Laser based surface treatment of bioactive glass: Dependence on pulsed laser ablation

Experimental results and theoretical simulation of material ablation on nanosecond Nd:YAG laser irradiation of bioactive glass targets, is presented. The process of pulsed laser ablation critically affects both, laser based surface modification and pulsed laser deposition (PLD) of bioactive glass (B...

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Main Author: Sucharita Sinha
Format: Article
Language:English
Published: Elsevier 2022-10-01
Series:Applied Surface Science Advances
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S266652392200085X
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author Sucharita Sinha
author_facet Sucharita Sinha
author_sort Sucharita Sinha
collection DOAJ
description Experimental results and theoretical simulation of material ablation on nanosecond Nd:YAG laser irradiation of bioactive glass targets, is presented. The process of pulsed laser ablation critically affects both, laser based surface modification and pulsed laser deposition (PLD) of bioactive glass (BG). A thermal model based theoretical simulation has been carried out describing heat-transport, melting and vaporization of a laser irradiated BG target under near-threshold ablation conditions. Calculated mass ablation rate per laser pulse has been compared with our experimental observations over the average laser fluence of 0.5J/cm2 to 6J/cm2. With increasing laser fluence, possibility of material ablation approaching phase explosion has been discussed by comparing the calculated maximum temperature reached by the laser irradiated target and the estimated thermodynamic critical temperature for BG. Our investigations indicate that with average laser fluence restricted to ∼5 J/cm2 material ablation occurs largely via normal vaporization ensuring deposition of an uniform, homogeneous BG coating through PLD. Target surface temperatures estimated from our calculations also suggest that laser based surface modification of BG can be reproducibly carried out without causing target crystallization and surface damage through crater formation for irradiating laser fluence in the region of ∼ 5J/cm2.
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spelling doaj.art-588964addae245e09e3c7ae6389be8942022-12-22T03:33:18ZengElsevierApplied Surface Science Advances2666-52392022-10-0111100295Laser based surface treatment of bioactive glass: Dependence on pulsed laser ablationSucharita Sinha0Beam Technology Development Group, Bhabha Atomic Research Centre, Trombay, Mumbai 400085; Corresponding author at: Bhabha Atomic Research Centre, India.Experimental results and theoretical simulation of material ablation on nanosecond Nd:YAG laser irradiation of bioactive glass targets, is presented. The process of pulsed laser ablation critically affects both, laser based surface modification and pulsed laser deposition (PLD) of bioactive glass (BG). A thermal model based theoretical simulation has been carried out describing heat-transport, melting and vaporization of a laser irradiated BG target under near-threshold ablation conditions. Calculated mass ablation rate per laser pulse has been compared with our experimental observations over the average laser fluence of 0.5J/cm2 to 6J/cm2. With increasing laser fluence, possibility of material ablation approaching phase explosion has been discussed by comparing the calculated maximum temperature reached by the laser irradiated target and the estimated thermodynamic critical temperature for BG. Our investigations indicate that with average laser fluence restricted to ∼5 J/cm2 material ablation occurs largely via normal vaporization ensuring deposition of an uniform, homogeneous BG coating through PLD. Target surface temperatures estimated from our calculations also suggest that laser based surface modification of BG can be reproducibly carried out without causing target crystallization and surface damage through crater formation for irradiating laser fluence in the region of ∼ 5J/cm2.http://www.sciencedirect.com/science/article/pii/S266652392200085XBioactive glassLaser ablationSurfacesCoatings
spellingShingle Sucharita Sinha
Laser based surface treatment of bioactive glass: Dependence on pulsed laser ablation
Applied Surface Science Advances
Bioactive glass
Laser ablation
Surfaces
Coatings
title Laser based surface treatment of bioactive glass: Dependence on pulsed laser ablation
title_full Laser based surface treatment of bioactive glass: Dependence on pulsed laser ablation
title_fullStr Laser based surface treatment of bioactive glass: Dependence on pulsed laser ablation
title_full_unstemmed Laser based surface treatment of bioactive glass: Dependence on pulsed laser ablation
title_short Laser based surface treatment of bioactive glass: Dependence on pulsed laser ablation
title_sort laser based surface treatment of bioactive glass dependence on pulsed laser ablation
topic Bioactive glass
Laser ablation
Surfaces
Coatings
url http://www.sciencedirect.com/science/article/pii/S266652392200085X
work_keys_str_mv AT sucharitasinha laserbasedsurfacetreatmentofbioactiveglassdependenceonpulsedlaserablation