Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family

Ceramics of quaternary garnets (Gd,Y)3Al2Ga3O12 doped with Ce, Tb have been fabricated and evaluated as prospective materials for indirect energy converters of α-and β-voltaic. Samples were characterized at excitation with an X-ray source and an intense 150 keV electron beam and showed good temperat...

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Main Authors: M. Korzhik, R. Abashev, A. Fedorov, G. Dosovitskiy, E. Gordienko, I. Kamenskikh, D. Kazlou, D. Kuznecova, V. Mechinsky, V. Pustovarov, V. Retivov, A. Vasil'ev
Format: Article
Language:English
Published: Elsevier 2022-07-01
Series:Nuclear Engineering and Technology
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S1738573322000791
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author M. Korzhik
R. Abashev
A. Fedorov
G. Dosovitskiy
E. Gordienko
I. Kamenskikh
D. Kazlou
D. Kuznecova
V. Mechinsky
V. Pustovarov
V. Retivov
A. Vasil'ev
author_facet M. Korzhik
R. Abashev
A. Fedorov
G. Dosovitskiy
E. Gordienko
I. Kamenskikh
D. Kazlou
D. Kuznecova
V. Mechinsky
V. Pustovarov
V. Retivov
A. Vasil'ev
author_sort M. Korzhik
collection DOAJ
description Ceramics of quaternary garnets (Gd,Y)3Al2Ga3O12 doped with Ce, Tb have been fabricated and evaluated as prospective materials for indirect energy converters of α-and β-voltaic. Samples were characterized at excitation with an X-ray source and an intense 150 keV electron beam and showed good temperature stability of their emission and tolerance to irradiation. The role of X-rays accompanied the α-particle emitting in the increase of the conversion efficiency is clarified. The garnet-type structure of the matrix in the developed materials allows the production of quality crystalline mass with a light yield exceeding that of the commonly used YAG: Ce scintillator by a factor of two times.
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spelling doaj.art-624e0a1035024cb488935697c7e801892022-12-22T02:27:37ZengElsevierNuclear Engineering and Technology1738-57332022-07-0154725792585Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 familyM. Korzhik0R. Abashev1A. Fedorov2G. Dosovitskiy3E. Gordienko4I. Kamenskikh5D. Kazlou6D. Kuznecova7V. Mechinsky8V. Pustovarov9V. Retivov10A. Vasil'ev11Institute for Nuclear Problems of Belarus State University, Minsk, Belarus; National Research Center “Kurchatov Institute”, Moscow, Russia; Corresponding author. Institute for Nuclear Problems of Belarus State University, Minsk, Belarus.Ural Federal University, Yekaterinburg, RussiaInstitute for Nuclear Problems of Belarus State University, Minsk, Belarus; National Research Center “Kurchatov Institute”, Moscow, RussiaNational Research Center “Kurchatov Institute”, Moscow, Russia; NRC “Kurchatov Institute” – IREA, Moscow, RussiaNational Research Center “Kurchatov Institute”, Moscow, Russia; NRC “Kurchatov Institute” – IREA, Moscow, RussiaPhysical Department of Moscow State University, Moscow, RussiaInstitute for Nuclear Problems of Belarus State University, Minsk, BelarusNational Research Center “Kurchatov Institute”, Moscow, Russia; NRC “Kurchatov Institute” – IREA, Moscow, RussiaInstitute for Nuclear Problems of Belarus State University, Minsk, Belarus; National Research Center “Kurchatov Institute”, Moscow, RussiaUral Federal University, Yekaterinburg, RussiaNational Research Center “Kurchatov Institute”, Moscow, Russia; NRC “Kurchatov Institute” – IREA, Moscow, RussiaSkobelchin Institute for Nuclear Physiocs of Moscow State University, Moscow, RussiaCeramics of quaternary garnets (Gd,Y)3Al2Ga3O12 doped with Ce, Tb have been fabricated and evaluated as prospective materials for indirect energy converters of α-and β-voltaic. Samples were characterized at excitation with an X-ray source and an intense 150 keV electron beam and showed good temperature stability of their emission and tolerance to irradiation. The role of X-rays accompanied the α-particle emitting in the increase of the conversion efficiency is clarified. The garnet-type structure of the matrix in the developed materials allows the production of quality crystalline mass with a light yield exceeding that of the commonly used YAG: Ce scintillator by a factor of two times.http://www.sciencedirect.com/science/article/pii/S1738573322000791Indirect converterBeta-voltaicsAlpha-voltaicsQuaternary garnetTerbiumCerium
spellingShingle M. Korzhik
R. Abashev
A. Fedorov
G. Dosovitskiy
E. Gordienko
I. Kamenskikh
D. Kazlou
D. Kuznecova
V. Mechinsky
V. Pustovarov
V. Retivov
A. Vasil'ev
Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family
Nuclear Engineering and Technology
Indirect converter
Beta-voltaics
Alpha-voltaics
Quaternary garnet
Terbium
Cerium
title Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family
title_full Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family
title_fullStr Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family
title_full_unstemmed Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family
title_short Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family
title_sort towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of gd y 3al2ga3o12 family
topic Indirect converter
Beta-voltaics
Alpha-voltaics
Quaternary garnet
Terbium
Cerium
url http://www.sciencedirect.com/science/article/pii/S1738573322000791
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