A Sustainable Dual Cross-Linked Cellulose Hydrogel Electrolyte for High-Performance Zinc-Metal Batteries
Highlights A sustainable dual cross-linked cellulose hydrogel with excellent mechanical strength was fabricated from aqueous alkali hydroxide/urea solution using a sequential chemical and physical cross-linking strategy. The hydrogel electrolyte effectively suppresses dendrites growth and side react...
| Main Authors: | , , , |
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| Format: | Article |
| Language: | English |
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SpringerOpen
2024-02-01
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| Series: | Nano-Micro Letters |
| Subjects: | |
| Online Access: | https://doi.org/10.1007/s40820-024-01329-0 |
| _version_ | 1797273524686028800 |
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| author | Haodong Zhang Xiaotang Gan Yuyang Yan Jinping Zhou |
| author_facet | Haodong Zhang Xiaotang Gan Yuyang Yan Jinping Zhou |
| author_sort | Haodong Zhang |
| collection | DOAJ |
| description | Highlights A sustainable dual cross-linked cellulose hydrogel with excellent mechanical strength was fabricated from aqueous alkali hydroxide/urea solution using a sequential chemical and physical cross-linking strategy. The hydrogel electrolyte effectively suppresses dendrites growth and side reactions to achieve a stable Zn anode (over 2000 h for Zn||Zn cell), which are proved by a multi-perspective and in-depth mechanism investigation. The hydrogel electrolyte is easily accessible and biodegradable, making the zinc batteries attractive in terms of scalability and sustainability. |
| first_indexed | 2024-03-07T14:45:37Z |
| format | Article |
| id | doaj.art-53a8767d156f40abbe4499e5a1d9bd97 |
| institution | Directory Open Access Journal |
| issn | 2311-6706 2150-5551 |
| language | English |
| last_indexed | 2024-03-07T14:45:37Z |
| publishDate | 2024-02-01 |
| publisher | SpringerOpen |
| record_format | Article |
| series | Nano-Micro Letters |
| spelling | doaj.art-53a8767d156f40abbe4499e5a1d9bd972024-03-05T20:01:12ZengSpringerOpenNano-Micro Letters2311-67062150-55512024-02-0116111310.1007/s40820-024-01329-0A Sustainable Dual Cross-Linked Cellulose Hydrogel Electrolyte for High-Performance Zinc-Metal BatteriesHaodong Zhang0Xiaotang Gan1Yuyang Yan2Jinping Zhou3Hubei Engineering Center of Natural Polymers-Based Medical Materials, Key Laboratory of Biomedical Polymers of Ministry of Education, College of Chemistry and Molecular Sciences, Wuhan UniversityHubei Engineering Center of Natural Polymers-Based Medical Materials, Key Laboratory of Biomedical Polymers of Ministry of Education, College of Chemistry and Molecular Sciences, Wuhan UniversityHubei Engineering Center of Natural Polymers-Based Medical Materials, Key Laboratory of Biomedical Polymers of Ministry of Education, College of Chemistry and Molecular Sciences, Wuhan UniversityHubei Engineering Center of Natural Polymers-Based Medical Materials, Key Laboratory of Biomedical Polymers of Ministry of Education, College of Chemistry and Molecular Sciences, Wuhan UniversityHighlights A sustainable dual cross-linked cellulose hydrogel with excellent mechanical strength was fabricated from aqueous alkali hydroxide/urea solution using a sequential chemical and physical cross-linking strategy. The hydrogel electrolyte effectively suppresses dendrites growth and side reactions to achieve a stable Zn anode (over 2000 h for Zn||Zn cell), which are proved by a multi-perspective and in-depth mechanism investigation. The hydrogel electrolyte is easily accessible and biodegradable, making the zinc batteries attractive in terms of scalability and sustainability.https://doi.org/10.1007/s40820-024-01329-0CelluloseDual cross-linkedAqueous rechargeable Zn-metal batteriesHydrogel electrolyte |
| spellingShingle | Haodong Zhang Xiaotang Gan Yuyang Yan Jinping Zhou A Sustainable Dual Cross-Linked Cellulose Hydrogel Electrolyte for High-Performance Zinc-Metal Batteries Nano-Micro Letters Cellulose Dual cross-linked Aqueous rechargeable Zn-metal batteries Hydrogel electrolyte |
| title | A Sustainable Dual Cross-Linked Cellulose Hydrogel Electrolyte for High-Performance Zinc-Metal Batteries |
| title_full | A Sustainable Dual Cross-Linked Cellulose Hydrogel Electrolyte for High-Performance Zinc-Metal Batteries |
| title_fullStr | A Sustainable Dual Cross-Linked Cellulose Hydrogel Electrolyte for High-Performance Zinc-Metal Batteries |
| title_full_unstemmed | A Sustainable Dual Cross-Linked Cellulose Hydrogel Electrolyte for High-Performance Zinc-Metal Batteries |
| title_short | A Sustainable Dual Cross-Linked Cellulose Hydrogel Electrolyte for High-Performance Zinc-Metal Batteries |
| title_sort | sustainable dual cross linked cellulose hydrogel electrolyte for high performance zinc metal batteries |
| topic | Cellulose Dual cross-linked Aqueous rechargeable Zn-metal batteries Hydrogel electrolyte |
| url | https://doi.org/10.1007/s40820-024-01329-0 |
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