Terahertz Absorption Spectroscopy in Bicrystal Josephson Junctions Formed from Mutually Tilted <i>c</i>-Axes YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> Films

Spectral analysis of terahertz (THz) and sub-THz emission from quantum cascade lasers has been recently demonstrated using conventional YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> bicrystal Josephson junctions made from <i>c</i>-axes thin films. Josep...

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Main Author: Yuriy Divin
Format: Article
Language:English
Published: MDPI AG 2023-05-01
Series:Applied Sciences
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Online Access:https://www.mdpi.com/2076-3417/13/9/5766
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author Yuriy Divin
author_facet Yuriy Divin
author_sort Yuriy Divin
collection DOAJ
description Spectral analysis of terahertz (THz) and sub-THz emission from quantum cascade lasers has been recently demonstrated using conventional YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> bicrystal Josephson junctions made from <i>c</i>-axes thin films. Josephson frequencies of alternative bicrystal junctions made from YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> films with mutually tilted c-axes extend further into the THz range. However, these THz oscillations can weaken due to new absorption channels in the junction environment. Here, using Josephson admittance spectroscopy, THz losses in YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> bicrystal junctions with mutually tilted <i>c</i>-axes are studied. Absorption maximizes at a reproducible set of THz frequencies close to those of collective modes in bulk YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> recovered by Fourier spectroscopy. Annealing junctions in atomic oxygen reduces the losses at frequencies of 2.7 and 3.6 THz, while the losses increase at frequencies of 2.3 and 4.6 THz. Thus, as a THz spectrum analyzer, YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> bicrystal junctions require post-fabrication correction of the oxygen content. In addition, the fine structure of the absorption spectrum appears at frequencies near 4.6 THz. Significant absorption near 2.3 THz may be due to effects associated with the second Josephson harmonic or second-order nonlinearity of the susceptibility in YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub>. This work paves the way towards probing collective modes in high-<i>T<sub>c</sub></i> materials in situ using the Josephson oscillations.
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spelling doaj.art-611a60056cd6477198f1ec4d5ffc74572023-11-17T22:38:31ZengMDPI AGApplied Sciences2076-34172023-05-01139576610.3390/app13095766Terahertz Absorption Spectroscopy in Bicrystal Josephson Junctions Formed from Mutually Tilted <i>c</i>-Axes YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> FilmsYuriy Divin0Kotelnikov Institute of Radioengineering and Electronics, Russian Academy of Sciences, 125009 Moscow, RussiaSpectral analysis of terahertz (THz) and sub-THz emission from quantum cascade lasers has been recently demonstrated using conventional YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> bicrystal Josephson junctions made from <i>c</i>-axes thin films. Josephson frequencies of alternative bicrystal junctions made from YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> films with mutually tilted c-axes extend further into the THz range. However, these THz oscillations can weaken due to new absorption channels in the junction environment. Here, using Josephson admittance spectroscopy, THz losses in YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> bicrystal junctions with mutually tilted <i>c</i>-axes are studied. Absorption maximizes at a reproducible set of THz frequencies close to those of collective modes in bulk YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> recovered by Fourier spectroscopy. Annealing junctions in atomic oxygen reduces the losses at frequencies of 2.7 and 3.6 THz, while the losses increase at frequencies of 2.3 and 4.6 THz. Thus, as a THz spectrum analyzer, YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> bicrystal junctions require post-fabrication correction of the oxygen content. In addition, the fine structure of the absorption spectrum appears at frequencies near 4.6 THz. Significant absorption near 2.3 THz may be due to effects associated with the second Josephson harmonic or second-order nonlinearity of the susceptibility in YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub>. This work paves the way towards probing collective modes in high-<i>T<sub>c</sub></i> materials in situ using the Josephson oscillations.https://www.mdpi.com/2076-3417/13/9/5766Josephson junctionsspectroscopyterahertzhigh-temperature superconductorsabsorption
spellingShingle Yuriy Divin
Terahertz Absorption Spectroscopy in Bicrystal Josephson Junctions Formed from Mutually Tilted <i>c</i>-Axes YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> Films
Applied Sciences
Josephson junctions
spectroscopy
terahertz
high-temperature superconductors
absorption
title Terahertz Absorption Spectroscopy in Bicrystal Josephson Junctions Formed from Mutually Tilted <i>c</i>-Axes YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> Films
title_full Terahertz Absorption Spectroscopy in Bicrystal Josephson Junctions Formed from Mutually Tilted <i>c</i>-Axes YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> Films
title_fullStr Terahertz Absorption Spectroscopy in Bicrystal Josephson Junctions Formed from Mutually Tilted <i>c</i>-Axes YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> Films
title_full_unstemmed Terahertz Absorption Spectroscopy in Bicrystal Josephson Junctions Formed from Mutually Tilted <i>c</i>-Axes YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> Films
title_short Terahertz Absorption Spectroscopy in Bicrystal Josephson Junctions Formed from Mutually Tilted <i>c</i>-Axes YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7−x</sub> Films
title_sort terahertz absorption spectroscopy in bicrystal josephson junctions formed from mutually tilted i c i axes yba sub 2 sub cu sub 3 sub o sub 7 x sub films
topic Josephson junctions
spectroscopy
terahertz
high-temperature superconductors
absorption
url https://www.mdpi.com/2076-3417/13/9/5766
work_keys_str_mv AT yuriydivin terahertzabsorptionspectroscopyinbicrystaljosephsonjunctionsformedfrommutuallytiltediciaxesybasub2subcusub3subosub7xsubfilms