Impact of NH<sub>3</sub> Emissions on Particulate Matter Pollution in South Korea: A Case Study of the Seoul Metropolitan Area

We analyzed the multi-year relationship between particulate matter (PM<sub>10</sub> and PM<sub>2.5</sub>) concentrations and possible precursors including NO<sub>2</sub>, SO<sub>2</sub>, and NH<sub>3</sub> based on local observations over t...

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Main Authors: Changsub Shim, Jihyun Han, Daven K. Henze, Mark W. Shephard, Liye Zhu, Nankyoung Moon, Shailesh K. Kharol, Enrico Dammers, Karen Cady-Pereira
Format: Article
Language:English
Published: MDPI AG 2022-08-01
Series:Atmosphere
Subjects:
Online Access:https://www.mdpi.com/2073-4433/13/8/1227
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author Changsub Shim
Jihyun Han
Daven K. Henze
Mark W. Shephard
Liye Zhu
Nankyoung Moon
Shailesh K. Kharol
Enrico Dammers
Karen Cady-Pereira
author_facet Changsub Shim
Jihyun Han
Daven K. Henze
Mark W. Shephard
Liye Zhu
Nankyoung Moon
Shailesh K. Kharol
Enrico Dammers
Karen Cady-Pereira
author_sort Changsub Shim
collection DOAJ
description We analyzed the multi-year relationship between particulate matter (PM<sub>10</sub> and PM<sub>2.5</sub>) concentrations and possible precursors including NO<sub>2</sub>, SO<sub>2</sub>, and NH<sub>3</sub> based on local observations over the Seoul Metropolitan Area (SMA) from 2015 to 2017. Surface NH<sub>3</sub> concentrations were obtained from Cross-track Infrared Sounder (CrIS) retrievals, while other pollutants were observed at 142 ground sites. We found that NH<sub>3</sub> had the highest correlation with PM<sub>2.5</sub> (R = 0.51) compared to other precursors such as NO<sub>2</sub> and SO<sub>2</sub> (R of 0.16 and 0.14, respectively). The correlations indicate that NH<sub>3</sub> emissions are likely a limiting factor in controlling PM<sub>2.5</sub> over the SMA in a high-NOx environment. This implies that the current Korean policy urgently requires tools for controlling local NH<sub>3</sub> emissions from the livestock industry (for example, from hog manure). These findings provide the first satellite-based trace gas evidence that implementing an NH<sub>3</sub> control strategy could play a key role in improving air quality in the SMA.
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spelling doaj.art-60cf5cc875eb4f81bd7db5693e8bd52b2023-11-30T23:10:15ZengMDPI AGAtmosphere2073-44332022-08-01138122710.3390/atmos13081227Impact of NH<sub>3</sub> Emissions on Particulate Matter Pollution in South Korea: A Case Study of the Seoul Metropolitan AreaChangsub Shim0Jihyun Han1Daven K. Henze2Mark W. Shephard3Liye Zhu4Nankyoung Moon5Shailesh K. Kharol6Enrico Dammers7Karen Cady-Pereira8Korea Environment Institute (KEI), Sejong 30147, KoreaDivision of Climate & Environmental Research, Seoul Institute of Technology (SIT), Seoul 03909, KoreaDepartment of Mechanical Engineering, College of Engineering and Applied Science, University of Colorado, Boulder, CO 80309, USAEnvironment and Climate Change Canada, Toronto, ON M3H 5T4, CanadaSchool of Atmospheric Sciences, Sun Yat-Sen University, Gunagzhou 519082, ChinaKorea Environment Institute (KEI), Sejong 30147, KoreaEnvironment and Climate Change Canada, Toronto, ON M3H 5T4, CanadaClimate Air and Sustainability, TNO, Netherlands Organization for Applied Scientific Research, NL-3508 TA Utrecht, The NetherlandsAtmospheric and Environment Research, Lexington, MA 02421, USAWe analyzed the multi-year relationship between particulate matter (PM<sub>10</sub> and PM<sub>2.5</sub>) concentrations and possible precursors including NO<sub>2</sub>, SO<sub>2</sub>, and NH<sub>3</sub> based on local observations over the Seoul Metropolitan Area (SMA) from 2015 to 2017. Surface NH<sub>3</sub> concentrations were obtained from Cross-track Infrared Sounder (CrIS) retrievals, while other pollutants were observed at 142 ground sites. We found that NH<sub>3</sub> had the highest correlation with PM<sub>2.5</sub> (R = 0.51) compared to other precursors such as NO<sub>2</sub> and SO<sub>2</sub> (R of 0.16 and 0.14, respectively). The correlations indicate that NH<sub>3</sub> emissions are likely a limiting factor in controlling PM<sub>2.5</sub> over the SMA in a high-NOx environment. This implies that the current Korean policy urgently requires tools for controlling local NH<sub>3</sub> emissions from the livestock industry (for example, from hog manure). These findings provide the first satellite-based trace gas evidence that implementing an NH<sub>3</sub> control strategy could play a key role in improving air quality in the SMA.https://www.mdpi.com/2073-4433/13/8/1227ammoniaparticulate pollutionSeoul Metropolitan AreaKoreaCrIS
spellingShingle Changsub Shim
Jihyun Han
Daven K. Henze
Mark W. Shephard
Liye Zhu
Nankyoung Moon
Shailesh K. Kharol
Enrico Dammers
Karen Cady-Pereira
Impact of NH<sub>3</sub> Emissions on Particulate Matter Pollution in South Korea: A Case Study of the Seoul Metropolitan Area
Atmosphere
ammonia
particulate pollution
Seoul Metropolitan Area
Korea
CrIS
title Impact of NH<sub>3</sub> Emissions on Particulate Matter Pollution in South Korea: A Case Study of the Seoul Metropolitan Area
title_full Impact of NH<sub>3</sub> Emissions on Particulate Matter Pollution in South Korea: A Case Study of the Seoul Metropolitan Area
title_fullStr Impact of NH<sub>3</sub> Emissions on Particulate Matter Pollution in South Korea: A Case Study of the Seoul Metropolitan Area
title_full_unstemmed Impact of NH<sub>3</sub> Emissions on Particulate Matter Pollution in South Korea: A Case Study of the Seoul Metropolitan Area
title_short Impact of NH<sub>3</sub> Emissions on Particulate Matter Pollution in South Korea: A Case Study of the Seoul Metropolitan Area
title_sort impact of nh sub 3 sub emissions on particulate matter pollution in south korea a case study of the seoul metropolitan area
topic ammonia
particulate pollution
Seoul Metropolitan Area
Korea
CrIS
url https://www.mdpi.com/2073-4433/13/8/1227
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