The pseudochiral Fermi surface of α-RuI3

Abstract In continuation of research into RuCl3 and RuBr3 as potential quantum spin liquids, a phase with unique magnetic order characterised by long-range quantum entanglement and fractionalised excitations, the compound RuI3 has been recently synthesised. Here, we show RuI3 is a moderately correla...

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Bibliographic Details
Main Authors: Alex Louat, Matthew D. Watson, Timur K. Kim, Danrui Ni, Robert J. Cava, Cephise Cacho
Format: Article
Language:English
Published: Nature Portfolio 2024-01-01
Series:Communications Physics
Online Access:https://doi.org/10.1038/s42005-024-01533-9
Description
Summary:Abstract In continuation of research into RuCl3 and RuBr3 as potential quantum spin liquids, a phase with unique magnetic order characterised by long-range quantum entanglement and fractionalised excitations, the compound RuI3 has been recently synthesised. Here, we show RuI3 is a moderately correlated metal with two bands crossing the Fermi level, implying the absence of any quantum spin liquids phase. We find that the Fermi surface as measured or calculated for a 2D (k x, k y) slice at any k z lacks mirror symmetry, i.e. is pseudochiral. We link this phenomenon to the ABC stacking in the R $$\bar{3}$$ 3 ¯ space group of α-RuI3, which is achiral but lacks any mirror or glide symmetries. We further provide a formal framework for understanding when such a pseudochiral electronic structure may be observed.
ISSN:2399-3650