Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating
Abstract Domestic heating is an important source of carbonaceous aerosols in northern China in winter. The seasonal variations, sources, and regional transport of carbonaceous species in PM2.5 in Yuncheng in the winter and summer of 2020–2021 were investigated in this study, with a particular focus...
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Springer
2023-11-01
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Series: | Carbon Research |
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Online Access: | https://doi.org/10.1007/s44246-023-00078-w |
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author | Yuewei Sun Ke Xin Jing Ai Huiying Huang Lingyun Zhang Weihua Qin Qing Yu Jing Chen |
author_facet | Yuewei Sun Ke Xin Jing Ai Huiying Huang Lingyun Zhang Weihua Qin Qing Yu Jing Chen |
author_sort | Yuewei Sun |
collection | DOAJ |
description | Abstract Domestic heating is an important source of carbonaceous aerosols in northern China in winter. The seasonal variations, sources, and regional transport of carbonaceous species in PM2.5 in Yuncheng in the winter and summer of 2020–2021 were investigated in this study, with a particular focus on the role of domestic heating. Meanwhile, the pollution characteristics of carbonaceous aerosols in Beijing in winter were also investigated for comparison. The mass concentrations of organic carbon (OC) and elemental carbon (EC) and their contributions to PM2.5 were significantly enhanced during the heating period compared to other sampling periods in Yuncheng, however, no obvious differences were observed before and during the heating periods in Beijing. Source apportionment results showed that the heating related emission (50.9%) was the dominant source of total carbon in Yuncheng in the heating period, while vehicular emission (49.6%) was dominant in summer. Combing the positive matrix factorization (PMF) and potential source contribution function (PSCF) analysis, it was concluded that both local and regional heating activities contributed highly to carbonaceous aerosols in Yuncheng. It would be therefore of great environmental benefits to promote the clean residential heating transition in Yuncheng and other similar cities. Graphical Abstract |
first_indexed | 2024-03-11T11:00:05Z |
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id | doaj.art-53b2e0d4f785445b94065a8f6acaf149 |
institution | Directory Open Access Journal |
issn | 2731-6696 |
language | English |
last_indexed | 2024-03-11T11:00:05Z |
publishDate | 2023-11-01 |
publisher | Springer |
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series | Carbon Research |
spelling | doaj.art-53b2e0d4f785445b94065a8f6acaf1492023-11-12T12:31:25ZengSpringerCarbon Research2731-66962023-11-012111310.1007/s44246-023-00078-wTemporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heatingYuewei Sun0Ke Xin1Jing Ai2Huiying Huang3Lingyun Zhang4Weihua Qin5Qing Yu6Jing Chen7State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Beijing Normal UniversityAbstract Domestic heating is an important source of carbonaceous aerosols in northern China in winter. The seasonal variations, sources, and regional transport of carbonaceous species in PM2.5 in Yuncheng in the winter and summer of 2020–2021 were investigated in this study, with a particular focus on the role of domestic heating. Meanwhile, the pollution characteristics of carbonaceous aerosols in Beijing in winter were also investigated for comparison. The mass concentrations of organic carbon (OC) and elemental carbon (EC) and their contributions to PM2.5 were significantly enhanced during the heating period compared to other sampling periods in Yuncheng, however, no obvious differences were observed before and during the heating periods in Beijing. Source apportionment results showed that the heating related emission (50.9%) was the dominant source of total carbon in Yuncheng in the heating period, while vehicular emission (49.6%) was dominant in summer. Combing the positive matrix factorization (PMF) and potential source contribution function (PSCF) analysis, it was concluded that both local and regional heating activities contributed highly to carbonaceous aerosols in Yuncheng. It would be therefore of great environmental benefits to promote the clean residential heating transition in Yuncheng and other similar cities. Graphical Abstracthttps://doi.org/10.1007/s44246-023-00078-wCarbonaceous aerosolFenwei plainHeating policySource apportionmentRegional transport |
spellingShingle | Yuewei Sun Ke Xin Jing Ai Huiying Huang Lingyun Zhang Weihua Qin Qing Yu Jing Chen Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating Carbon Research Carbonaceous aerosol Fenwei plain Heating policy Source apportionment Regional transport |
title | Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating |
title_full | Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating |
title_fullStr | Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating |
title_full_unstemmed | Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating |
title_short | Temporal variations, sources, and regional transport of carbonaceous species in PM2.5 in a northern China city: the role of domestic heating |
title_sort | temporal variations sources and regional transport of carbonaceous species in pm2 5 in a northern china city the role of domestic heating |
topic | Carbonaceous aerosol Fenwei plain Heating policy Source apportionment Regional transport |
url | https://doi.org/10.1007/s44246-023-00078-w |
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