An Insight into the Medicinal Chemistry Perspective of Macrocyclic Derivatives with Antitumor Activity: A Systematic Review

The profound pharmacological properties of macrocyclic compounds have led to their development as drugs. In conformationally pre-organized ring structures, the multiple functions and stereochemical complexity provided by the macrocycle result in high affinity and selectivity of protein targets while...

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Main Authors: Yan Liang, Ru Fang, Qiu Rao
Format: Article
Language:English
Published: MDPI AG 2022-04-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/27/9/2837
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author Yan Liang
Ru Fang
Qiu Rao
author_facet Yan Liang
Ru Fang
Qiu Rao
author_sort Yan Liang
collection DOAJ
description The profound pharmacological properties of macrocyclic compounds have led to their development as drugs. In conformationally pre-organized ring structures, the multiple functions and stereochemical complexity provided by the macrocycle result in high affinity and selectivity of protein targets while maintaining sufficient bioavailability to reach intracellular locations. Therefore, the construction of macrocycles is an ideal choice to solve the problem of “undruggable” targets. Inspection of 68 macrocyclic drugs on the market showed that 10 of them were used to treat cancer, but this structural class still has been poorly explored within drug discovery. This perspective considers the macrocyclic compounds used for anti-tumor with different targets, their advantages and disadvantages, and the various synthetic methods of them.
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spelling doaj.art-572dc8640a804ee8b3d4aa8f2ca78ba52023-11-23T08:50:31ZengMDPI AGMolecules1420-30492022-04-01279283710.3390/molecules27092837An Insight into the Medicinal Chemistry Perspective of Macrocyclic Derivatives with Antitumor Activity: A Systematic ReviewYan Liang0Ru Fang1Qiu Rao2Department of Pathology, Jinling Hospital, Nanjing University School of Medicine, Nanjing 210000, ChinaDepartment of Pathology, Jinling Hospital, Nanjing University School of Medicine, Nanjing 210000, ChinaDepartment of Pathology, Jinling Hospital, Nanjing University School of Medicine, Nanjing 210000, ChinaThe profound pharmacological properties of macrocyclic compounds have led to their development as drugs. In conformationally pre-organized ring structures, the multiple functions and stereochemical complexity provided by the macrocycle result in high affinity and selectivity of protein targets while maintaining sufficient bioavailability to reach intracellular locations. Therefore, the construction of macrocycles is an ideal choice to solve the problem of “undruggable” targets. Inspection of 68 macrocyclic drugs on the market showed that 10 of them were used to treat cancer, but this structural class still has been poorly explored within drug discovery. This perspective considers the macrocyclic compounds used for anti-tumor with different targets, their advantages and disadvantages, and the various synthetic methods of them.https://www.mdpi.com/1420-3049/27/9/2837macrocyclic compoundantitumorsynthetic methods
spellingShingle Yan Liang
Ru Fang
Qiu Rao
An Insight into the Medicinal Chemistry Perspective of Macrocyclic Derivatives with Antitumor Activity: A Systematic Review
Molecules
macrocyclic compound
antitumor
synthetic methods
title An Insight into the Medicinal Chemistry Perspective of Macrocyclic Derivatives with Antitumor Activity: A Systematic Review
title_full An Insight into the Medicinal Chemistry Perspective of Macrocyclic Derivatives with Antitumor Activity: A Systematic Review
title_fullStr An Insight into the Medicinal Chemistry Perspective of Macrocyclic Derivatives with Antitumor Activity: A Systematic Review
title_full_unstemmed An Insight into the Medicinal Chemistry Perspective of Macrocyclic Derivatives with Antitumor Activity: A Systematic Review
title_short An Insight into the Medicinal Chemistry Perspective of Macrocyclic Derivatives with Antitumor Activity: A Systematic Review
title_sort insight into the medicinal chemistry perspective of macrocyclic derivatives with antitumor activity a systematic review
topic macrocyclic compound
antitumor
synthetic methods
url https://www.mdpi.com/1420-3049/27/9/2837
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