Aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol ERF

<p>Changes in aerosols cause a change in net top-of-the-atmosphere (ToA) short-wave and long-wave radiative fluxes; rapid adjustments in clouds, water vapour and temperature; and an effective radiative forcing (ERF) of the planetary energy budget. The diverse sources of model uncertainty an...

Full description

Bibliographic Details
Main Authors: L. A. Regayre, J. S. Johnson, M. Yoshioka, K. J. Pringle, D. M. H. Sexton, B. B. B. Booth, L. A. Lee, N. Bellouin, K. S. Carslaw
Format: Article
Language:English
Published: Copernicus Publications 2018-07-01
Series:Atmospheric Chemistry and Physics
Online Access:https://www.atmos-chem-phys.net/18/9975/2018/acp-18-9975-2018.pdf
_version_ 1818148018851938304
author L. A. Regayre
J. S. Johnson
M. Yoshioka
K. J. Pringle
D. M. H. Sexton
B. B. B. Booth
L. A. Lee
N. Bellouin
K. S. Carslaw
author_facet L. A. Regayre
J. S. Johnson
M. Yoshioka
K. J. Pringle
D. M. H. Sexton
B. B. B. Booth
L. A. Lee
N. Bellouin
K. S. Carslaw
author_sort L. A. Regayre
collection DOAJ
description <p>Changes in aerosols cause a change in net top-of-the-atmosphere (ToA) short-wave and long-wave radiative fluxes; rapid adjustments in clouds, water vapour and temperature; and an effective radiative forcing (ERF) of the planetary energy budget. The diverse sources of model uncertainty and the computational cost of running climate models make it difficult to isolate the main causes of aerosol ERF uncertainty and to understand how observations can be used to constrain it. We explore the aerosol ERF uncertainty by using fast model emulators to generate a very large set of aerosol–climate model variants that span the model uncertainty due to 27 parameters related to atmospheric and aerosol processes. Sensitivity analyses shows that the uncertainty in the ToA flux is dominated (around 80&thinsp;%) by uncertainties in the physical atmosphere model, particularly parameters that affect cloud reflectivity. However, uncertainty in the change in ToA flux caused by aerosol emissions over the industrial period (the aerosol ERF) is controlled by a combination of uncertainties in aerosol (around 60&thinsp;%) and physical atmosphere (around 40&thinsp;%) parameters. Four atmospheric and aerosol parameters account for around 80&thinsp;% of the uncertainty in short-wave ToA flux (mostly parameters that directly scale cloud reflectivity, cloud water content or cloud droplet concentrations), and these parameters also account for around 60&thinsp;% of the aerosol ERF uncertainty. The common causes of uncertainty mean that constraining the modelled planetary brightness to tightly match satellite observations changes the lower 95&thinsp;% credible aerosol ERF value from −2.65 to −2.37&thinsp;W&thinsp;m<sup>−2</sup>. This suggests the strongest forcings (below around −2.4&thinsp;W&thinsp;m<sup>−2</sup>) are inconsistent with observations. These results show that, regardless of the fact that the ToA flux is 2 orders of magnitude larger than the aerosol ERF, the observed flux can constrain the uncertainty in ERF because their values are connected by constrainable process parameters. The key to reducing the aerosol ERF uncertainty further will be to identify observations that can additionally constrain individual parameter ranges and/or combined parameter effects, which can be achieved through sensitivity analysis of perturbed parameter ensembles.</p>
first_indexed 2024-12-11T12:44:28Z
format Article
id doaj.art-5f25839312a142c3a94b133eeffa4a46
institution Directory Open Access Journal
issn 1680-7316
1680-7324
language English
last_indexed 2024-12-11T12:44:28Z
publishDate 2018-07-01
publisher Copernicus Publications
record_format Article
series Atmospheric Chemistry and Physics
spelling doaj.art-5f25839312a142c3a94b133eeffa4a462022-12-22T01:06:52ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242018-07-011899751000610.5194/acp-18-9975-2018Aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol ERFL. A. Regayre0J. S. Johnson1M. Yoshioka2K. J. Pringle3D. M. H. Sexton4B. B. B. Booth5L. A. Lee6N. Bellouin7K. S. Carslaw8Institute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UKInstitute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UKInstitute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UKInstitute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UKUK Hadley Centre Met Office, Exeter, Fitzroy Road, Exeter, Devon, EX1 3PB, UKUK Hadley Centre Met Office, Exeter, Fitzroy Road, Exeter, Devon, EX1 3PB, UKInstitute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UKDepartment of Meteorology, School of Mathematical & Physical Sciences, Faculty of Science,University of Reading, Reading, RG6 6BB, UKInstitute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK<p>Changes in aerosols cause a change in net top-of-the-atmosphere (ToA) short-wave and long-wave radiative fluxes; rapid adjustments in clouds, water vapour and temperature; and an effective radiative forcing (ERF) of the planetary energy budget. The diverse sources of model uncertainty and the computational cost of running climate models make it difficult to isolate the main causes of aerosol ERF uncertainty and to understand how observations can be used to constrain it. We explore the aerosol ERF uncertainty by using fast model emulators to generate a very large set of aerosol–climate model variants that span the model uncertainty due to 27 parameters related to atmospheric and aerosol processes. Sensitivity analyses shows that the uncertainty in the ToA flux is dominated (around 80&thinsp;%) by uncertainties in the physical atmosphere model, particularly parameters that affect cloud reflectivity. However, uncertainty in the change in ToA flux caused by aerosol emissions over the industrial period (the aerosol ERF) is controlled by a combination of uncertainties in aerosol (around 60&thinsp;%) and physical atmosphere (around 40&thinsp;%) parameters. Four atmospheric and aerosol parameters account for around 80&thinsp;% of the uncertainty in short-wave ToA flux (mostly parameters that directly scale cloud reflectivity, cloud water content or cloud droplet concentrations), and these parameters also account for around 60&thinsp;% of the aerosol ERF uncertainty. The common causes of uncertainty mean that constraining the modelled planetary brightness to tightly match satellite observations changes the lower 95&thinsp;% credible aerosol ERF value from −2.65 to −2.37&thinsp;W&thinsp;m<sup>−2</sup>. This suggests the strongest forcings (below around −2.4&thinsp;W&thinsp;m<sup>−2</sup>) are inconsistent with observations. These results show that, regardless of the fact that the ToA flux is 2 orders of magnitude larger than the aerosol ERF, the observed flux can constrain the uncertainty in ERF because their values are connected by constrainable process parameters. The key to reducing the aerosol ERF uncertainty further will be to identify observations that can additionally constrain individual parameter ranges and/or combined parameter effects, which can be achieved through sensitivity analysis of perturbed parameter ensembles.</p>https://www.atmos-chem-phys.net/18/9975/2018/acp-18-9975-2018.pdf
spellingShingle L. A. Regayre
J. S. Johnson
M. Yoshioka
K. J. Pringle
D. M. H. Sexton
B. B. B. Booth
L. A. Lee
N. Bellouin
K. S. Carslaw
Aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol ERF
Atmospheric Chemistry and Physics
title Aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol ERF
title_full Aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol ERF
title_fullStr Aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol ERF
title_full_unstemmed Aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol ERF
title_short Aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol ERF
title_sort aerosol and physical atmosphere model parameters are both important sources of uncertainty in aerosol erf
url https://www.atmos-chem-phys.net/18/9975/2018/acp-18-9975-2018.pdf
work_keys_str_mv AT laregayre aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf
AT jsjohnson aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf
AT myoshioka aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf
AT kjpringle aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf
AT dmhsexton aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf
AT bbbbooth aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf
AT lalee aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf
AT nbellouin aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf
AT kscarslaw aerosolandphysicalatmospheremodelparametersarebothimportantsourcesofuncertaintyinaerosolerf