Engineering helimagnetism in MnSi thin films

Magnetic skyrmion materials have the great advantage of a robust topological magnetic structure, which makes them stable against the superparamagnetic effect and therefore a candidate for the next-generation of spintronic memory devices. Bulk MnSi, with an ordering temperature of 29.5 K, is a typica...

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Main Authors: S. L. Zhang, R. Chalasani, A. A. Baker, N.-J. Steinke, A. I. Figueroa, A. Kohn, G. van der Laan, T. Hesjedal
Format: Article
Language:English
Published: AIP Publishing LLC 2016-01-01
Series:AIP Advances
Online Access:http://dx.doi.org/10.1063/1.4941316
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author S. L. Zhang
R. Chalasani
A. A. Baker
N.-J. Steinke
A. I. Figueroa
A. Kohn
G. van der Laan
T. Hesjedal
author_facet S. L. Zhang
R. Chalasani
A. A. Baker
N.-J. Steinke
A. I. Figueroa
A. Kohn
G. van der Laan
T. Hesjedal
author_sort S. L. Zhang
collection DOAJ
description Magnetic skyrmion materials have the great advantage of a robust topological magnetic structure, which makes them stable against the superparamagnetic effect and therefore a candidate for the next-generation of spintronic memory devices. Bulk MnSi, with an ordering temperature of 29.5 K, is a typical skyrmion system with a propagation vector periodicity of ∼18 nm. One crucial prerequisite for any kind of application, however, is the observation and precise control of skyrmions in thin films at room-temperature. Strain in epitaxial MnSi thin films is known to raise the transition temperature to 43 K. Here we show, using magnetometry and x-ray spectroscopy, that the transition temperature can be raised further through proximity coupling to a ferromagnetic layer. Similarly, the external field required to stabilize the helimagnetic phase is lowered. Transmission electron microscopy with element-sensitive detection is used to explore the structural origin of ferromagnetism in these Mn-doped substrates. Our work suggests that an artificial pinning layer, not limited to the MnSi/Si system, may enable room temperature, zero-field skyrmion thin-film systems, thereby opening the door to device applications.
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spelling doaj.art-66c9441d105e4bada3114bd3e9f634912022-12-22T03:15:11ZengAIP Publishing LLCAIP Advances2158-32262016-01-0161015217015217-810.1063/1.4941316069601ADVEngineering helimagnetism in MnSi thin filmsS. L. Zhang0R. Chalasani1A. A. Baker2N.-J. Steinke3A. I. Figueroa4A. Kohn5G. van der Laan6T. Hesjedal7Department of Physics, Clarendon Laboratory, University of Oxford, Oxford, OX1 3PU, United KingdomDepartment of Materials Science and Engineering, Tel Aviv University, Ramat Aviv 6997801, Tel Aviv, IsraelDepartment of Physics, Clarendon Laboratory, University of Oxford, Oxford, OX1 3PU, United KingdomISIS, Harwell Science and Innovation Campus, Didcot, Oxfordshire, OX11 0QX, United KingdomMagnetic Spectroscopy Group, Diamond Light Source, Didcot, OX11 0DE, United KingdomDepartment of Materials Science and Engineering, Tel Aviv University, Ramat Aviv 6997801, Tel Aviv, IsraelMagnetic Spectroscopy Group, Diamond Light Source, Didcot, OX11 0DE, United KingdomDepartment of Physics, Clarendon Laboratory, University of Oxford, Oxford, OX1 3PU, United KingdomMagnetic skyrmion materials have the great advantage of a robust topological magnetic structure, which makes them stable against the superparamagnetic effect and therefore a candidate for the next-generation of spintronic memory devices. Bulk MnSi, with an ordering temperature of 29.5 K, is a typical skyrmion system with a propagation vector periodicity of ∼18 nm. One crucial prerequisite for any kind of application, however, is the observation and precise control of skyrmions in thin films at room-temperature. Strain in epitaxial MnSi thin films is known to raise the transition temperature to 43 K. Here we show, using magnetometry and x-ray spectroscopy, that the transition temperature can be raised further through proximity coupling to a ferromagnetic layer. Similarly, the external field required to stabilize the helimagnetic phase is lowered. Transmission electron microscopy with element-sensitive detection is used to explore the structural origin of ferromagnetism in these Mn-doped substrates. Our work suggests that an artificial pinning layer, not limited to the MnSi/Si system, may enable room temperature, zero-field skyrmion thin-film systems, thereby opening the door to device applications.http://dx.doi.org/10.1063/1.4941316
spellingShingle S. L. Zhang
R. Chalasani
A. A. Baker
N.-J. Steinke
A. I. Figueroa
A. Kohn
G. van der Laan
T. Hesjedal
Engineering helimagnetism in MnSi thin films
AIP Advances
title Engineering helimagnetism in MnSi thin films
title_full Engineering helimagnetism in MnSi thin films
title_fullStr Engineering helimagnetism in MnSi thin films
title_full_unstemmed Engineering helimagnetism in MnSi thin films
title_short Engineering helimagnetism in MnSi thin films
title_sort engineering helimagnetism in mnsi thin films
url http://dx.doi.org/10.1063/1.4941316
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