Preparation and characterization of high-performance ceramic proppant from recycling utilization of oil-based drilling cuttings pyrolysis residues

Abstract Oil-based drilling cutting pyrolysis residues (ODCPRs), bauxite, and sintering additives were applied to manufacture ceramic proppants with low density and high strength in this work. The effect of ODCPRs ratio, sintering temperature, holding time, and the content of additives on the perfor...

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Main Authors: Yuanyi Yang, Hui Li, Zhenghuan Lei, Hongwu Liu, Mingyou Zeng, Tingting Yang, Keming Chen, Yi Duan
Format: Article
Language:English
Published: Nature Portfolio 2024-01-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-024-52334-7
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author Yuanyi Yang
Hui Li
Zhenghuan Lei
Hongwu Liu
Mingyou Zeng
Tingting Yang
Keming Chen
Yi Duan
author_facet Yuanyi Yang
Hui Li
Zhenghuan Lei
Hongwu Liu
Mingyou Zeng
Tingting Yang
Keming Chen
Yi Duan
author_sort Yuanyi Yang
collection DOAJ
description Abstract Oil-based drilling cutting pyrolysis residues (ODCPRs), bauxite, and sintering additives were applied to manufacture ceramic proppants with low density and high strength in this work. The effect of ODCPRs ratio, sintering temperature, holding time, and the content of additives on the performance of the proppants was comprehensively investigated, respectively. And the sintering mechanism of proppants was also discussed according to the phase, microstructure, and thermal behavior analyses. The results revealed that at the best sintering condition (1280 °C, holding for 60 min), and a mass ratio (ODCPRs: bauxite: MnO2 at 3:7:0.1), the well-developed granular corundum and acicular mullite formed inside the proppants and interspersed with each other to form a dense structure. The proppants presented low density and high strength as the bulk density of 1.48 g/cm3, the apparent density of 2.94 g/cm3, a breakage ratio of 5.25% under 52 MPa closed pressure, and the acid solubility of 4.80%, which could well meet the requirement of the standards of SY/T 5108-2014. This work provided a new pathway for recycling ODCPRs and the fabrication of high-performance proppants.
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spelling doaj.art-585b26e7f7354519bdf29b3ad5966ee42024-03-05T19:10:56ZengNature PortfolioScientific Reports2045-23222024-01-0114111410.1038/s41598-024-52334-7Preparation and characterization of high-performance ceramic proppant from recycling utilization of oil-based drilling cuttings pyrolysis residuesYuanyi Yang0Hui Li1Zhenghuan Lei2Hongwu Liu3Mingyou Zeng4Tingting Yang5Keming Chen6Yi Duan7School of Civil Engineering and Geometrics, Southwest Petroleum UniversityCNPCCCDE, Safety Environment Quality Surveillance & Inspection Research InstituteSchool of Civil Engineering and Geometrics, Southwest Petroleum UniversitySchool of Civil Engineering and Geometrics, Southwest Petroleum UniversitySchool of Civil Engineering and Geometrics, Southwest Petroleum UniversitySchool of Civil Engineering and Geometrics, Southwest Petroleum UniversityCNPCCCDE, Safety Environment Quality Surveillance & Inspection Research InstituteCNPCCCDE, Safety Environment Quality Surveillance & Inspection Research InstituteAbstract Oil-based drilling cutting pyrolysis residues (ODCPRs), bauxite, and sintering additives were applied to manufacture ceramic proppants with low density and high strength in this work. The effect of ODCPRs ratio, sintering temperature, holding time, and the content of additives on the performance of the proppants was comprehensively investigated, respectively. And the sintering mechanism of proppants was also discussed according to the phase, microstructure, and thermal behavior analyses. The results revealed that at the best sintering condition (1280 °C, holding for 60 min), and a mass ratio (ODCPRs: bauxite: MnO2 at 3:7:0.1), the well-developed granular corundum and acicular mullite formed inside the proppants and interspersed with each other to form a dense structure. The proppants presented low density and high strength as the bulk density of 1.48 g/cm3, the apparent density of 2.94 g/cm3, a breakage ratio of 5.25% under 52 MPa closed pressure, and the acid solubility of 4.80%, which could well meet the requirement of the standards of SY/T 5108-2014. This work provided a new pathway for recycling ODCPRs and the fabrication of high-performance proppants.https://doi.org/10.1038/s41598-024-52334-7
spellingShingle Yuanyi Yang
Hui Li
Zhenghuan Lei
Hongwu Liu
Mingyou Zeng
Tingting Yang
Keming Chen
Yi Duan
Preparation and characterization of high-performance ceramic proppant from recycling utilization of oil-based drilling cuttings pyrolysis residues
Scientific Reports
title Preparation and characterization of high-performance ceramic proppant from recycling utilization of oil-based drilling cuttings pyrolysis residues
title_full Preparation and characterization of high-performance ceramic proppant from recycling utilization of oil-based drilling cuttings pyrolysis residues
title_fullStr Preparation and characterization of high-performance ceramic proppant from recycling utilization of oil-based drilling cuttings pyrolysis residues
title_full_unstemmed Preparation and characterization of high-performance ceramic proppant from recycling utilization of oil-based drilling cuttings pyrolysis residues
title_short Preparation and characterization of high-performance ceramic proppant from recycling utilization of oil-based drilling cuttings pyrolysis residues
title_sort preparation and characterization of high performance ceramic proppant from recycling utilization of oil based drilling cuttings pyrolysis residues
url https://doi.org/10.1038/s41598-024-52334-7
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