Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity
Measurements of cloud condensation nuclei (CCN) concentrations, single particle composition and size distributions at a high-elevation research site from March 2011 are presented. <br><br> The temporal evolution of detailed single particle composition is compared with changes in CCN acti...
Main Authors: | , , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Copernicus Publications
2013-12-01
|
Series: | Atmospheric Chemistry and Physics |
Online Access: | http://www.atmos-chem-phys.net/13/11839/2013/acp-13-11839-2013.pdf |
_version_ | 1819239915421958144 |
---|---|
author | B. Friedman A. Zelenyuk J. Beranek G. Kulkarni M. Pekour A. Gannet Hallar I. B. McCubbin J. A. Thornton D. J Cziczo |
author_facet | B. Friedman A. Zelenyuk J. Beranek G. Kulkarni M. Pekour A. Gannet Hallar I. B. McCubbin J. A. Thornton D. J Cziczo |
author_sort | B. Friedman |
collection | DOAJ |
description | Measurements of cloud condensation nuclei (CCN) concentrations, single
particle composition and size distributions at a high-elevation research
site from March 2011 are presented.
<br><br>
The temporal evolution of detailed single particle composition is compared
with changes in CCN activation on four days, two of which include new
particle formation and growth events. Sulfate-containing particles dominated
the single particle composition by number; biomass burning particles, sea
salt particles, and particles containing organic components were also
present. CCN activation largely followed the behavior of the
sulfate-containing particle types; biomass burning particle types also
likely contained hygroscopic material that impacted CCN activation. Newly
formed particles also may contribute to CCN activation at higher
supersaturation conditions. Derived aerosol hygroscopicity parameters from
the size distribution and CCN concentration measurements are within the
range of previous reports of remote continental kappa values. |
first_indexed | 2024-12-23T13:59:42Z |
format | Article |
id | doaj.art-56028d26111a48d88c7f28d23588ad1b |
institution | Directory Open Access Journal |
issn | 1680-7316 1680-7324 |
language | English |
last_indexed | 2024-12-23T13:59:42Z |
publishDate | 2013-12-01 |
publisher | Copernicus Publications |
record_format | Article |
series | Atmospheric Chemistry and Physics |
spelling | doaj.art-56028d26111a48d88c7f28d23588ad1b2022-12-21T17:44:21ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242013-12-011323118391185110.5194/acp-13-11839-2013Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activityB. Friedman0A. Zelenyuk1J. Beranek2G. Kulkarni3M. Pekour4A. Gannet Hallar5I. B. McCubbin6J. A. Thornton7D. J Cziczo8Department of Atmospheric Sciences, University of Washington, Seattle, WA, USAPacific Northwest National Laboratory, Richland, WA, USAPacific Northwest National Laboratory, Richland, WA, USAPacific Northwest National Laboratory, Richland, WA, USAPacific Northwest National Laboratory, Richland, WA, USAStorm Peak Laboratory, Desert Research Institute, Steamboat Springs, CO, USAStorm Peak Laboratory, Desert Research Institute, Steamboat Springs, CO, USADepartment of Atmospheric Sciences, University of Washington, Seattle, WA, USAEarth, Atmospheric, and Planetary Sciences Department, Massachusetts Institute of Technology, Cambridge, MA, USAMeasurements of cloud condensation nuclei (CCN) concentrations, single particle composition and size distributions at a high-elevation research site from March 2011 are presented. <br><br> The temporal evolution of detailed single particle composition is compared with changes in CCN activation on four days, two of which include new particle formation and growth events. Sulfate-containing particles dominated the single particle composition by number; biomass burning particles, sea salt particles, and particles containing organic components were also present. CCN activation largely followed the behavior of the sulfate-containing particle types; biomass burning particle types also likely contained hygroscopic material that impacted CCN activation. Newly formed particles also may contribute to CCN activation at higher supersaturation conditions. Derived aerosol hygroscopicity parameters from the size distribution and CCN concentration measurements are within the range of previous reports of remote continental kappa values.http://www.atmos-chem-phys.net/13/11839/2013/acp-13-11839-2013.pdf |
spellingShingle | B. Friedman A. Zelenyuk J. Beranek G. Kulkarni M. Pekour A. Gannet Hallar I. B. McCubbin J. A. Thornton D. J Cziczo Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity Atmospheric Chemistry and Physics |
title | Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity |
title_full | Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity |
title_fullStr | Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity |
title_full_unstemmed | Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity |
title_short | Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity |
title_sort | aerosol measurements at a high elevation site composition size and cloud condensation nuclei activity |
url | http://www.atmos-chem-phys.net/13/11839/2013/acp-13-11839-2013.pdf |
work_keys_str_mv | AT bfriedman aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity AT azelenyuk aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity AT jberanek aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity AT gkulkarni aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity AT mpekour aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity AT agannethallar aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity AT ibmccubbin aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity AT jathornton aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity AT djcziczo aerosolmeasurementsatahighelevationsitecompositionsizeandcloudcondensationnucleiactivity |