African biomass burning affects aerosol cycling over the Amazon

Abstract Smoke from vegetation fires affects air quality, atmospheric cycling, and the climate in the Amazon rain forest. A major unknown has remained the quantity of long-range transported smoke from Africa in relation to local and regional fire emissions. Here we quantify the abundance, seasonalit...

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Main Authors: Bruna A. Holanda, Marco A. Franco, David Walter, Paulo Artaxo, Samara Carbone, Yafang Cheng, Sourangsu Chowdhury, Florian Ditas, Martin Gysel-Beer, Thomas Klimach, Leslie A. Kremper, Ovid O. Krüger, Jost V. Lavric, Jos Lelieveld, Chaoqun Ma, Luiz A. T. Machado, Robin L. Modini, Fernando G. Morais, Andrea Pozzer, Jorge Saturno, Hang Su, Manfred Wendisch, Stefan Wolff, Mira L. Pöhlker, Meinrat O. Andreae, Ulrich Pöschl, Christopher Pöhlker
Format: Article
Language:English
Published: Nature Portfolio 2023-05-01
Series:Communications Earth & Environment
Online Access:https://doi.org/10.1038/s43247-023-00795-5
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author Bruna A. Holanda
Marco A. Franco
David Walter
Paulo Artaxo
Samara Carbone
Yafang Cheng
Sourangsu Chowdhury
Florian Ditas
Martin Gysel-Beer
Thomas Klimach
Leslie A. Kremper
Ovid O. Krüger
Jost V. Lavric
Jos Lelieveld
Chaoqun Ma
Luiz A. T. Machado
Robin L. Modini
Fernando G. Morais
Andrea Pozzer
Jorge Saturno
Hang Su
Manfred Wendisch
Stefan Wolff
Mira L. Pöhlker
Meinrat O. Andreae
Ulrich Pöschl
Christopher Pöhlker
author_facet Bruna A. Holanda
Marco A. Franco
David Walter
Paulo Artaxo
Samara Carbone
Yafang Cheng
Sourangsu Chowdhury
Florian Ditas
Martin Gysel-Beer
Thomas Klimach
Leslie A. Kremper
Ovid O. Krüger
Jost V. Lavric
Jos Lelieveld
Chaoqun Ma
Luiz A. T. Machado
Robin L. Modini
Fernando G. Morais
Andrea Pozzer
Jorge Saturno
Hang Su
Manfred Wendisch
Stefan Wolff
Mira L. Pöhlker
Meinrat O. Andreae
Ulrich Pöschl
Christopher Pöhlker
author_sort Bruna A. Holanda
collection DOAJ
description Abstract Smoke from vegetation fires affects air quality, atmospheric cycling, and the climate in the Amazon rain forest. A major unknown has remained the quantity of long-range transported smoke from Africa in relation to local and regional fire emissions. Here we quantify the abundance, seasonality, and properties of African smoke in central Amazonia. We show that it accounts for ~ 60% of the black carbon concentrations during the wet season and ~ 30% during the dry season. The African smoke influences aerosol-radiation interactions across the entire Amazon, with the strongest impact on the vulnerable eastern basin, a hot spot of climate and land use change. Our findings further suggest that the direct influence of African smoke has been historically relevant for soil fertilization, the carbon and water cycles, and, thus, the development of the Amazon forest ecosystem, even in the pre-industrial era.
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spelling doaj.art-587ad1fc3f5b4ee5a33b93b77cd65f962023-05-07T11:25:12ZengNature PortfolioCommunications Earth & Environment2662-44352023-05-014111510.1038/s43247-023-00795-5African biomass burning affects aerosol cycling over the AmazonBruna A. Holanda0Marco A. Franco1David Walter2Paulo Artaxo3Samara Carbone4Yafang Cheng5Sourangsu Chowdhury6Florian Ditas7Martin Gysel-Beer8Thomas Klimach9Leslie A. Kremper10Ovid O. Krüger11Jost V. Lavric12Jos Lelieveld13Chaoqun Ma14Luiz A. T. Machado15Robin L. Modini16Fernando G. Morais17Andrea Pozzer18Jorge Saturno19Hang Su20Manfred Wendisch21Stefan Wolff22Mira L. Pöhlker23Meinrat O. Andreae24Ulrich Pöschl25Christopher Pöhlker26Multiphase Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryInstitute of Physics, University of São PauloInstitute of Agrarian Sciences, Federal University of UberlândiaMultiphase Chemistry Department, Max Planck Institute for ChemistryAtmospheric Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryLaboratory of Atmospheric Chemistry, Paul Scherrer InstituteMultiphase Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryDepartment of Biogeochemical Processes, Max Planck Institute for BiogeochemistryAtmospheric Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryLaboratory of Atmospheric Chemistry, Paul Scherrer InstituteInstitute of Physics, University of São PauloAtmospheric Chemistry Department, Max Planck Institute for ChemistryBiogeochemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryLeipzig Institute for Meteorology, Leipzig UniversityMultiphase Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryBiogeochemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryMultiphase Chemistry Department, Max Planck Institute for ChemistryAbstract Smoke from vegetation fires affects air quality, atmospheric cycling, and the climate in the Amazon rain forest. A major unknown has remained the quantity of long-range transported smoke from Africa in relation to local and regional fire emissions. Here we quantify the abundance, seasonality, and properties of African smoke in central Amazonia. We show that it accounts for ~ 60% of the black carbon concentrations during the wet season and ~ 30% during the dry season. The African smoke influences aerosol-radiation interactions across the entire Amazon, with the strongest impact on the vulnerable eastern basin, a hot spot of climate and land use change. Our findings further suggest that the direct influence of African smoke has been historically relevant for soil fertilization, the carbon and water cycles, and, thus, the development of the Amazon forest ecosystem, even in the pre-industrial era.https://doi.org/10.1038/s43247-023-00795-5
spellingShingle Bruna A. Holanda
Marco A. Franco
David Walter
Paulo Artaxo
Samara Carbone
Yafang Cheng
Sourangsu Chowdhury
Florian Ditas
Martin Gysel-Beer
Thomas Klimach
Leslie A. Kremper
Ovid O. Krüger
Jost V. Lavric
Jos Lelieveld
Chaoqun Ma
Luiz A. T. Machado
Robin L. Modini
Fernando G. Morais
Andrea Pozzer
Jorge Saturno
Hang Su
Manfred Wendisch
Stefan Wolff
Mira L. Pöhlker
Meinrat O. Andreae
Ulrich Pöschl
Christopher Pöhlker
African biomass burning affects aerosol cycling over the Amazon
Communications Earth & Environment
title African biomass burning affects aerosol cycling over the Amazon
title_full African biomass burning affects aerosol cycling over the Amazon
title_fullStr African biomass burning affects aerosol cycling over the Amazon
title_full_unstemmed African biomass burning affects aerosol cycling over the Amazon
title_short African biomass burning affects aerosol cycling over the Amazon
title_sort african biomass burning affects aerosol cycling over the amazon
url https://doi.org/10.1038/s43247-023-00795-5
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