaBeijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaBeijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaBeijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaCorresponding author.; Beijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes, National Laboratory of Mineral Materials, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing, 100083, PR ChinaPhase change material (PCM) with thermal energy storage capacity has been a hot topic due to the advantages of satisfying the demand for energy storage, saving and conversion. In this work, graphene oxide (GO) was introduced to prepare a three-dimensional (3D) continuous network of graphene aerogel (GA) via a simple hydrothermal process, and the GA was further employed to pack polyethylene glycols (PEG). Benefited from the abundant porous structure and high specific surface area, the mass fraction of PEG in the composite PCM was up to 96.0 wt%. Besides, the heat latent of the composite was 223.2 J/g, illustrating a high energy storage density. Moreover, due to the crosslinking graphene skeleton and its inherent high thermal conductivity, the heat transfer rate was enhanced to 116% of the pure PEG. This work could simultaneously solve the drawbacks of leakage and low thermal conductivity of PCM. And the composite PCM could be considered as a clean, energy-saving and recycled material in the application of building heat preservation.http://www.sciencedirect.com/science/article/pii/S2214157X22007341Graphene aerogelPolyethylene glycolsThree-dimensional porous structureThermal conductivityPhase change material
spellingShingle Yajing Zhao
Kai Zhang
Xin Min
Jun Xiao
Ziling Xu
Zhaohui Huang
Yan'gai Liu
Xiaowen Wu
Minghao Fang
Graphene aerogel stabilized phase change material for thermal energy storage
Case Studies in Thermal Engineering
Graphene aerogel
Polyethylene glycols
Three-dimensional porous structure
Thermal conductivity
Phase change material
title Graphene aerogel stabilized phase change material for thermal energy storage
title_full Graphene aerogel stabilized phase change material for thermal energy storage
title_fullStr Graphene aerogel stabilized phase change material for thermal energy storage
title_full_unstemmed Graphene aerogel stabilized phase change material for thermal energy storage
title_short Graphene aerogel stabilized phase change material for thermal energy storage
title_sort graphene aerogel stabilized phase change material for thermal energy storage
topic Graphene aerogel
Polyethylene glycols
Three-dimensional porous structure
Thermal conductivity
Phase change material
url http://www.sciencedirect.com/science/article/pii/S2214157X22007341
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AT kaizhang grapheneaerogelstabilizedphasechangematerialforthermalenergystorage
AT xinmin grapheneaerogelstabilizedphasechangematerialforthermalenergystorage
AT junxiao grapheneaerogelstabilizedphasechangematerialforthermalenergystorage
AT zilingxu grapheneaerogelstabilizedphasechangematerialforthermalenergystorage
AT zhaohuihuang grapheneaerogelstabilizedphasechangematerialforthermalenergystorage
AT yangailiu grapheneaerogelstabilizedphasechangematerialforthermalenergystorage
AT xiaowenwu grapheneaerogelstabilizedphasechangematerialforthermalenergystorage
AT minghaofang grapheneaerogelstabilizedphasechangematerialforthermalenergystorage