Bright Silicon Carbide Single-Photon Emitting Diodes at Low Temperatures: Toward Quantum Photonics Applications

Color centers in silicon carbide have recently emerged as one of the most promising emitters for bright single-photon emitting diodes (SPEDs). It has been shown that, at room temperature, they can emit more than 10<sup>9</sup> photons per second under electrical excitation. However, the...

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Main Authors: Igor A. Khramtsov, Dmitry Yu. Fedyanin
Format: Article
Language:English
Published: MDPI AG 2021-11-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/11/12/3177
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author Igor A. Khramtsov
Dmitry Yu. Fedyanin
author_facet Igor A. Khramtsov
Dmitry Yu. Fedyanin
author_sort Igor A. Khramtsov
collection DOAJ
description Color centers in silicon carbide have recently emerged as one of the most promising emitters for bright single-photon emitting diodes (SPEDs). It has been shown that, at room temperature, they can emit more than 10<sup>9</sup> photons per second under electrical excitation. However, the spectral emission properties of color centers in SiC at room temperature are far from ideal. The spectral properties could be significantly improved by decreasing the operating temperature. However, the densities of free charge carriers in SiC rapidly decrease as temperature decreases, which reduces the efficiency of electrical excitation of color centers by many orders of magnitude. Here, we study for the first time the temperature characteristics of SPEDs based on color centers in 4H-SiC. Using a rigorous numerical approach, we demonstrate that although the single-photon electroluminescence rate does rapidly decrease as temperature decreases, it is possible to increase the SPED brightness to 10<sup>7</sup> photons/s at 100 K using the recently predicted effect of hole superinjection in homojunction p-i-n diodes. This gives the possibility to achieve high brightness and good spectral properties at the same time, which paves the way toward novel quantum photonics applications of electrically driven color centers in silicon carbide.
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spelling doaj.art-574f1233b0154bfd8e1e485bb6d770952023-11-23T09:48:54ZengMDPI AGNanomaterials2079-49912021-11-011112317710.3390/nano11123177Bright Silicon Carbide Single-Photon Emitting Diodes at Low Temperatures: Toward Quantum Photonics ApplicationsIgor A. Khramtsov0Dmitry Yu. Fedyanin1Laboratory of Nanooptics and Plasmonics, Center for Photonics and 2D Materials, Moscow Institute of Physics and Technology, 141700 Dolgoprudny, RussiaLaboratory of Nanooptics and Plasmonics, Center for Photonics and 2D Materials, Moscow Institute of Physics and Technology, 141700 Dolgoprudny, RussiaColor centers in silicon carbide have recently emerged as one of the most promising emitters for bright single-photon emitting diodes (SPEDs). It has been shown that, at room temperature, they can emit more than 10<sup>9</sup> photons per second under electrical excitation. However, the spectral emission properties of color centers in SiC at room temperature are far from ideal. The spectral properties could be significantly improved by decreasing the operating temperature. However, the densities of free charge carriers in SiC rapidly decrease as temperature decreases, which reduces the efficiency of electrical excitation of color centers by many orders of magnitude. Here, we study for the first time the temperature characteristics of SPEDs based on color centers in 4H-SiC. Using a rigorous numerical approach, we demonstrate that although the single-photon electroluminescence rate does rapidly decrease as temperature decreases, it is possible to increase the SPED brightness to 10<sup>7</sup> photons/s at 100 K using the recently predicted effect of hole superinjection in homojunction p-i-n diodes. This gives the possibility to achieve high brightness and good spectral properties at the same time, which paves the way toward novel quantum photonics applications of electrically driven color centers in silicon carbide.https://www.mdpi.com/2079-4991/11/12/3177color centerssilicon carbidesingle-photon sourcesingle-photon emitting diodesingle-photon electroluminescencesuperinjection in homojunctions
spellingShingle Igor A. Khramtsov
Dmitry Yu. Fedyanin
Bright Silicon Carbide Single-Photon Emitting Diodes at Low Temperatures: Toward Quantum Photonics Applications
Nanomaterials
color centers
silicon carbide
single-photon source
single-photon emitting diode
single-photon electroluminescence
superinjection in homojunctions
title Bright Silicon Carbide Single-Photon Emitting Diodes at Low Temperatures: Toward Quantum Photonics Applications
title_full Bright Silicon Carbide Single-Photon Emitting Diodes at Low Temperatures: Toward Quantum Photonics Applications
title_fullStr Bright Silicon Carbide Single-Photon Emitting Diodes at Low Temperatures: Toward Quantum Photonics Applications
title_full_unstemmed Bright Silicon Carbide Single-Photon Emitting Diodes at Low Temperatures: Toward Quantum Photonics Applications
title_short Bright Silicon Carbide Single-Photon Emitting Diodes at Low Temperatures: Toward Quantum Photonics Applications
title_sort bright silicon carbide single photon emitting diodes at low temperatures toward quantum photonics applications
topic color centers
silicon carbide
single-photon source
single-photon emitting diode
single-photon electroluminescence
superinjection in homojunctions
url https://www.mdpi.com/2079-4991/11/12/3177
work_keys_str_mv AT igorakhramtsov brightsiliconcarbidesinglephotonemittingdiodesatlowtemperaturestowardquantumphotonicsapplications
AT dmitryyufedyanin brightsiliconcarbidesinglephotonemittingdiodesatlowtemperaturestowardquantumphotonicsapplications