Analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundment

Results are presented of the characterization of radioactivity inventory of Zapadnoe uranium mill tailings impoundment situated at Pridneprovsky Chemical Plant (PChP; Dneprodzerzhinsk, Ukraine). Analyses of radioactivity data set based on analytical studies of core material from 15 characterization...

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Main Authors: D. O. Bugai, G. V. Laptev, O. S. Skalskyy, T. V. Lavrova, R. Avila
Format: Article
Language:English
Published: Institute for Nuclear Research, National Academy of Sciences of Ukraine 2015-10-01
Series:Âderna Fìzika ta Energetika
Subjects:
Online Access:http://jnpae.kinr.kiev.ua/16.3/html/16.3.0254.html
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author D. O. Bugai
G. V. Laptev
O. S. Skalskyy
T. V. Lavrova
R. Avila
author_facet D. O. Bugai
G. V. Laptev
O. S. Skalskyy
T. V. Lavrova
R. Avila
author_sort D. O. Bugai
collection DOAJ
description Results are presented of the characterization of radioactivity inventory of Zapadnoe uranium mill tailings impoundment situated at Pridneprovsky Chemical Plant (PChP; Dneprodzerzhinsk, Ukraine). Analyses of radioactivity data set based on analytical studies of core material from 15 characterization boreholes allowed significantly refining waste volume and radioactivity inventory estimates. Geostatistical analyses using variogram function have established that radioactivity distribution in Zapadnoe tailings is characterized by regular spatial correlation patterns. Ordinary kriging method was applied to assess distribution of radioactivity in 3D. Results of statistical analyses suggest significant redistribution of uranium in the dissolved form in the residues (presumably due to water infiltration process). The developed structural model for radioactivity distribution is used for further risk assessment analyses. Derived radioactivity correlation scales can be used for optimization of sample collection when characterizing the PChP Site and similar contaminated sites elsewhere.
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spelling doaj.art-56025d32e79d4a4eb6c62c117796ea812022-12-22T02:46:05ZengInstitute for Nuclear Research, National Academy of Sciences of UkraineÂderna Fìzika ta Energetika1818-331X2074-05652015-10-01163254262Analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundmentD. O. Bugai0G. V. Laptev1O. S. Skalskyy2T. V. Lavrova3R. Avila4Institute of Geological Sciences, National Academy of Sciences of Ukraine, Kyiv, Ukraine Ukrainian Hydrometeorological Institute, National Academy of Sciences and State Emergency Service of Ukraine, Kyiv, Ukraine Institute of Geological Sciences, National Academy of Sciences of Ukraine, Kyiv, Ukraine Ukrainian Hydrometeorological Institute, National Academy of Sciences and State Emergency Service of Ukraine, Kyiv, Ukraine Facilia AB, Bromma, Sweden Results are presented of the characterization of radioactivity inventory of Zapadnoe uranium mill tailings impoundment situated at Pridneprovsky Chemical Plant (PChP; Dneprodzerzhinsk, Ukraine). Analyses of radioactivity data set based on analytical studies of core material from 15 characterization boreholes allowed significantly refining waste volume and radioactivity inventory estimates. Geostatistical analyses using variogram function have established that radioactivity distribution in Zapadnoe tailings is characterized by regular spatial correlation patterns. Ordinary kriging method was applied to assess distribution of radioactivity in 3D. Results of statistical analyses suggest significant redistribution of uranium in the dissolved form in the residues (presumably due to water infiltration process). The developed structural model for radioactivity distribution is used for further risk assessment analyses. Derived radioactivity correlation scales can be used for optimization of sample collection when characterizing the PChP Site and similar contaminated sites elsewhere.http://jnpae.kinr.kiev.ua/16.3/html/16.3.0254.htmluranium mill tailingsPridneprovsky Chemical Plantcharacterization of radioactivity inventorygeostatistical analysis
spellingShingle D. O. Bugai
G. V. Laptev
O. S. Skalskyy
T. V. Lavrova
R. Avila
Analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundment
Âderna Fìzika ta Energetika
uranium mill tailings
Pridneprovsky Chemical Plant
characterization of radioactivity inventory
geostatistical analysis
title Analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundment
title_full Analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundment
title_fullStr Analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundment
title_full_unstemmed Analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundment
title_short Analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundment
title_sort analysis of spatial distribution and inventory of radioactivity within the uranium mill tailings impoundment
topic uranium mill tailings
Pridneprovsky Chemical Plant
characterization of radioactivity inventory
geostatistical analysis
url http://jnpae.kinr.kiev.ua/16.3/html/16.3.0254.html
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AT osskalskyy analysisofspatialdistributionandinventoryofradioactivitywithintheuraniummilltailingsimpoundment
AT tvlavrova analysisofspatialdistributionandinventoryofradioactivitywithintheuraniummilltailingsimpoundment
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