Subsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation
The working temperature of boron-based catalysts reduces their thermodynamic advantages in the oxidative dehydrogenation of propane (ODHP). Here the authors demonstrate encapsulated Ni nanoparticles as effective subsurface promoters to enhance the low temperature activity and selectivity of the boro...
Main Authors: | , , , , , , , , , , , |
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Format: | Article |
Language: | English |
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Nature Portfolio
2023-03-01
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Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-023-37261-x |
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author | Xiaofeng Gao Ling Zhu Feng Yang Lei Zhang Wenhao Xu Xian Zhou Yongkang Huang Houhong Song Lili Lin Xiaodong Wen Ding Ma Siyu Yao |
author_facet | Xiaofeng Gao Ling Zhu Feng Yang Lei Zhang Wenhao Xu Xian Zhou Yongkang Huang Houhong Song Lili Lin Xiaodong Wen Ding Ma Siyu Yao |
author_sort | Xiaofeng Gao |
collection | DOAJ |
description | The working temperature of boron-based catalysts reduces their thermodynamic advantages in the oxidative dehydrogenation of propane (ODHP). Here the authors demonstrate encapsulated Ni nanoparticles as effective subsurface promoters to enhance the low temperature activity and selectivity of the boron oxide overlayer in ODHP. |
first_indexed | 2024-04-09T22:46:56Z |
format | Article |
id | doaj.art-60d579693bba484a869caf3e3a3e5069 |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-04-09T22:46:56Z |
publishDate | 2023-03-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-60d579693bba484a869caf3e3a3e50692023-03-22T11:47:08ZengNature PortfolioNature Communications2041-17232023-03-011411910.1038/s41467-023-37261-xSubsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenationXiaofeng Gao0Ling Zhu1Feng Yang2Lei Zhang3Wenhao Xu4Xian Zhou5Yongkang Huang6Houhong Song7Lili Lin8Xiaodong Wen9Ding Ma10Siyu Yao11Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang UniversityState Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of SciencesDepartment of Chemistry, Guangdong Provincial Key Laboratory of Catalysis, Southern University of Science and TechnologyDepartment of Chemistry, Guangdong Provincial Key Laboratory of Catalysis, Southern University of Science and TechnologyKey Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang UniversityKey Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang UniversityKey Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang UniversityKey Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang UniversityInstitute of Industrial Catalysis, State Key Laboratory of Green Chemistry Synthesis Technology, College of Chemical Engineering, Zhejiang University of TechnologyState Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, Peking UniversityKey Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang UniversityThe working temperature of boron-based catalysts reduces their thermodynamic advantages in the oxidative dehydrogenation of propane (ODHP). Here the authors demonstrate encapsulated Ni nanoparticles as effective subsurface promoters to enhance the low temperature activity and selectivity of the boron oxide overlayer in ODHP.https://doi.org/10.1038/s41467-023-37261-x |
spellingShingle | Xiaofeng Gao Ling Zhu Feng Yang Lei Zhang Wenhao Xu Xian Zhou Yongkang Huang Houhong Song Lili Lin Xiaodong Wen Ding Ma Siyu Yao Subsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation Nature Communications |
title | Subsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation |
title_full | Subsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation |
title_fullStr | Subsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation |
title_full_unstemmed | Subsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation |
title_short | Subsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation |
title_sort | subsurface nickel boosts the low temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation |
url | https://doi.org/10.1038/s41467-023-37261-x |
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