Schrödinger's Red Beyond 65,000 Pixel‐Per‐Inch by Multipolar Interaction in Freeform Meta‐Atom through Efficient Neural Optimizer

Abstract Freeform nanostructures have the potential to support complex resonances and their interactions, which are crucial for achieving desired spectral responses. However, the design optimization of such structures is nontrivial and computationally intensive. Furthermore, the current “black box”...

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Główni autorzy: Ronghui Lin, Vytautas Valuckas, Thi Thu Ha Do, Arash Nemati, Arseniy I. Kuznetsov, Jinghua Teng, Son Tung Ha
Format: Artykuł
Język:English
Wydane: Wiley 2024-04-01
Seria:Advanced Science
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Dostęp online:https://doi.org/10.1002/advs.202303929
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author Ronghui Lin
Vytautas Valuckas
Thi Thu Ha Do
Arash Nemati
Arseniy I. Kuznetsov
Jinghua Teng
Son Tung Ha
author_facet Ronghui Lin
Vytautas Valuckas
Thi Thu Ha Do
Arash Nemati
Arseniy I. Kuznetsov
Jinghua Teng
Son Tung Ha
author_sort Ronghui Lin
collection DOAJ
description Abstract Freeform nanostructures have the potential to support complex resonances and their interactions, which are crucial for achieving desired spectral responses. However, the design optimization of such structures is nontrivial and computationally intensive. Furthermore, the current “black box” design approaches for freeform nanostructures often neglect the underlying physics. Here, a hybrid data‐efficient neural optimizer for resonant nanostructures by combining a reinforcement learning algorithm and Powell's local optimization technique is presented. As a case study, silicon nanostructures with a highly‐saturated red color are designed and experimentally demonstrated. Specifically, color coordinates of (0.677, 0.304) in the International Commission on Illumination (CIE) chromaticity diagram – close to the ideal Schrödinger's red, with polarization independence, high reflectance (>85%), and a large viewing angle (i.e., up to ± 25°) is achieved. The remarkable performance is attributed to underlying generalized multipolar interferences within each nanostructure rather than the collective array effects. Based on that, pixel size down to ≈400 nm, corresponding to a printing resolution of 65000 pixels per inch is demonstrated. Moreover, the proposed design model requires only ≈300 iterations to effectively search a thirteen‐dimensional (13D) design space – an order of magnitude more efficient than the previously reported approaches. The work significantly extends the free‐form optical design toolbox for high‐performance flat‐optical components and metadevices.
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spelling doaj.art-65715dba58174dc8b92cf4a2e52fbb2d2024-04-02T20:51:56ZengWileyAdvanced Science2198-38442024-04-011113n/an/a10.1002/advs.202303929Schrödinger's Red Beyond 65,000 Pixel‐Per‐Inch by Multipolar Interaction in Freeform Meta‐Atom through Efficient Neural OptimizerRonghui Lin0Vytautas Valuckas1Thi Thu Ha Do2Arash Nemati3Arseniy I. Kuznetsov4Jinghua Teng5Son Tung Ha6Agency for Science, Technology and Research (A*STAR) Institute of Materials Research and Engineering (IMRE) 2 Fusionopolis Way, Innovis #08‐03 Singapore 138634 Republic of SingaporeAgency for Science, Technology and Research (A*STAR) Institute of Materials Research and Engineering (IMRE) 2 Fusionopolis Way, Innovis #08‐03 Singapore 138634 Republic of SingaporeAgency for Science, Technology and Research (A*STAR) Institute of Materials Research and Engineering (IMRE) 2 Fusionopolis Way, Innovis #08‐03 Singapore 138634 Republic of SingaporeAgency for Science, Technology and Research (A*STAR) Institute of Materials Research and Engineering (IMRE) 2 Fusionopolis Way, Innovis #08‐03 Singapore 138634 Republic of SingaporeAgency for Science, Technology and Research (A*STAR) Institute of Materials Research and Engineering (IMRE) 2 Fusionopolis Way, Innovis #08‐03 Singapore 138634 Republic of SingaporeAgency for Science, Technology and Research (A*STAR) Institute of Materials Research and Engineering (IMRE) 2 Fusionopolis Way, Innovis #08‐03 Singapore 138634 Republic of SingaporeAgency for Science, Technology and Research (A*STAR) Institute of Materials Research and Engineering (IMRE) 2 Fusionopolis Way, Innovis #08‐03 Singapore 138634 Republic of SingaporeAbstract Freeform nanostructures have the potential to support complex resonances and their interactions, which are crucial for achieving desired spectral responses. However, the design optimization of such structures is nontrivial and computationally intensive. Furthermore, the current “black box” design approaches for freeform nanostructures often neglect the underlying physics. Here, a hybrid data‐efficient neural optimizer for resonant nanostructures by combining a reinforcement learning algorithm and Powell's local optimization technique is presented. As a case study, silicon nanostructures with a highly‐saturated red color are designed and experimentally demonstrated. Specifically, color coordinates of (0.677, 0.304) in the International Commission on Illumination (CIE) chromaticity diagram – close to the ideal Schrödinger's red, with polarization independence, high reflectance (>85%), and a large viewing angle (i.e., up to ± 25°) is achieved. The remarkable performance is attributed to underlying generalized multipolar interferences within each nanostructure rather than the collective array effects. Based on that, pixel size down to ≈400 nm, corresponding to a printing resolution of 65000 pixels per inch is demonstrated. Moreover, the proposed design model requires only ≈300 iterations to effectively search a thirteen‐dimensional (13D) design space – an order of magnitude more efficient than the previously reported approaches. The work significantly extends the free‐form optical design toolbox for high‐performance flat‐optical components and metadevices.https://doi.org/10.1002/advs.202303929machine learningmetasurfacesmonte Carlo tree searchmultipole interferencestructural colors
spellingShingle Ronghui Lin
Vytautas Valuckas
Thi Thu Ha Do
Arash Nemati
Arseniy I. Kuznetsov
Jinghua Teng
Son Tung Ha
Schrödinger's Red Beyond 65,000 Pixel‐Per‐Inch by Multipolar Interaction in Freeform Meta‐Atom through Efficient Neural Optimizer
Advanced Science
machine learning
metasurfaces
monte Carlo tree search
multipole interference
structural colors
title Schrödinger's Red Beyond 65,000 Pixel‐Per‐Inch by Multipolar Interaction in Freeform Meta‐Atom through Efficient Neural Optimizer
title_full Schrödinger's Red Beyond 65,000 Pixel‐Per‐Inch by Multipolar Interaction in Freeform Meta‐Atom through Efficient Neural Optimizer
title_fullStr Schrödinger's Red Beyond 65,000 Pixel‐Per‐Inch by Multipolar Interaction in Freeform Meta‐Atom through Efficient Neural Optimizer
title_full_unstemmed Schrödinger's Red Beyond 65,000 Pixel‐Per‐Inch by Multipolar Interaction in Freeform Meta‐Atom through Efficient Neural Optimizer
title_short Schrödinger's Red Beyond 65,000 Pixel‐Per‐Inch by Multipolar Interaction in Freeform Meta‐Atom through Efficient Neural Optimizer
title_sort schrodinger s red beyond 65 000 pixel per inch by multipolar interaction in freeform meta atom through efficient neural optimizer
topic machine learning
metasurfaces
monte Carlo tree search
multipole interference
structural colors
url https://doi.org/10.1002/advs.202303929
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