Large positive magnetoresistance and high mobility in topological insulator candidate LaP

Abstract We reported herein the single crystal growth and the comprehensive study of basic physical properties including electronic transport, magnetic, specific heat of topological insulator candidate LaP. Single crystal LaP of rock salt type structure was synthesized by Sn flux method. Under low t...

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Main Authors: Desheng Wu, Jianlin Luo
Format: Article
Language:English
Published: Springer 2023-11-01
Series:Quantum Frontiers
Subjects:
Online Access:https://doi.org/10.1007/s44214-023-00038-w
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author Desheng Wu
Jianlin Luo
author_facet Desheng Wu
Jianlin Luo
author_sort Desheng Wu
collection DOAJ
description Abstract We reported herein the single crystal growth and the comprehensive study of basic physical properties including electronic transport, magnetic, specific heat of topological insulator candidate LaP. Single crystal LaP of rock salt type structure was synthesized by Sn flux method. Under low temperature and high magnetic field of T = 2 $T= 2$  K and B = 9 $B= 9$ T, large positive magnetoresistance (LMR) of 500% was discovered. The Hall effect measurements show that the conduction carriers are dominated by holes among the temperature range from 300 K to 2 K, the carrier concentration n h = 4.94 × 10 19 $n_{h} =4.94\times 10^{19}$ cm−3 and n e = 5.02 × 10 16 $n_{e} =5.02\times 10^{16}$ cm−3 and the mobility of LaP reached as high as μ h = 1.57 × 10 4 $\mu _{h}=1.57\times 10^{4}$ cm2 V−1 S−1 and μ e = 1.55 × 10 3 $\mu _{e} = 1.55\times 10^{3}$ cm2 V−1 S−1 obtained at 2 K, which can be explained by multiband model physics like other topological quantum material systems with large MR. LaP shows diamagnetism over a wide temperature range from 2 K to 300 K without any magnetic phase transition by susceptibility measurements. No evidence of phase transitions from 2 K to 300 K was observed in the specific heat measurement. The electronic specific heat coefficient is obtained 0.538 m J mol−1 K−2 for LaP single crystal, which responds to a small electron density state near the Fermi level. Our results would be helpful in renewing interest in studying emergent phenomena arisen from topological semimetals. LaP offers a platform for understanding the interactions between large magnetoresistance, high mobility and topological band structure.
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spelling doaj.art-5b627bfeed6745a1ae5e526e42964a712023-11-12T12:25:43ZengSpringerQuantum Frontiers2731-61062023-11-01211610.1007/s44214-023-00038-wLarge positive magnetoresistance and high mobility in topological insulator candidate LaPDesheng Wu0Jianlin Luo1Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesAbstract We reported herein the single crystal growth and the comprehensive study of basic physical properties including electronic transport, magnetic, specific heat of topological insulator candidate LaP. Single crystal LaP of rock salt type structure was synthesized by Sn flux method. Under low temperature and high magnetic field of T = 2 $T= 2$  K and B = 9 $B= 9$ T, large positive magnetoresistance (LMR) of 500% was discovered. The Hall effect measurements show that the conduction carriers are dominated by holes among the temperature range from 300 K to 2 K, the carrier concentration n h = 4.94 × 10 19 $n_{h} =4.94\times 10^{19}$ cm−3 and n e = 5.02 × 10 16 $n_{e} =5.02\times 10^{16}$ cm−3 and the mobility of LaP reached as high as μ h = 1.57 × 10 4 $\mu _{h}=1.57\times 10^{4}$ cm2 V−1 S−1 and μ e = 1.55 × 10 3 $\mu _{e} = 1.55\times 10^{3}$ cm2 V−1 S−1 obtained at 2 K, which can be explained by multiband model physics like other topological quantum material systems with large MR. LaP shows diamagnetism over a wide temperature range from 2 K to 300 K without any magnetic phase transition by susceptibility measurements. No evidence of phase transitions from 2 K to 300 K was observed in the specific heat measurement. The electronic specific heat coefficient is obtained 0.538 m J mol−1 K−2 for LaP single crystal, which responds to a small electron density state near the Fermi level. Our results would be helpful in renewing interest in studying emergent phenomena arisen from topological semimetals. LaP offers a platform for understanding the interactions between large magnetoresistance, high mobility and topological band structure.https://doi.org/10.1007/s44214-023-00038-wSingle crystal synthesisLarge magnetoresistanceHall effectBand structure
spellingShingle Desheng Wu
Jianlin Luo
Large positive magnetoresistance and high mobility in topological insulator candidate LaP
Quantum Frontiers
Single crystal synthesis
Large magnetoresistance
Hall effect
Band structure
title Large positive magnetoresistance and high mobility in topological insulator candidate LaP
title_full Large positive magnetoresistance and high mobility in topological insulator candidate LaP
title_fullStr Large positive magnetoresistance and high mobility in topological insulator candidate LaP
title_full_unstemmed Large positive magnetoresistance and high mobility in topological insulator candidate LaP
title_short Large positive magnetoresistance and high mobility in topological insulator candidate LaP
title_sort large positive magnetoresistance and high mobility in topological insulator candidate lap
topic Single crystal synthesis
Large magnetoresistance
Hall effect
Band structure
url https://doi.org/10.1007/s44214-023-00038-w
work_keys_str_mv AT deshengwu largepositivemagnetoresistanceandhighmobilityintopologicalinsulatorcandidatelap
AT jianlinluo largepositivemagnetoresistanceandhighmobilityintopologicalinsulatorcandidatelap