Effect of neutron irradiation on the microstructure of tungsten

Two grades of pure tungsten, single and polycrystalline, were irradiated for 282 days in the HFR reactor, Petten, at 900 °C to an average damage level of 1.6dpa. Each grade of tungsten was investigated using the transmission electron microscope (TEM) to assess the effect of neutron irradiation on tu...

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Main Authors: M. Klimenkov, U. Jäntsch, M. Rieth, H.C. Schneider, D.E.J. Armstrong, J. Gibson, S.G. Roberts
Format: Article
Language:English
Published: Elsevier 2016-12-01
Series:Nuclear Materials and Energy
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2352179115300867
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author M. Klimenkov
U. Jäntsch
M. Rieth
H.C. Schneider
D.E.J. Armstrong
J. Gibson
S.G. Roberts
author_facet M. Klimenkov
U. Jäntsch
M. Rieth
H.C. Schneider
D.E.J. Armstrong
J. Gibson
S.G. Roberts
author_sort M. Klimenkov
collection DOAJ
description Two grades of pure tungsten, single and polycrystalline, were irradiated for 282 days in the HFR reactor, Petten, at 900 °C to an average damage level of 1.6dpa. Each grade of tungsten was investigated using the transmission electron microscope (TEM) to assess the effect of neutron irradiation on tungsten microstructure. Investigations revealed the formation of faceted cavities, whose diameter varies from 4 to 14nm in both materials. The cavities are homogeneously distributed only inside single crystalline tungsten. The local distribution of cavities in polycrystalline tungsten is strongly influenced by grain boundaries. The number densities of cavities were measured to be 4×1021 m−3 for polycrystalline and 2.5×1021 m−3 for single crystalline tungsten. This corresponds to volumetric densities of 0.45% and 0.33% respectively. High-resolution transmission electron microscopy (HRTEM) revealed that faces of cavities are oriented in (110) plane. Analytical investigations showed precipitation of rhenium and osmium produced by a transmutation reaction around cavities and at grain boundaries.
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spelling doaj.art-55220a788be54d2b99fa598395e798592022-12-22T02:15:43ZengElsevierNuclear Materials and Energy2352-17912016-12-019C48048310.1016/j.nme.2016.09.010Effect of neutron irradiation on the microstructure of tungstenM. Klimenkov0U. Jäntsch1M. Rieth2H.C. Schneider3D.E.J. Armstrong4J. Gibson5S.G. Roberts6Karlsruhe Institute of Technology (KIT), Institute for Applied Materials, 76021 Karlsruhe, GermanyKarlsruhe Institute of Technology (KIT), Institute for Applied Materials, 76021 Karlsruhe, GermanyKarlsruhe Institute of Technology (KIT), Institute for Applied Materials, 76021 Karlsruhe, GermanyKarlsruhe Institute of Technology (KIT), Institute for Applied Materials, 76021 Karlsruhe, GermanyUniversity of Oxford, Department of Materials, Oxford, UKUniversity of Oxford, Department of Materials, Oxford, UKUniversity of Oxford, Department of Materials, Oxford, UKTwo grades of pure tungsten, single and polycrystalline, were irradiated for 282 days in the HFR reactor, Petten, at 900 °C to an average damage level of 1.6dpa. Each grade of tungsten was investigated using the transmission electron microscope (TEM) to assess the effect of neutron irradiation on tungsten microstructure. Investigations revealed the formation of faceted cavities, whose diameter varies from 4 to 14nm in both materials. The cavities are homogeneously distributed only inside single crystalline tungsten. The local distribution of cavities in polycrystalline tungsten is strongly influenced by grain boundaries. The number densities of cavities were measured to be 4×1021 m−3 for polycrystalline and 2.5×1021 m−3 for single crystalline tungsten. This corresponds to volumetric densities of 0.45% and 0.33% respectively. High-resolution transmission electron microscopy (HRTEM) revealed that faces of cavities are oriented in (110) plane. Analytical investigations showed precipitation of rhenium and osmium produced by a transmutation reaction around cavities and at grain boundaries.http://www.sciencedirect.com/science/article/pii/S2352179115300867TungstenNeutron irradiationMicrostructureTransmutation
spellingShingle M. Klimenkov
U. Jäntsch
M. Rieth
H.C. Schneider
D.E.J. Armstrong
J. Gibson
S.G. Roberts
Effect of neutron irradiation on the microstructure of tungsten
Nuclear Materials and Energy
Tungsten
Neutron irradiation
Microstructure
Transmutation
title Effect of neutron irradiation on the microstructure of tungsten
title_full Effect of neutron irradiation on the microstructure of tungsten
title_fullStr Effect of neutron irradiation on the microstructure of tungsten
title_full_unstemmed Effect of neutron irradiation on the microstructure of tungsten
title_short Effect of neutron irradiation on the microstructure of tungsten
title_sort effect of neutron irradiation on the microstructure of tungsten
topic Tungsten
Neutron irradiation
Microstructure
Transmutation
url http://www.sciencedirect.com/science/article/pii/S2352179115300867
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