Direct observation of topological magnon polarons in a multiferroic material

Abstract Magnon polarons are novel elementary excitations possessing hybrid magnonic and phononic signatures, and are responsible for many exotic spintronic and magnonic phenomena. Despite long-term sustained experimental efforts in chasing for magnon polarons, direct spectroscopic evidence of their...

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Main Authors: Song Bao, Zhao-Long Gu, Yanyan Shangguan, Zhentao Huang, Junbo Liao, Xiaoxue Zhao, Bo Zhang, Zhao-Yang Dong, Wei Wang, Ryoichi Kajimoto, Mitsutaka Nakamura, Tom Fennell, Shun-Li Yu, Jian-Xin Li, Jinsheng Wen
Format: Article
Language:English
Published: Nature Portfolio 2023-09-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-41791-9
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author Song Bao
Zhao-Long Gu
Yanyan Shangguan
Zhentao Huang
Junbo Liao
Xiaoxue Zhao
Bo Zhang
Zhao-Yang Dong
Wei Wang
Ryoichi Kajimoto
Mitsutaka Nakamura
Tom Fennell
Shun-Li Yu
Jian-Xin Li
Jinsheng Wen
author_facet Song Bao
Zhao-Long Gu
Yanyan Shangguan
Zhentao Huang
Junbo Liao
Xiaoxue Zhao
Bo Zhang
Zhao-Yang Dong
Wei Wang
Ryoichi Kajimoto
Mitsutaka Nakamura
Tom Fennell
Shun-Li Yu
Jian-Xin Li
Jinsheng Wen
author_sort Song Bao
collection DOAJ
description Abstract Magnon polarons are novel elementary excitations possessing hybrid magnonic and phononic signatures, and are responsible for many exotic spintronic and magnonic phenomena. Despite long-term sustained experimental efforts in chasing for magnon polarons, direct spectroscopic evidence of their existence is hardly observed. Here, we report the direct observation of magnon polarons using neutron spectroscopy on a multiferroic Fe2Mo3O8 possessing strong magnon-phonon coupling. Specifically, below the magnetic ordering temperature, a gap opens at the nominal intersection of the original magnon and phonon bands, leading to two separated magnon-polaron bands. Each of the bands undergoes mixing, interconverting and reversing between its magnonic and phononic components. We attribute the formation of magnon polarons to the strong magnon-phonon coupling induced by Dzyaloshinskii-Moriya interaction. Intriguingly, we find that the band-inverted magnon polarons are topologically nontrivial. These results uncover exotic elementary excitations arising from the magnon-phonon coupling, and offer a new route to topological states by considering hybridizations between different types of fundamental excitations.
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spelling doaj.art-5af7db7a8f58480b96c6e6bbfb85a49e2023-11-20T10:06:42ZengNature PortfolioNature Communications2041-17232023-09-011411910.1038/s41467-023-41791-9Direct observation of topological magnon polarons in a multiferroic materialSong Bao0Zhao-Long Gu1Yanyan Shangguan2Zhentao Huang3Junbo Liao4Xiaoxue Zhao5Bo Zhang6Zhao-Yang Dong7Wei Wang8Ryoichi Kajimoto9Mitsutaka Nakamura10Tom Fennell11Shun-Li Yu12Jian-Xin Li13Jinsheng Wen14National Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityNational Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityNational Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityNational Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityNational Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityNational Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityNational Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityDepartment of Applied Physics, Nanjing University of Science and TechnologySchool of Science, Nanjing University of Posts and TelecommunicationsJ-PARC Center, Japan Atomic Energy Agency (JAEA)J-PARC Center, Japan Atomic Energy Agency (JAEA)Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institute (PSI)National Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityNational Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityNational Laboratory of Solid State Microstructures and Department of Physics, Nanjing UniversityAbstract Magnon polarons are novel elementary excitations possessing hybrid magnonic and phononic signatures, and are responsible for many exotic spintronic and magnonic phenomena. Despite long-term sustained experimental efforts in chasing for magnon polarons, direct spectroscopic evidence of their existence is hardly observed. Here, we report the direct observation of magnon polarons using neutron spectroscopy on a multiferroic Fe2Mo3O8 possessing strong magnon-phonon coupling. Specifically, below the magnetic ordering temperature, a gap opens at the nominal intersection of the original magnon and phonon bands, leading to two separated magnon-polaron bands. Each of the bands undergoes mixing, interconverting and reversing between its magnonic and phononic components. We attribute the formation of magnon polarons to the strong magnon-phonon coupling induced by Dzyaloshinskii-Moriya interaction. Intriguingly, we find that the band-inverted magnon polarons are topologically nontrivial. These results uncover exotic elementary excitations arising from the magnon-phonon coupling, and offer a new route to topological states by considering hybridizations between different types of fundamental excitations.https://doi.org/10.1038/s41467-023-41791-9
spellingShingle Song Bao
Zhao-Long Gu
Yanyan Shangguan
Zhentao Huang
Junbo Liao
Xiaoxue Zhao
Bo Zhang
Zhao-Yang Dong
Wei Wang
Ryoichi Kajimoto
Mitsutaka Nakamura
Tom Fennell
Shun-Li Yu
Jian-Xin Li
Jinsheng Wen
Direct observation of topological magnon polarons in a multiferroic material
Nature Communications
title Direct observation of topological magnon polarons in a multiferroic material
title_full Direct observation of topological magnon polarons in a multiferroic material
title_fullStr Direct observation of topological magnon polarons in a multiferroic material
title_full_unstemmed Direct observation of topological magnon polarons in a multiferroic material
title_short Direct observation of topological magnon polarons in a multiferroic material
title_sort direct observation of topological magnon polarons in a multiferroic material
url https://doi.org/10.1038/s41467-023-41791-9
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