Probing multiphoton light-induced molecular potentials
Conical intersections, a hallmark of polyatomic molecules, can be induced with light, leading to new reaction pathways. Here, the authors show that intense fields can create complex, beyond-conical intersections even in diatomics, resulting in an unexpected angular distribution of fragment ions.
Main Authors: | , , , , , , , , , |
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Format: | Article |
Language: | English |
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Nature Portfolio
2020-05-01
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Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-020-16422-2 |
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author | M. Kübel M. Spanner Z. Dube A. Yu. Naumov S. Chelkowski A. D. Bandrauk M. J. J. Vrakking P. B. Corkum D. M. Villeneuve A. Staudte |
author_facet | M. Kübel M. Spanner Z. Dube A. Yu. Naumov S. Chelkowski A. D. Bandrauk M. J. J. Vrakking P. B. Corkum D. M. Villeneuve A. Staudte |
author_sort | M. Kübel |
collection | DOAJ |
description | Conical intersections, a hallmark of polyatomic molecules, can be induced with light, leading to new reaction pathways. Here, the authors show that intense fields can create complex, beyond-conical intersections even in diatomics, resulting in an unexpected angular distribution of fragment ions. |
first_indexed | 2024-12-19T04:14:20Z |
format | Article |
id | doaj.art-66c90847b61c4555a424eec408aff96a |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-12-19T04:14:20Z |
publishDate | 2020-05-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-66c90847b61c4555a424eec408aff96a2022-12-21T20:36:21ZengNature PortfolioNature Communications2041-17232020-05-011111810.1038/s41467-020-16422-2Probing multiphoton light-induced molecular potentialsM. Kübel0M. Spanner1Z. Dube2A. Yu. Naumov3S. Chelkowski4A. D. Bandrauk5M. J. J. Vrakking6P. B. Corkum7D. M. Villeneuve8A. Staudte9Joint Attosecond Science Laboratory, National Research Council and University of Ottawa, 100 Sussex DriveJoint Attosecond Science Laboratory, National Research Council and University of Ottawa, 100 Sussex DriveJoint Attosecond Science Laboratory, National Research Council and University of Ottawa, 100 Sussex DriveJoint Attosecond Science Laboratory, National Research Council and University of Ottawa, 100 Sussex DriveLaboratoire de Chimie Théoretique, Faculté des Sciences, Université de SherbrookeLaboratoire de Chimie Théoretique, Faculté des Sciences, Université de SherbrookeMax-Born-Institute, Max-Born-Straße 2AJoint Attosecond Science Laboratory, National Research Council and University of Ottawa, 100 Sussex DriveJoint Attosecond Science Laboratory, National Research Council and University of Ottawa, 100 Sussex DriveJoint Attosecond Science Laboratory, National Research Council and University of Ottawa, 100 Sussex DriveConical intersections, a hallmark of polyatomic molecules, can be induced with light, leading to new reaction pathways. Here, the authors show that intense fields can create complex, beyond-conical intersections even in diatomics, resulting in an unexpected angular distribution of fragment ions.https://doi.org/10.1038/s41467-020-16422-2 |
spellingShingle | M. Kübel M. Spanner Z. Dube A. Yu. Naumov S. Chelkowski A. D. Bandrauk M. J. J. Vrakking P. B. Corkum D. M. Villeneuve A. Staudte Probing multiphoton light-induced molecular potentials Nature Communications |
title | Probing multiphoton light-induced molecular potentials |
title_full | Probing multiphoton light-induced molecular potentials |
title_fullStr | Probing multiphoton light-induced molecular potentials |
title_full_unstemmed | Probing multiphoton light-induced molecular potentials |
title_short | Probing multiphoton light-induced molecular potentials |
title_sort | probing multiphoton light induced molecular potentials |
url | https://doi.org/10.1038/s41467-020-16422-2 |
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