Localization Phenomena in Disordered Tantalum Films

Using dc transport and wide-band spectroscopic ellipsometry techniques we study localization phenomena in highly disordered metallic β -Ta films grown by rf sputtering deposition. The dc transport study implies non-metallic behavior (d ρ /dT < 0), with negative temperature coefficien...

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Main Authors: Natalia Kovaleva, Dagmar Chvostova, Alexandr Dejneka
Format: Article
Language:English
Published: MDPI AG 2017-07-01
Series:Metals
Subjects:
Online Access:https://www.mdpi.com/2075-4701/7/7/257
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author Natalia Kovaleva
Dagmar Chvostova
Alexandr Dejneka
author_facet Natalia Kovaleva
Dagmar Chvostova
Alexandr Dejneka
author_sort Natalia Kovaleva
collection DOAJ
description Using dc transport and wide-band spectroscopic ellipsometry techniques we study localization phenomena in highly disordered metallic β -Ta films grown by rf sputtering deposition. The dc transport study implies non-metallic behavior (d ρ /dT < 0), with negative temperature coefficient of resistivity (TCR). We found that as the absolute TCR value increased, specifying an elevated degree of disorder, the free charge carrier Drude response decreases, indicating the enhanced charge carrier localization. Moreover, we found that the pronounced changes occur at the extended spectral range, involving not only the Drude resonance, but also the higher-energy Lorentz bands, in evidence of the attendant electronic correlations. We propose that the charge carrier localization, or delocalization, is accompanied by the pronounced electronic band structure reconstruction due to many-body effects, which may be the key feature for understanding the physics of highly disordered metals.
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spelling doaj.art-57f3d2e038b449b189ed46bb8826e46f2022-12-21T23:57:27ZengMDPI AGMetals2075-47012017-07-017725710.3390/met7070257met7070257Localization Phenomena in Disordered Tantalum FilmsNatalia Kovaleva0Dagmar Chvostova1Alexandr Dejneka2Institute of Physics, Academy of Sciences of the Czech Republic, Na Slovance 2, Prague 18221, Czech RepublicInstitute of Physics, Academy of Sciences of the Czech Republic, Na Slovance 2, Prague 18221, Czech RepublicInstitute of Physics, Academy of Sciences of the Czech Republic, Na Slovance 2, Prague 18221, Czech RepublicUsing dc transport and wide-band spectroscopic ellipsometry techniques we study localization phenomena in highly disordered metallic β -Ta films grown by rf sputtering deposition. The dc transport study implies non-metallic behavior (d ρ /dT < 0), with negative temperature coefficient of resistivity (TCR). We found that as the absolute TCR value increased, specifying an elevated degree of disorder, the free charge carrier Drude response decreases, indicating the enhanced charge carrier localization. Moreover, we found that the pronounced changes occur at the extended spectral range, involving not only the Drude resonance, but also the higher-energy Lorentz bands, in evidence of the attendant electronic correlations. We propose that the charge carrier localization, or delocalization, is accompanied by the pronounced electronic band structure reconstruction due to many-body effects, which may be the key feature for understanding the physics of highly disordered metals.https://www.mdpi.com/2075-4701/7/7/257disordered metalsweak and Anderson localizationdc transportspectroscopic ellipsometry
spellingShingle Natalia Kovaleva
Dagmar Chvostova
Alexandr Dejneka
Localization Phenomena in Disordered Tantalum Films
Metals
disordered metals
weak and Anderson localization
dc transport
spectroscopic ellipsometry
title Localization Phenomena in Disordered Tantalum Films
title_full Localization Phenomena in Disordered Tantalum Films
title_fullStr Localization Phenomena in Disordered Tantalum Films
title_full_unstemmed Localization Phenomena in Disordered Tantalum Films
title_short Localization Phenomena in Disordered Tantalum Films
title_sort localization phenomena in disordered tantalum films
topic disordered metals
weak and Anderson localization
dc transport
spectroscopic ellipsometry
url https://www.mdpi.com/2075-4701/7/7/257
work_keys_str_mv AT nataliakovaleva localizationphenomenaindisorderedtantalumfilms
AT dagmarchvostova localizationphenomenaindisorderedtantalumfilms
AT alexandrdejneka localizationphenomenaindisorderedtantalumfilms