Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonics

We describe a powerful and intuitive theoretical technique for modeling light–matter interactions in classical and quantum nanoplasmonics. Our approach uses a quasinormal mode (QNM) expansion of the photon Green function within a metal nanoresonator of arbitrary shape, together with a Dyson equation...

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Main Authors: Rong-Chun Ge, Philip Trøst Kristensen, Jeff F Young, Stephen Hughes
Format: Article
Language:English
Published: IOP Publishing 2014-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/16/11/113048
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author Rong-Chun Ge
Philip Trøst Kristensen
Jeff F Young
Stephen Hughes
author_facet Rong-Chun Ge
Philip Trøst Kristensen
Jeff F Young
Stephen Hughes
author_sort Rong-Chun Ge
collection DOAJ
description We describe a powerful and intuitive theoretical technique for modeling light–matter interactions in classical and quantum nanoplasmonics. Our approach uses a quasinormal mode (QNM) expansion of the photon Green function within a metal nanoresonator of arbitrary shape, together with a Dyson equation, to derive an expression for the spontaneous decay rate and far field propagator from dipole oscillators outside resonators. For a single QNM, at field positions outside the quasi-static coupling regime, we give a closed form solution for the Purcell factor and generalized effective mode volume. We augment this with an analytic expression for the divergent local density of optical states very near the metal surface, which allows us to derive a simple and highly accurate expression for the electric field outside the metal resonator at distances from a few nanometers to infinity. This intuitive formalism provides an enormous simplification over full numerical calculations and fixes several pending problems in QNM theory.
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spelling doaj.art-55273a5da1af4cbb8b98ff0cf8cd57312023-08-08T11:21:56ZengIOP PublishingNew Journal of Physics1367-26302014-01-01161111304810.1088/1367-2630/16/11/113048Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonicsRong-Chun Ge0Philip Trøst Kristensen1Jeff F Young2Stephen Hughes3Department of Physics , Engineering Physics and Astronomy, Queenʼs University, Kingston, Ontario, K7L 3N6, CanadaDTU Fotonik, Technical University of Denmark , DK-2800 Kongens Lyngby, DenmarkDepartment of Physics and Astronomy , University of British Columbia, 6224 Agricultural Road, Vancouver, British Columbia, V6T 1Z1, CanadaDepartment of Physics , Engineering Physics and Astronomy, Queenʼs University, Kingston, Ontario, K7L 3N6, CanadaWe describe a powerful and intuitive theoretical technique for modeling light–matter interactions in classical and quantum nanoplasmonics. Our approach uses a quasinormal mode (QNM) expansion of the photon Green function within a metal nanoresonator of arbitrary shape, together with a Dyson equation, to derive an expression for the spontaneous decay rate and far field propagator from dipole oscillators outside resonators. For a single QNM, at field positions outside the quasi-static coupling regime, we give a closed form solution for the Purcell factor and generalized effective mode volume. We augment this with an analytic expression for the divergent local density of optical states very near the metal surface, which allows us to derive a simple and highly accurate expression for the electric field outside the metal resonator at distances from a few nanometers to infinity. This intuitive formalism provides an enormous simplification over full numerical calculations and fixes several pending problems in QNM theory.https://doi.org/10.1088/1367-2630/16/11/113048nanoplasmonicsquasinormal modeseffective mode volumePurcell factorsquantum dotslight–matter interactions
spellingShingle Rong-Chun Ge
Philip Trøst Kristensen
Jeff F Young
Stephen Hughes
Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonics
New Journal of Physics
nanoplasmonics
quasinormal modes
effective mode volume
Purcell factors
quantum dots
light–matter interactions
title Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonics
title_full Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonics
title_fullStr Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonics
title_full_unstemmed Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonics
title_short Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonics
title_sort quasinormal mode approach to modelling light emission and propagation in nanoplasmonics
topic nanoplasmonics
quasinormal modes
effective mode volume
Purcell factors
quantum dots
light–matter interactions
url https://doi.org/10.1088/1367-2630/16/11/113048
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