Electrode Impact on the Electrical Breakdown of Dielectric Elastomer Thin Films

Dielectric Elastomer Actuators (DEAs) enable the realization of energy-efficient and compact actuator systems. DEAs operate at the kilovolt range with typically microampere-level currents and hence minimize thermal losses in comparison to low voltage/high current actuators such as shape memory alloy...

Full description

Bibliographic Details
Main Authors: Bettina Fasolt, Fabio Beco Albuquerque, Jonas Hubertus, Günter Schultes, Herbert Shea, Stefan Seelecke
Format: Article
Language:English
Published: MDPI AG 2023-10-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/15/20/4071
_version_ 1797572462777466880
author Bettina Fasolt
Fabio Beco Albuquerque
Jonas Hubertus
Günter Schultes
Herbert Shea
Stefan Seelecke
author_facet Bettina Fasolt
Fabio Beco Albuquerque
Jonas Hubertus
Günter Schultes
Herbert Shea
Stefan Seelecke
author_sort Bettina Fasolt
collection DOAJ
description Dielectric Elastomer Actuators (DEAs) enable the realization of energy-efficient and compact actuator systems. DEAs operate at the kilovolt range with typically microampere-level currents and hence minimize thermal losses in comparison to low voltage/high current actuators such as shape memory alloys or solenoids. The main limiting factor for reaching high energy density in high voltage applications is dielectric breakdown. In previous investigations on silicone-based thin films, we reported that not only do environmental conditions and film parameters such as pre-stretch play an important role but that electrode composition also has a significant impact on the breakdown behavior. In this paper, we present a comprehensive study of electrical breakdown on thin silicone films coated with electrodes manufactured by five different methods: screen printing, inkjet printing, pad printing, gold sputtering, and nickel sputtering. For each method, breakdown was studied under environmental conditions ranging from 1 °C to 80 °C and 10% to 90% relative humidity. The effect of different manufacturing methods was analyzed as was the influence of parameters such as solvents, silicone content, and the particle processing method. The breakdown field increases with increasing temperature and decreases with increasing humidity for all electrode types. The stiffer metal electrodes have a higher breakdown field than the carbon-based electrodes, for which particle size also plays a large role.
first_indexed 2024-03-10T20:56:38Z
format Article
id doaj.art-65d82bcbd6714a009276e16a78c54254
institution Directory Open Access Journal
issn 2073-4360
language English
last_indexed 2024-03-10T20:56:38Z
publishDate 2023-10-01
publisher MDPI AG
record_format Article
series Polymers
spelling doaj.art-65d82bcbd6714a009276e16a78c542542023-11-19T17:50:44ZengMDPI AGPolymers2073-43602023-10-011520407110.3390/polym15204071Electrode Impact on the Electrical Breakdown of Dielectric Elastomer Thin FilmsBettina Fasolt0Fabio Beco Albuquerque1Jonas Hubertus2Günter Schultes3Herbert Shea4Stefan Seelecke5Intelligent Material Systems Lab, Center for Mechatronics and Automation Technology, ZeMA gGmbH, DE-66121 Saarbrücken, GermanyLMTS Soft Transducers Laboratory, EPFL Ecole Polytechnique Fédérale de Lausanne, CH-2002 Neuchâtel, SwitzerlandSensors and Thin Film Group, University of Applied Sciences, DE-66117 Saarbrücken, GermanySensors and Thin Film Group, University of Applied Sciences, DE-66117 Saarbrücken, GermanyLMTS Soft Transducers Laboratory, EPFL Ecole Polytechnique Fédérale de Lausanne, CH-2002 Neuchâtel, SwitzerlandIntelligent Material Systems Lab, Department of Systems Engineering, Department of Materials Science and Engineering, Saarland University, DE-66121 Saarbrücken, GermanyDielectric Elastomer Actuators (DEAs) enable the realization of energy-efficient and compact actuator systems. DEAs operate at the kilovolt range with typically microampere-level currents and hence minimize thermal losses in comparison to low voltage/high current actuators such as shape memory alloys or solenoids. The main limiting factor for reaching high energy density in high voltage applications is dielectric breakdown. In previous investigations on silicone-based thin films, we reported that not only do environmental conditions and film parameters such as pre-stretch play an important role but that electrode composition also has a significant impact on the breakdown behavior. In this paper, we present a comprehensive study of electrical breakdown on thin silicone films coated with electrodes manufactured by five different methods: screen printing, inkjet printing, pad printing, gold sputtering, and nickel sputtering. For each method, breakdown was studied under environmental conditions ranging from 1 °C to 80 °C and 10% to 90% relative humidity. The effect of different manufacturing methods was analyzed as was the influence of parameters such as solvents, silicone content, and the particle processing method. The breakdown field increases with increasing temperature and decreases with increasing humidity for all electrode types. The stiffer metal electrodes have a higher breakdown field than the carbon-based electrodes, for which particle size also plays a large role.https://www.mdpi.com/2073-4360/15/20/4071dielectric breakdown testelectrode manufacturing methodsinfluence electrodessilicone filmscarbon blackenvironmental conditions
spellingShingle Bettina Fasolt
Fabio Beco Albuquerque
Jonas Hubertus
Günter Schultes
Herbert Shea
Stefan Seelecke
Electrode Impact on the Electrical Breakdown of Dielectric Elastomer Thin Films
Polymers
dielectric breakdown test
electrode manufacturing methods
influence electrodes
silicone films
carbon black
environmental conditions
title Electrode Impact on the Electrical Breakdown of Dielectric Elastomer Thin Films
title_full Electrode Impact on the Electrical Breakdown of Dielectric Elastomer Thin Films
title_fullStr Electrode Impact on the Electrical Breakdown of Dielectric Elastomer Thin Films
title_full_unstemmed Electrode Impact on the Electrical Breakdown of Dielectric Elastomer Thin Films
title_short Electrode Impact on the Electrical Breakdown of Dielectric Elastomer Thin Films
title_sort electrode impact on the electrical breakdown of dielectric elastomer thin films
topic dielectric breakdown test
electrode manufacturing methods
influence electrodes
silicone films
carbon black
environmental conditions
url https://www.mdpi.com/2073-4360/15/20/4071
work_keys_str_mv AT bettinafasolt electrodeimpactontheelectricalbreakdownofdielectricelastomerthinfilms
AT fabiobecoalbuquerque electrodeimpactontheelectricalbreakdownofdielectricelastomerthinfilms
AT jonashubertus electrodeimpactontheelectricalbreakdownofdielectricelastomerthinfilms
AT gunterschultes electrodeimpactontheelectricalbreakdownofdielectricelastomerthinfilms
AT herbertshea electrodeimpactontheelectricalbreakdownofdielectricelastomerthinfilms
AT stefanseelecke electrodeimpactontheelectricalbreakdownofdielectricelastomerthinfilms