A Biomimetic Lignocellulose Aerogel-Based Membrane for Efficient Phenol Extraction from Water

Rapid extraction and concentration systems based on green materials such as cellulose or lignin are promising. However, there is still a need to optimize the material properties and production processes. Unlike conventional cellulose or lignin sorbent materials, aquatic reed root cells can concentra...

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Main Authors: Peipei Liu, Chunling Zheng, Zhong Yao, Fang Zhang
Format: Article
Language:English
Published: MDPI AG 2024-01-01
Series:Gels
Subjects:
Online Access:https://www.mdpi.com/2310-2861/10/1/59
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author Peipei Liu
Chunling Zheng
Zhong Yao
Fang Zhang
author_facet Peipei Liu
Chunling Zheng
Zhong Yao
Fang Zhang
author_sort Peipei Liu
collection DOAJ
description Rapid extraction and concentration systems based on green materials such as cellulose or lignin are promising. However, there is still a need to optimize the material properties and production processes. Unlike conventional cellulose or lignin sorbent materials, aquatic reed root cells can concentrate external organic pollutants in the water and accumulate them in the plant. Inspired by this, a new nanocellulose–lignin aerogel (NLAG) was designed, in which nanocellulose was used as a substrate and lignin and polyamide epoxy chloropropane were used to crosslink cellulose in order to enhance the strength of the NLGA, resulting in good mechanical stability and water–oil amphiphilic properties. In practical applications, the organic membrane on the NLAG can transport organic pollutants from water to the NLAG, where they are immobilized. This is evidenced by the fact that the aerogel can remove more than 93% of exogenous phenol within a few minutes, highly enriching it inside. In addition, the aerogel facilitates filtration and shape recovery for reuse. This work establishes a novel biopolymer–aerogel-based extraction system with the advantages of sustainability, high efficiency, stability, and easy detachability, which are hard for the traditional adsorbent materials to attain.
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spelling doaj.art-6647a4ae4c774ccf93592d56c95709ca2024-01-26T16:40:11ZengMDPI AGGels2310-28612024-01-011015910.3390/gels10010059A Biomimetic Lignocellulose Aerogel-Based Membrane for Efficient Phenol Extraction from WaterPeipei Liu0Chunling Zheng1Zhong Yao2Fang Zhang3College of Food Science and Light Industry, Nanjing Tech University, Nanjing 211800, ChinaCollege of Food Science and Light Industry, Nanjing Tech University, Nanjing 211800, ChinaCollege of Food Science and Light Industry, Nanjing Tech University, Nanjing 211800, ChinaCollege of Food Science and Light Industry, Nanjing Tech University, Nanjing 211800, ChinaRapid extraction and concentration systems based on green materials such as cellulose or lignin are promising. However, there is still a need to optimize the material properties and production processes. Unlike conventional cellulose or lignin sorbent materials, aquatic reed root cells can concentrate external organic pollutants in the water and accumulate them in the plant. Inspired by this, a new nanocellulose–lignin aerogel (NLAG) was designed, in which nanocellulose was used as a substrate and lignin and polyamide epoxy chloropropane were used to crosslink cellulose in order to enhance the strength of the NLGA, resulting in good mechanical stability and water–oil amphiphilic properties. In practical applications, the organic membrane on the NLAG can transport organic pollutants from water to the NLAG, where they are immobilized. This is evidenced by the fact that the aerogel can remove more than 93% of exogenous phenol within a few minutes, highly enriching it inside. In addition, the aerogel facilitates filtration and shape recovery for reuse. This work establishes a novel biopolymer–aerogel-based extraction system with the advantages of sustainability, high efficiency, stability, and easy detachability, which are hard for the traditional adsorbent materials to attain.https://www.mdpi.com/2310-2861/10/1/59biomimetic membranecellulose–lignin aerogelphenolextraction and enrichment
spellingShingle Peipei Liu
Chunling Zheng
Zhong Yao
Fang Zhang
A Biomimetic Lignocellulose Aerogel-Based Membrane for Efficient Phenol Extraction from Water
Gels
biomimetic membrane
cellulose–lignin aerogel
phenol
extraction and enrichment
title A Biomimetic Lignocellulose Aerogel-Based Membrane for Efficient Phenol Extraction from Water
title_full A Biomimetic Lignocellulose Aerogel-Based Membrane for Efficient Phenol Extraction from Water
title_fullStr A Biomimetic Lignocellulose Aerogel-Based Membrane for Efficient Phenol Extraction from Water
title_full_unstemmed A Biomimetic Lignocellulose Aerogel-Based Membrane for Efficient Phenol Extraction from Water
title_short A Biomimetic Lignocellulose Aerogel-Based Membrane for Efficient Phenol Extraction from Water
title_sort biomimetic lignocellulose aerogel based membrane for efficient phenol extraction from water
topic biomimetic membrane
cellulose–lignin aerogel
phenol
extraction and enrichment
url https://www.mdpi.com/2310-2861/10/1/59
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