Brightening and Directionality Control of Dark Excitons through Quasi-Bound States in the Continuum

Thanks to their long lifetime, spin-forbidden dark excitons in transition metal dichalcogenides are promising candidates for storage applications in opto-electronics and valleytronics. To date, their study has been hindered by inefficient generation mechanisms and the necessity for elaborate detecti...

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Bibliographic Details
Main Authors: Sebastian Klimmer, Giancarlo Soavi, Isabelle Staude, Ángela Barreda
Format: Article
Language:English
Published: MDPI AG 2023-11-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/13/23/3028
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Summary:Thanks to their long lifetime, spin-forbidden dark excitons in transition metal dichalcogenides are promising candidates for storage applications in opto-electronics and valleytronics. To date, their study has been hindered by inefficient generation mechanisms and the necessity for elaborate detection schemes. In this work, we propose a new hybrid platform that simultaneously addresses both challenges. We study an all-dielectric metasurface with two symmetrically protected quasi-bound states in the continuum to enhance both the excitation and emission of dark excitons in a tungsten diselenide monolayer under normal light incidence. Our simulations show a giant photoluminescence signal enhancement (∼520) along with directional emission, thus offering distinct advantages for opto-electronic and valleytronic devices.
ISSN:2079-4991