Experimental Study and Modeling of Mass Transfer Flux of CO2 Absorption with Amine Solution in Bubble Column

In this study, the effective parameters in mass transfer in the process of gas absorption in the bubble column by amine solvents have been investigated. Also, the aim of this study is to present a general and accurate correlation with the least simplifying assumptions to calculate the mass transfer...

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Main Authors: Hasan Pashaei, Fahimeh Mirzaei, Ahad Ghaemi
Format: Article
Language:English
Published: University of Tehran 2022-12-01
Series:Journal of Chemical and Petroleum Engineering
Subjects:
Online Access:https://jchpe.ut.ac.ir/article_88813.html
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author Hasan Pashaei
Fahimeh Mirzaei
Ahad Ghaemi
author_facet Hasan Pashaei
Fahimeh Mirzaei
Ahad Ghaemi
author_sort Hasan Pashaei
collection DOAJ
description In this study, the effective parameters in mass transfer in the process of gas absorption in the bubble column by amine solvents have been investigated. Also, the aim of this study is to present a general and accurate correlation with the least simplifying assumptions to calculate the mass transfer flux of gas phase to liquid phase components in three electrolyte systems MDEA-Pz, MEA-Pz, and MEA-MDEA. The effect of parameters on mass transfer such as retention time, apparent gas velocity, liquid phase properties, operating conditions, type of distributor, and bubble characteristics was analyzed. Effective parameters were expressed to achieve functional correlations using dimensionless numbers by using the pi-Buckingham theorem. The correlation coefficients for MDEA-Pz, MEA-Pz, and MDEA-MEA were obtained at 0.951, 0.981, and 0.924, respectively. The mean relative error obtained from predicting the mass transfer flux correlation for all three MDEA-Pz, MEA-Pz, and MDEA-MEA amine combination systems was 3.6, 4.5, and 4.8%, respectively. The results showed that the proposed correlations for mass transfer flux compared to other correlations have high accuracy.
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spelling doaj.art-54d3571ca345415982d0f0f88b7d3d782023-02-09T10:46:36ZengUniversity of TehranJournal of Chemical and Petroleum Engineering2423-673X2423-67212022-12-0156221523110.22059/JCHPE.2022.345476.1396Experimental Study and Modeling of Mass Transfer Flux of CO2 Absorption with Amine Solution in Bubble ColumnHasan Pashaei0Fahimeh Mirzaei1Ahad Ghaemi2School of Chemical, Petroleum, and Gas Engineering, Iran University of Science and Technology, IranSchool of Chemical, Petroleum, and Gas Engineering, Iran University of Science and Technology, IranSchool of Chemical, Petroleum, and Gas Engineering, Iran University of Science and Technology, IranIn this study, the effective parameters in mass transfer in the process of gas absorption in the bubble column by amine solvents have been investigated. Also, the aim of this study is to present a general and accurate correlation with the least simplifying assumptions to calculate the mass transfer flux of gas phase to liquid phase components in three electrolyte systems MDEA-Pz, MEA-Pz, and MEA-MDEA. The effect of parameters on mass transfer such as retention time, apparent gas velocity, liquid phase properties, operating conditions, type of distributor, and bubble characteristics was analyzed. Effective parameters were expressed to achieve functional correlations using dimensionless numbers by using the pi-Buckingham theorem. The correlation coefficients for MDEA-Pz, MEA-Pz, and MDEA-MEA were obtained at 0.951, 0.981, and 0.924, respectively. The mean relative error obtained from predicting the mass transfer flux correlation for all three MDEA-Pz, MEA-Pz, and MDEA-MEA amine combination systems was 3.6, 4.5, and 4.8%, respectively. The results showed that the proposed correlations for mass transfer flux compared to other correlations have high accuracy.https://jchpe.ut.ac.ir/article_88813.htmlabsorptioncarbon dioxidemass transfer fluxamine solutionbubble columnpi-buckingham
spellingShingle Hasan Pashaei
Fahimeh Mirzaei
Ahad Ghaemi
Experimental Study and Modeling of Mass Transfer Flux of CO2 Absorption with Amine Solution in Bubble Column
Journal of Chemical and Petroleum Engineering
absorption
carbon dioxide
mass transfer flux
amine solution
bubble column
pi-buckingham
title Experimental Study and Modeling of Mass Transfer Flux of CO2 Absorption with Amine Solution in Bubble Column
title_full Experimental Study and Modeling of Mass Transfer Flux of CO2 Absorption with Amine Solution in Bubble Column
title_fullStr Experimental Study and Modeling of Mass Transfer Flux of CO2 Absorption with Amine Solution in Bubble Column
title_full_unstemmed Experimental Study and Modeling of Mass Transfer Flux of CO2 Absorption with Amine Solution in Bubble Column
title_short Experimental Study and Modeling of Mass Transfer Flux of CO2 Absorption with Amine Solution in Bubble Column
title_sort experimental study and modeling of mass transfer flux of co2 absorption with amine solution in bubble column
topic absorption
carbon dioxide
mass transfer flux
amine solution
bubble column
pi-buckingham
url https://jchpe.ut.ac.ir/article_88813.html
work_keys_str_mv AT hasanpashaei experimentalstudyandmodelingofmasstransferfluxofco2absorptionwithaminesolutioninbubblecolumn
AT fahimehmirzaei experimentalstudyandmodelingofmasstransferfluxofco2absorptionwithaminesolutioninbubblecolumn
AT ahadghaemi experimentalstudyandmodelingofmasstransferfluxofco2absorptionwithaminesolutioninbubblecolumn