Unveiling surface and bulk contributions in temperature dependent THz emission from Bi2Te3

We report evolution of the pulsed terahertz (THz) emission from Bi _2 Te _3 topological insulator in a wide temperature range, where an interplay between the topological surface and bulk contributions can be addressed in a distinguishable manner. A circular photogalvanic effect-induced topological s...

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Main Authors: Anand Nivedan, Sunil Kumar
Format: Article
Language:English
Published: IOP Publishing 2024-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/ad345a
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author Anand Nivedan
Sunil Kumar
author_facet Anand Nivedan
Sunil Kumar
author_sort Anand Nivedan
collection DOAJ
description We report evolution of the pulsed terahertz (THz) emission from Bi _2 Te _3 topological insulator in a wide temperature range, where an interplay between the topological surface and bulk contributions can be addressed in a distinguishable manner. A circular photogalvanic effect-induced topological surface current contribution to THz generation can be clearly identified in the signal, otherwise, overwhelmed by the hot carrier decoherence in the bulk states. With the decreasing temperature, an initial sharp increase in the topological surface THz signal is observed before it attains a constant value below ∼200 K. The scattering channels between topological surface and bulk regions via carrier-phonon scattering are dominantly active only above the bulk-Debye temperature of ∼180 K, and the temperature-independent behavior of it at lower temperatures is indicative of robust nature of topological surface states. THz emission due to ultrafast photon-drag current in the bulk states is almost independent of temperature in the entire range, while the combined photo-Dember and band-bending effects induced photocurrent is doubled at 10 K.
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spelling doaj.art-633d030366bd476ba6c437aa0718d9a52024-03-26T10:20:05ZengIOP PublishingNew Journal of Physics1367-26302024-01-0126303304410.1088/1367-2630/ad345aUnveiling surface and bulk contributions in temperature dependent THz emission from Bi2Te3Anand Nivedan0Sunil Kumar1https://orcid.org/0000-0002-1065-9883Femtosecond Spectroscopy and Nonlinear Photonics Laboratory, Department of Physics, Indian Institute of Technology Delhi , Hauz Khas, New Delhi 110016, IndiaFemtosecond Spectroscopy and Nonlinear Photonics Laboratory, Department of Physics, Indian Institute of Technology Delhi , Hauz Khas, New Delhi 110016, IndiaWe report evolution of the pulsed terahertz (THz) emission from Bi _2 Te _3 topological insulator in a wide temperature range, where an interplay between the topological surface and bulk contributions can be addressed in a distinguishable manner. A circular photogalvanic effect-induced topological surface current contribution to THz generation can be clearly identified in the signal, otherwise, overwhelmed by the hot carrier decoherence in the bulk states. With the decreasing temperature, an initial sharp increase in the topological surface THz signal is observed before it attains a constant value below ∼200 K. The scattering channels between topological surface and bulk regions via carrier-phonon scattering are dominantly active only above the bulk-Debye temperature of ∼180 K, and the temperature-independent behavior of it at lower temperatures is indicative of robust nature of topological surface states. THz emission due to ultrafast photon-drag current in the bulk states is almost independent of temperature in the entire range, while the combined photo-Dember and band-bending effects induced photocurrent is doubled at 10 K.https://doi.org/10.1088/1367-2630/ad345aTHz emissiontime-domain spectroscopybismuth telluridelow-temperature physics
spellingShingle Anand Nivedan
Sunil Kumar
Unveiling surface and bulk contributions in temperature dependent THz emission from Bi2Te3
New Journal of Physics
THz emission
time-domain spectroscopy
bismuth telluride
low-temperature physics
title Unveiling surface and bulk contributions in temperature dependent THz emission from Bi2Te3
title_full Unveiling surface and bulk contributions in temperature dependent THz emission from Bi2Te3
title_fullStr Unveiling surface and bulk contributions in temperature dependent THz emission from Bi2Te3
title_full_unstemmed Unveiling surface and bulk contributions in temperature dependent THz emission from Bi2Te3
title_short Unveiling surface and bulk contributions in temperature dependent THz emission from Bi2Te3
title_sort unveiling surface and bulk contributions in temperature dependent thz emission from bi2te3
topic THz emission
time-domain spectroscopy
bismuth telluride
low-temperature physics
url https://doi.org/10.1088/1367-2630/ad345a
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AT sunilkumar unveilingsurfaceandbulkcontributionsintemperaturedependentthzemissionfrombi2te3