Design and direct preparation of a novel silicon carbide support for zeolite membrane

Abstract The support for the membrane is the basis for the preparation and application of the zeolite membrane. Moreover, its cost and properties directly determine the performance of the zeolite membrane and its industrial applications. A novel porous silicon carbide (SiC) support for zeolite membr...

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Main Authors: Gangling Chen, Jianying Zhang, Miaomiao Geng, Jaka Sunarso, Ngie Hing Wong, Tianlin Ma, Yujie Wang, Guihua Chen
Format: Article
Language:English
Published: SpringerOpen 2022-10-01
Series:Applied Water Science
Subjects:
Online Access:https://doi.org/10.1007/s13201-022-01779-0
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author Gangling Chen
Jianying Zhang
Miaomiao Geng
Jaka Sunarso
Ngie Hing Wong
Tianlin Ma
Yujie Wang
Guihua Chen
author_facet Gangling Chen
Jianying Zhang
Miaomiao Geng
Jaka Sunarso
Ngie Hing Wong
Tianlin Ma
Yujie Wang
Guihua Chen
author_sort Gangling Chen
collection DOAJ
description Abstract The support for the membrane is the basis for the preparation and application of the zeolite membrane. Moreover, its cost and properties directly determine the performance of the zeolite membrane and its industrial applications. A novel porous silicon carbide (SiC) support for zeolite membrane bonded with needle-like mullite (3Al2O3·2SiO2) was prepared using SiC powders as the raw material and kaolin, Al(OH)3, and AlF3 as the needle-like mullite precursor additives via an in situ high-temperature reactions in an air atmosphere. Effects of the support material composition and the sintering temperature on the sintering behavior, pore structure, permeability, and microstructure of the resultant supports were extensively investigated. The needle-like mullite formation consumed silicon oxide (SiO2) and generated a rigid skeleton structure with a good pore structure and bonding phase. Hence, the porous SiC support exhibited high porosity, with relatively large pore size and mechanical strength, which helped improve the support performance. Notably, the porous SiC support sintered at 1480 °C with in situ inter-particle needle-like mullite bonding exhibited excellent filtration and permeability performance. The porous support materials and methods used in this work are suitable for designing and preparing a novel porous SiC support for zeolite membranes.
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spelling doaj.art-6518ea671cd9480fa6ac308a5f09b6002022-12-22T04:31:55ZengSpringerOpenApplied Water Science2190-54872190-54952022-10-0112111910.1007/s13201-022-01779-0Design and direct preparation of a novel silicon carbide support for zeolite membraneGangling Chen0Jianying Zhang1Miaomiao Geng2Jaka Sunarso3Ngie Hing Wong4Tianlin Ma5Yujie Wang6Guihua Chen7School of Material Science and Chemical Engineering, Chuzhou UniversitySchool of Material Science and Chemical Engineering, Chuzhou UniversitySchool of Material Science and Chemical Engineering, Chuzhou UniversityResearch Centre for Sustainable Technologies, Faculty of Engineering, Computing and Science, Swinburne University of TechnologyResearch Centre for Sustainable Technologies, Faculty of Engineering, Computing and Science, Swinburne University of TechnologySchool of Material Science and Chemical Engineering, Chuzhou UniversitySchool of Material Science and Chemical Engineering, Chuzhou UniversitySchool of Pharmaceutical and Material Engineering, Taizhou UniversityAbstract The support for the membrane is the basis for the preparation and application of the zeolite membrane. Moreover, its cost and properties directly determine the performance of the zeolite membrane and its industrial applications. A novel porous silicon carbide (SiC) support for zeolite membrane bonded with needle-like mullite (3Al2O3·2SiO2) was prepared using SiC powders as the raw material and kaolin, Al(OH)3, and AlF3 as the needle-like mullite precursor additives via an in situ high-temperature reactions in an air atmosphere. Effects of the support material composition and the sintering temperature on the sintering behavior, pore structure, permeability, and microstructure of the resultant supports were extensively investigated. The needle-like mullite formation consumed silicon oxide (SiO2) and generated a rigid skeleton structure with a good pore structure and bonding phase. Hence, the porous SiC support exhibited high porosity, with relatively large pore size and mechanical strength, which helped improve the support performance. Notably, the porous SiC support sintered at 1480 °C with in situ inter-particle needle-like mullite bonding exhibited excellent filtration and permeability performance. The porous support materials and methods used in this work are suitable for designing and preparing a novel porous SiC support for zeolite membranes.https://doi.org/10.1007/s13201-022-01779-0Needle-like mulliteSilicon carbideZeolite membrane support
spellingShingle Gangling Chen
Jianying Zhang
Miaomiao Geng
Jaka Sunarso
Ngie Hing Wong
Tianlin Ma
Yujie Wang
Guihua Chen
Design and direct preparation of a novel silicon carbide support for zeolite membrane
Applied Water Science
Needle-like mullite
Silicon carbide
Zeolite membrane support
title Design and direct preparation of a novel silicon carbide support for zeolite membrane
title_full Design and direct preparation of a novel silicon carbide support for zeolite membrane
title_fullStr Design and direct preparation of a novel silicon carbide support for zeolite membrane
title_full_unstemmed Design and direct preparation of a novel silicon carbide support for zeolite membrane
title_short Design and direct preparation of a novel silicon carbide support for zeolite membrane
title_sort design and direct preparation of a novel silicon carbide support for zeolite membrane
topic Needle-like mullite
Silicon carbide
Zeolite membrane support
url https://doi.org/10.1007/s13201-022-01779-0
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