X-ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °C

Two types of dedicated Tristructural isotropic (TRISO) nuclear fuel particles, PyC-1 (Kernel/Buffer/PyC) and PyC-2 (Kernel/Buffer/SiC/PyC) from PYCASSO (Pyrocarbon irradiation for creep and swelling/shrinkage of objects) neutron irradiation experiments, were studied. For unirradiated particles, crus...

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Main Authors: Dong Liu, Steven Knol, Jon Ell, Harold Barnard, Mark Davies, Jan A. Vreeling, Robert O. Ritchie
Format: Article
Language:English
Published: Elsevier 2020-02-01
Series:Materials & Design
Online Access:http://www.sciencedirect.com/science/article/pii/S0264127519308202
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author Dong Liu
Steven Knol
Jon Ell
Harold Barnard
Mark Davies
Jan A. Vreeling
Robert O. Ritchie
author_facet Dong Liu
Steven Knol
Jon Ell
Harold Barnard
Mark Davies
Jan A. Vreeling
Robert O. Ritchie
author_sort Dong Liu
collection DOAJ
description Two types of dedicated Tristructural isotropic (TRISO) nuclear fuel particles, PyC-1 (Kernel/Buffer/PyC) and PyC-2 (Kernel/Buffer/SiC/PyC) from PYCASSO (Pyrocarbon irradiation for creep and swelling/shrinkage of objects) neutron irradiation experiments, were studied. For unirradiated particles, crushing experiments using a unique hot cell, combined with in situ X-ray computed micro-tomography (XCT) imaging, were conducted at room temperature (RT) and at 1000 °C. Although the SiC layer on the particles is presumed to provide ‘mechanical stability’ to the TRISO particles, results showed a remarkable reduction (~45%) in the crushing strength of the PyC-2 particles at 1000 °C compared to RT. The fracture patterns of the two types of particles, both at the contact zone and on subsequent propagation, differ significantly at RT and 1000 °C. Further, irradiated particles (irradiation temperature: 1000 ± 20 °C; irradiation doses: 1.08–1.23 dpa and 1.49–1.51 dpa) were imaged by XCT; 250 PyC-1 particles and 223 PyC-2 particles were studied in total and the change in radius/layer thickness in each type was examined. It was found that the buffer densification was lower in PyC-1 particles compared to PyC-2 particles, and the PyC layer shrank in the PyC-I particles, whereas it expanded in PyC-2. Results are discussed in terms of how the residual stresses can impact the high-temperature and post-irradiation behavior of these particles. Keywords: TRISO, PYCASSO, High-temperature X-ray computed micro-tomography, Irradiation induced dimensional change, Uniaxial compression, Contact crushing
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spelling doaj.art-53b0f6ac92514dfb9437eed3a8e665492022-12-21T18:29:17ZengElsevierMaterials & Design0264-12752020-02-01187X-ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °CDong Liu0Steven Knol1Jon Ell2Harold Barnard3Mark Davies4Jan A. Vreeling5Robert O. Ritchie6School of Physics, University of Bristol, UK; Corresponding author.NRG, Petten, the NetherlandsMaterials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, USAAdvanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, USAUSNC, Seattle, USANRG, Petten, the NetherlandsDepartment of Materials Science & Engineering, University of California, Berkeley, USA; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, USATwo types of dedicated Tristructural isotropic (TRISO) nuclear fuel particles, PyC-1 (Kernel/Buffer/PyC) and PyC-2 (Kernel/Buffer/SiC/PyC) from PYCASSO (Pyrocarbon irradiation for creep and swelling/shrinkage of objects) neutron irradiation experiments, were studied. For unirradiated particles, crushing experiments using a unique hot cell, combined with in situ X-ray computed micro-tomography (XCT) imaging, were conducted at room temperature (RT) and at 1000 °C. Although the SiC layer on the particles is presumed to provide ‘mechanical stability’ to the TRISO particles, results showed a remarkable reduction (~45%) in the crushing strength of the PyC-2 particles at 1000 °C compared to RT. The fracture patterns of the two types of particles, both at the contact zone and on subsequent propagation, differ significantly at RT and 1000 °C. Further, irradiated particles (irradiation temperature: 1000 ± 20 °C; irradiation doses: 1.08–1.23 dpa and 1.49–1.51 dpa) were imaged by XCT; 250 PyC-1 particles and 223 PyC-2 particles were studied in total and the change in radius/layer thickness in each type was examined. It was found that the buffer densification was lower in PyC-1 particles compared to PyC-2 particles, and the PyC layer shrank in the PyC-I particles, whereas it expanded in PyC-2. Results are discussed in terms of how the residual stresses can impact the high-temperature and post-irradiation behavior of these particles. Keywords: TRISO, PYCASSO, High-temperature X-ray computed micro-tomography, Irradiation induced dimensional change, Uniaxial compression, Contact crushinghttp://www.sciencedirect.com/science/article/pii/S0264127519308202
spellingShingle Dong Liu
Steven Knol
Jon Ell
Harold Barnard
Mark Davies
Jan A. Vreeling
Robert O. Ritchie
X-ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °C
Materials & Design
title X-ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °C
title_full X-ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °C
title_fullStr X-ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °C
title_full_unstemmed X-ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °C
title_short X-ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °C
title_sort x ray tomography study on the crushing strength and irradiation behaviour of dedicated tristructural isotropic nuclear fuel particles at 1000 °c
url http://www.sciencedirect.com/science/article/pii/S0264127519308202
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