Third-order nonlinear optical responses of CuO nanosheets for ultrafast pulse generation

As a representative transition metal oxide, cupric oxide (CuO) has attracted a lot of interest in miscellaneous fields. In the present work, the prominent third-order nonlinear optical (NLO) features of CuO nanosheets were demonstrated via the typical Z-scan technique at 1 μm. The open-aperture (OA)...

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Main Authors: Li Dong, Hongwei Chu, Ying Li, Shengzhi Zhao, Dechun Li
Format: Article
Language:English
Published: Elsevier 2022-03-01
Series:Journal of Materiomics
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2352847821001076
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author Li Dong
Hongwei Chu
Ying Li
Shengzhi Zhao
Dechun Li
author_facet Li Dong
Hongwei Chu
Ying Li
Shengzhi Zhao
Dechun Li
author_sort Li Dong
collection DOAJ
description As a representative transition metal oxide, cupric oxide (CuO) has attracted a lot of interest in miscellaneous fields. In the present work, the prominent third-order nonlinear optical (NLO) features of CuO nanosheets were demonstrated via the typical Z-scan technique at 1 μm. The open-aperture (OA) Z-scan measurements at different intensities clearly showed that CuO nanosheets possessed the saturable absorption (SA), reverse saturable absorption (RSA) and optical limiting behaviors. The closed-aperture (CA) Z-scan technology was implanted to investigate the nonlinear refractive index and the third-order nonlinear susceptibility. In virtue of the strong nonlinear optical absorption properties of CuO nanosheets, a stable all-solid-state mode-locked laser with the as-prepared CuO nanosheets as saturable absorber at 1.06 μm was realized for the first time. Our work confirmed that CuO nanosheets exhibited outstanding NLO properties, which might stimulate the development in ultrafast photonics and nonlinear optics.
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spelling doaj.art-563b2408602c4128ab022057333cd3a12023-09-02T19:40:09ZengElsevierJournal of Materiomics2352-84782022-03-0182511517Third-order nonlinear optical responses of CuO nanosheets for ultrafast pulse generationLi Dong0Hongwei Chu1Ying Li2Shengzhi Zhao3Dechun Li4School of Information Science and Engineering, Shandong University, Qingdao, 266237, ChinaSchool of Information Science and Engineering, Shandong University, Qingdao, 266237, China; Corresponding author.Key Laboratory of Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Jinan, 250100, ChinaSchool of Information Science and Engineering, Shandong University, Qingdao, 266237, ChinaSchool of Information Science and Engineering, Shandong University, Qingdao, 266237, China; Corresponding author.As a representative transition metal oxide, cupric oxide (CuO) has attracted a lot of interest in miscellaneous fields. In the present work, the prominent third-order nonlinear optical (NLO) features of CuO nanosheets were demonstrated via the typical Z-scan technique at 1 μm. The open-aperture (OA) Z-scan measurements at different intensities clearly showed that CuO nanosheets possessed the saturable absorption (SA), reverse saturable absorption (RSA) and optical limiting behaviors. The closed-aperture (CA) Z-scan technology was implanted to investigate the nonlinear refractive index and the third-order nonlinear susceptibility. In virtue of the strong nonlinear optical absorption properties of CuO nanosheets, a stable all-solid-state mode-locked laser with the as-prepared CuO nanosheets as saturable absorber at 1.06 μm was realized for the first time. Our work confirmed that CuO nanosheets exhibited outstanding NLO properties, which might stimulate the development in ultrafast photonics and nonlinear optics.http://www.sciencedirect.com/science/article/pii/S2352847821001076Transition metal oxideNonlinear saturable absorptionNonlinear susceptibilitySaturable absorberMode-locking
spellingShingle Li Dong
Hongwei Chu
Ying Li
Shengzhi Zhao
Dechun Li
Third-order nonlinear optical responses of CuO nanosheets for ultrafast pulse generation
Journal of Materiomics
Transition metal oxide
Nonlinear saturable absorption
Nonlinear susceptibility
Saturable absorber
Mode-locking
title Third-order nonlinear optical responses of CuO nanosheets for ultrafast pulse generation
title_full Third-order nonlinear optical responses of CuO nanosheets for ultrafast pulse generation
title_fullStr Third-order nonlinear optical responses of CuO nanosheets for ultrafast pulse generation
title_full_unstemmed Third-order nonlinear optical responses of CuO nanosheets for ultrafast pulse generation
title_short Third-order nonlinear optical responses of CuO nanosheets for ultrafast pulse generation
title_sort third order nonlinear optical responses of cuo nanosheets for ultrafast pulse generation
topic Transition metal oxide
Nonlinear saturable absorption
Nonlinear susceptibility
Saturable absorber
Mode-locking
url http://www.sciencedirect.com/science/article/pii/S2352847821001076
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