Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity

Measurements of cloud condensation nuclei (CCN) concentrations, single particle composition and size distributions at a high-elevation research site from March 2011 are presented. <br><br> The temporal evolution of detailed single particle composition is compared with changes in CCN acti...

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Main Authors: B. Friedman, A. Zelenyuk, J. Beranek, G. Kulkarni, M. Pekour, A. Gannet Hallar, I. B. McCubbin, J. A. Thornton, D. J Cziczo
Format: Article
Language:English
Published: Copernicus Publications 2013-12-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/13/11839/2013/acp-13-11839-2013.pdf
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author B. Friedman
A. Zelenyuk
J. Beranek
G. Kulkarni
M. Pekour
A. Gannet Hallar
I. B. McCubbin
J. A. Thornton
D. J Cziczo
author_facet B. Friedman
A. Zelenyuk
J. Beranek
G. Kulkarni
M. Pekour
A. Gannet Hallar
I. B. McCubbin
J. A. Thornton
D. J Cziczo
author_sort B. Friedman
collection DOAJ
description Measurements of cloud condensation nuclei (CCN) concentrations, single particle composition and size distributions at a high-elevation research site from March 2011 are presented. <br><br> The temporal evolution of detailed single particle composition is compared with changes in CCN activation on four days, two of which include new particle formation and growth events. Sulfate-containing particles dominated the single particle composition by number; biomass burning particles, sea salt particles, and particles containing organic components were also present. CCN activation largely followed the behavior of the sulfate-containing particle types; biomass burning particle types also likely contained hygroscopic material that impacted CCN activation. Newly formed particles also may contribute to CCN activation at higher supersaturation conditions. Derived aerosol hygroscopicity parameters from the size distribution and CCN concentration measurements are within the range of previous reports of remote continental kappa values.
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spelling doaj.art-56028d26111a48d88c7f28d23588ad1b2022-12-21T17:44:21ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242013-12-011323118391185110.5194/acp-13-11839-2013Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activityB. Friedman0A. Zelenyuk1J. Beranek2G. Kulkarni3M. Pekour4A. Gannet Hallar5I. B. McCubbin6J. A. Thornton7D. J Cziczo8Department of Atmospheric Sciences, University of Washington, Seattle, WA, USAPacific Northwest National Laboratory, Richland, WA, USAPacific Northwest National Laboratory, Richland, WA, USAPacific Northwest National Laboratory, Richland, WA, USAPacific Northwest National Laboratory, Richland, WA, USAStorm Peak Laboratory, Desert Research Institute, Steamboat Springs, CO, USAStorm Peak Laboratory, Desert Research Institute, Steamboat Springs, CO, USADepartment of Atmospheric Sciences, University of Washington, Seattle, WA, USAEarth, Atmospheric, and Planetary Sciences Department, Massachusetts Institute of Technology, Cambridge, MA, USAMeasurements of cloud condensation nuclei (CCN) concentrations, single particle composition and size distributions at a high-elevation research site from March 2011 are presented. <br><br> The temporal evolution of detailed single particle composition is compared with changes in CCN activation on four days, two of which include new particle formation and growth events. Sulfate-containing particles dominated the single particle composition by number; biomass burning particles, sea salt particles, and particles containing organic components were also present. CCN activation largely followed the behavior of the sulfate-containing particle types; biomass burning particle types also likely contained hygroscopic material that impacted CCN activation. Newly formed particles also may contribute to CCN activation at higher supersaturation conditions. Derived aerosol hygroscopicity parameters from the size distribution and CCN concentration measurements are within the range of previous reports of remote continental kappa values.http://www.atmos-chem-phys.net/13/11839/2013/acp-13-11839-2013.pdf
spellingShingle B. Friedman
A. Zelenyuk
J. Beranek
G. Kulkarni
M. Pekour
A. Gannet Hallar
I. B. McCubbin
J. A. Thornton
D. J Cziczo
Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity
Atmospheric Chemistry and Physics
title Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity
title_full Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity
title_fullStr Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity
title_full_unstemmed Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity
title_short Aerosol measurements at a high-elevation site: composition, size, and cloud condensation nuclei activity
title_sort aerosol measurements at a high elevation site composition size and cloud condensation nuclei activity
url http://www.atmos-chem-phys.net/13/11839/2013/acp-13-11839-2013.pdf
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