The impact of surface morphology on the magnetovolume transition in magnetocaloric LaFe11.8Si1.2

First order magnetocaloric materials reach high entropy changes but at the same time exhibit hysteresis losses which depend on the sample’s microstructure. We use non-destructive 3D X-ray microtomography to understand the role of surface morphology for the magnetovolume transition of LaFe11.8Si1.2....

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Main Authors: A. Waske, E. Lovell, A. Funk, K. Sellschopp, A. Rack, L. Giebeler, P. F. Gostin, S. Fähler, L. F. Cohen
Format: Article
Language:English
Published: AIP Publishing LLC 2016-10-01
Series:APL Materials
Online Access:http://dx.doi.org/10.1063/1.4963840
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author A. Waske
E. Lovell
A. Funk
K. Sellschopp
A. Rack
L. Giebeler
P. F. Gostin
S. Fähler
L. F. Cohen
author_facet A. Waske
E. Lovell
A. Funk
K. Sellschopp
A. Rack
L. Giebeler
P. F. Gostin
S. Fähler
L. F. Cohen
author_sort A. Waske
collection DOAJ
description First order magnetocaloric materials reach high entropy changes but at the same time exhibit hysteresis losses which depend on the sample’s microstructure. We use non-destructive 3D X-ray microtomography to understand the role of surface morphology for the magnetovolume transition of LaFe11.8Si1.2. The technique provides unique information on the spatial distribution of the volume change at the transition and its relationship with the surface morphology. Complementary Hall probe imaging confirms that on a morphologically complex surface minimization of strain energy dominates. Our findings sketch the way for a tailored surface morphology with low hysteresis without changing the underlying phase transition.
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spelling doaj.art-608b80e125e64be39f4c4d6d060606212022-12-21T17:30:38ZengAIP Publishing LLCAPL Materials2166-532X2016-10-01410106101106101-610.1063/1.4963840001610APMThe impact of surface morphology on the magnetovolume transition in magnetocaloric LaFe11.8Si1.2A. Waske0E. Lovell1A. Funk2K. Sellschopp3A. Rack4L. Giebeler5P. F. Gostin6S. Fähler7L. F. Cohen8IFW Dresden, P.O. 270116, 01171 Dresden, GermanyBlackett Laboratory, Imperial College London, SW7 2AZ London, United KingdomIFW Dresden, P.O. 270116, 01171 Dresden, GermanyIFW Dresden, P.O. 270116, 01171 Dresden, GermanyESRF - The European Synchrotron, CS 40220, 38043 Grenoble Cedex 9, FranceIFW Dresden, P.O. 270116, 01171 Dresden, GermanyIFW Dresden, P.O. 270116, 01171 Dresden, GermanyIFW Dresden, P.O. 270116, 01171 Dresden, GermanyBlackett Laboratory, Imperial College London, SW7 2AZ London, United KingdomFirst order magnetocaloric materials reach high entropy changes but at the same time exhibit hysteresis losses which depend on the sample’s microstructure. We use non-destructive 3D X-ray microtomography to understand the role of surface morphology for the magnetovolume transition of LaFe11.8Si1.2. The technique provides unique information on the spatial distribution of the volume change at the transition and its relationship with the surface morphology. Complementary Hall probe imaging confirms that on a morphologically complex surface minimization of strain energy dominates. Our findings sketch the way for a tailored surface morphology with low hysteresis without changing the underlying phase transition.http://dx.doi.org/10.1063/1.4963840
spellingShingle A. Waske
E. Lovell
A. Funk
K. Sellschopp
A. Rack
L. Giebeler
P. F. Gostin
S. Fähler
L. F. Cohen
The impact of surface morphology on the magnetovolume transition in magnetocaloric LaFe11.8Si1.2
APL Materials
title The impact of surface morphology on the magnetovolume transition in magnetocaloric LaFe11.8Si1.2
title_full The impact of surface morphology on the magnetovolume transition in magnetocaloric LaFe11.8Si1.2
title_fullStr The impact of surface morphology on the magnetovolume transition in magnetocaloric LaFe11.8Si1.2
title_full_unstemmed The impact of surface morphology on the magnetovolume transition in magnetocaloric LaFe11.8Si1.2
title_short The impact of surface morphology on the magnetovolume transition in magnetocaloric LaFe11.8Si1.2
title_sort impact of surface morphology on the magnetovolume transition in magnetocaloric lafe11 8si1 2
url http://dx.doi.org/10.1063/1.4963840
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