Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating

Abstract Domestic heating is an important source of carbonaceous aerosols in northern China in winter. The seasonal variations, sources, and regional transport of carbonaceous species in PM2.5 in Yuncheng in the winter and summer of 2020–2021 were investigated in this study, with a particular focus...

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Main Authors: Yuewei Sun, Ke Xin, Jing Ai, Huiying Huang, Lingyun Zhang, Weihua Qin, Qing Yu, Jing Chen
Format: Article
Language:English
Published: Springer 2023-11-01
Series:Carbon Research
Subjects:
Online Access:https://doi.org/10.1007/s44246-023-00078-w
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author Yuewei Sun
Ke Xin
Jing Ai
Huiying Huang
Lingyun Zhang
Weihua Qin
Qing Yu
Jing Chen
author_facet Yuewei Sun
Ke Xin
Jing Ai
Huiying Huang
Lingyun Zhang
Weihua Qin
Qing Yu
Jing Chen
author_sort Yuewei Sun
collection DOAJ
description Abstract Domestic heating is an important source of carbonaceous aerosols in northern China in winter. The seasonal variations, sources, and regional transport of carbonaceous species in PM2.5 in Yuncheng in the winter and summer of 2020–2021 were investigated in this study, with a particular focus on the role of domestic heating. Meanwhile, the pollution characteristics of carbonaceous aerosols in Beijing in winter were also investigated for comparison. The mass concentrations of organic carbon (OC) and elemental carbon (EC) and their contributions to PM2.5 were significantly enhanced during the heating period compared to other sampling periods in Yuncheng, however, no obvious differences were observed before and during the heating periods in Beijing. Source apportionment results showed that the heating related emission (50.9%) was the dominant source of total carbon in Yuncheng in the heating period, while vehicular emission (49.6%) was dominant in summer. Combing the positive matrix factorization (PMF) and potential source contribution function (PSCF) analysis, it was concluded that both local and regional heating activities contributed highly to carbonaceous aerosols in Yuncheng. It would be therefore of great environmental benefits to promote the clean residential heating transition in Yuncheng and other similar cities. Graphical Abstract
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spelling doaj.art-53b2e0d4f785445b94065a8f6acaf1492023-11-12T12:31:25ZengSpringerCarbon Research2731-66962023-11-012111310.1007/s44246-023-00078-wTemporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heatingYuewei Sun0Ke Xin1Jing Ai2Huiying Huang3Lingyun Zhang4Weihua Qin5Qing Yu6Jing Chen7State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityAbstract Domestic heating is an important source of carbonaceous aerosols in northern China in winter. The seasonal variations, sources, and regional transport of carbonaceous species in PM2.5 in Yuncheng in the winter and summer of 2020–2021 were investigated in this study, with a particular focus on the role of domestic heating. Meanwhile, the pollution characteristics of carbonaceous aerosols in Beijing in winter were also investigated for comparison. The mass concentrations of organic carbon (OC) and elemental carbon (EC) and their contributions to PM2.5 were significantly enhanced during the heating period compared to other sampling periods in Yuncheng, however, no obvious differences were observed before and during the heating periods in Beijing. Source apportionment results showed that the heating related emission (50.9%) was the dominant source of total carbon in Yuncheng in the heating period, while vehicular emission (49.6%) was dominant in summer. Combing the positive matrix factorization (PMF) and potential source contribution function (PSCF) analysis, it was concluded that both local and regional heating activities contributed highly to carbonaceous aerosols in Yuncheng. It would be therefore of great environmental benefits to promote the clean residential heating transition in Yuncheng and other similar cities. Graphical Abstracthttps://doi.org/10.1007/s44246-023-00078-wCarbonaceous aerosolFenwei plainHeating policySource apportionmentRegional transport
spellingShingle Yuewei Sun
Ke Xin
Jing Ai
Huiying Huang
Lingyun Zhang
Weihua Qin
Qing Yu
Jing Chen
Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating
Carbon Research
Carbonaceous aerosol
Fenwei plain
Heating policy
Source apportionment
Regional transport
title Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating
title_full Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating
title_fullStr Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating
title_full_unstemmed Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating
title_short Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating
title_sort temporal variations sources and regional transport of carbonaceous species in pm2 5 in a northern china city the role of domestic heating
topic Carbonaceous aerosol
Fenwei plain
Heating policy
Source apportionment
Regional transport
url https://doi.org/10.1007/s44246-023-00078-w
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