Parametric studies of contrail ice particle formation in jet regime using microphysical parcel modeling

Condensation trails (contrails) formed from water vapor emissions behind aircraft engines are the most uncertain components of the aviation impacts on climate change. To gain improved knowledge of contrail and contrail-induced cirrus cloud formation, understanding of contrail ice particle formation...

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Main Authors: H.-W. Wong, R. C. Miake-Lye
Format: Article
Language:English
Published: Copernicus Publications 2010-04-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/10/3261/2010/acp-10-3261-2010.pdf
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author H.-W. Wong
R. C. Miake-Lye
author_facet H.-W. Wong
R. C. Miake-Lye
author_sort H.-W. Wong
collection DOAJ
description Condensation trails (contrails) formed from water vapor emissions behind aircraft engines are the most uncertain components of the aviation impacts on climate change. To gain improved knowledge of contrail and contrail-induced cirrus cloud formation, understanding of contrail ice particle formation immediately after aircraft engines is needed. Despite many efforts spent in modeling the microphysics of ice crystal formation in jet regime (with a plume age <5 s), systematic understanding of parametric effects of variables affecting contrail ice particle formation is still limited. In this work, we apply a microphysical parcel modeling approach to study contrail ice particle formation in near-field aircraft plumes up to 1000 m downstream of an aircraft engine in the soot-rich regime (soot number emission index >1×10<sup>15</sup> (kg-fuel)<sup>−1</sup>) at cruise. The effects of dilution history, ion-mediated nucleation, ambient relative humidity, fuel sulfur contents, and initial soot emissions were investigated. Our simulation results suggest that ice particles are mainly formed by water condensation on emitted soot particles. The growth of ice coated soot particles is driven by water vapor emissions in the first 1000 m and by ambient relative humidity afterwards. The presence of chemi-ions does not significantly contribute to the formation of ice particles in the soot-rich regime, and the effect of fuel sulfur contents is small over the range typical of standard jet fuels. The initial properties of soot emissions play the most critical role, and our calculations suggest that higher number concentration and smaller size of contrail particle nuclei may be able to effectively suppress the formation of contrail ice particles. Further modeling and experimental studies are needed to verify if our findings can provide a possible approach for contrail mitigation.
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spelling doaj.art-63bb5e00dd37480fab6aaff960b788722022-12-21T19:51:29ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242010-04-011073261327210.5194/acp-10-3261-2010Parametric studies of contrail ice particle formation in jet regime using microphysical parcel modelingH.-W. WongR. C. Miake-LyeCondensation trails (contrails) formed from water vapor emissions behind aircraft engines are the most uncertain components of the aviation impacts on climate change. To gain improved knowledge of contrail and contrail-induced cirrus cloud formation, understanding of contrail ice particle formation immediately after aircraft engines is needed. Despite many efforts spent in modeling the microphysics of ice crystal formation in jet regime (with a plume age <5 s), systematic understanding of parametric effects of variables affecting contrail ice particle formation is still limited. In this work, we apply a microphysical parcel modeling approach to study contrail ice particle formation in near-field aircraft plumes up to 1000 m downstream of an aircraft engine in the soot-rich regime (soot number emission index >1×10<sup>15</sup> (kg-fuel)<sup>−1</sup>) at cruise. The effects of dilution history, ion-mediated nucleation, ambient relative humidity, fuel sulfur contents, and initial soot emissions were investigated. Our simulation results suggest that ice particles are mainly formed by water condensation on emitted soot particles. The growth of ice coated soot particles is driven by water vapor emissions in the first 1000 m and by ambient relative humidity afterwards. The presence of chemi-ions does not significantly contribute to the formation of ice particles in the soot-rich regime, and the effect of fuel sulfur contents is small over the range typical of standard jet fuels. The initial properties of soot emissions play the most critical role, and our calculations suggest that higher number concentration and smaller size of contrail particle nuclei may be able to effectively suppress the formation of contrail ice particles. Further modeling and experimental studies are needed to verify if our findings can provide a possible approach for contrail mitigation.http://www.atmos-chem-phys.net/10/3261/2010/acp-10-3261-2010.pdf
spellingShingle H.-W. Wong
R. C. Miake-Lye
Parametric studies of contrail ice particle formation in jet regime using microphysical parcel modeling
Atmospheric Chemistry and Physics
title Parametric studies of contrail ice particle formation in jet regime using microphysical parcel modeling
title_full Parametric studies of contrail ice particle formation in jet regime using microphysical parcel modeling
title_fullStr Parametric studies of contrail ice particle formation in jet regime using microphysical parcel modeling
title_full_unstemmed Parametric studies of contrail ice particle formation in jet regime using microphysical parcel modeling
title_short Parametric studies of contrail ice particle formation in jet regime using microphysical parcel modeling
title_sort parametric studies of contrail ice particle formation in jet regime using microphysical parcel modeling
url http://www.atmos-chem-phys.net/10/3261/2010/acp-10-3261-2010.pdf
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AT rcmiakelye parametricstudiesofcontrailiceparticleformationinjetregimeusingmicrophysicalparcelmodeling